Spectral dynamics of shift current in ferroelectric semiconductor SbSI
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Significance: Shift current is one of the bulk photovoltaic phenomena in the materials without inversion symmetry, originating from the geometric Berry phase of the constituting electron bands. This concept of photocurrent generation based on the real-space shift of the electron cloud on the short timescale of optical transition is distinct from that of conventional p–n junction photovoltaics, where the carriers are driven by the built-in Coulomb potential. We experimentally demonstrate for a ferroelectric polar semiconductor how the subpicosecond charge swing on the relevant chemical bond changes its dynamics while scanning the excitation photon energy across the bandgap. On the interband photoexcitation above the bandgap, a finite net charge flow is produced along the electrically polar direction.
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Shift currents can be traced to a local geometric property defined by the difference in Berry connection between bands participating in the optical transition.
“Shift currents, resulting from the real space coherent shift of electron density following photoexcitation42, can be traced to a local geometric property defined by the difference in Berry connection between bands participating in the optical transition86,87.”
From Ultrafast terahertz emission from emerging symmetry-broken materials (2023) · cites this paper as [87]
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- Authors
- Sotome, M., Nakamura, M., Fujioka, J., Ogino, M., Kaneko, Y., Morimoto, T., Zhang, Y., Kawasaki, M., Nagaosa, N., Tokura, Y., & Ogawa, N.
- Affiliations
- RIKEN Center for Emergent Matter Science (JP)
- Japan Science and Technology Agency (JP)
- The University of Tokyo (JP)
- University of California, Berkeley (US)
- Leibniz Institute for Solid State and Materials Research (DE)
- Corresponding author
- Sotome, M.
- ORCID
- Venue
- Proceedings of the National Academy of Sciences
- Publisher
- National Academy of Sciences
- Published
- 2019-01-22
- Volume
- 116
- Issue
- 6
- Pages
- 1929-1933
- ISSN
- 0027-8424 (ISSN-L)
- 1091-6490
- PMC
- PMC6369763
- OpenAlex
- W2785837563
- Cited by
- 138
- References
- 50
- Citations by year
- 2026: 16 · 2025: 17 · 2024: 18 · 2023: 14 · 2022: 20 · 2021: 15 · 2020: 25 · 2019: 12 · 2018: 1
- FWCI
- 7.91
- Type
- journal article
- Language
- en
- Open access
- hybrid
- doi.org
- Licence
- Locations
- Proceedings of the National Academy of Sciences (publishedVersion, cc-by-nc-nd)
- Europe PMC (PubMed Central) (publishedVersion, cc-by-nc-nd)
- PubMed Central (publishedVersion, cc-by-nc-nd)
- PubMed (publishedVersion)
- arXiv (Cornell University) (submittedVersion)
- OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
- RENATE (submittedVersion, cc-by-nc-nd)
- MPG.PuRe (Max Planck Society) (submittedVersion)
- arXiv (Cornell University)
- RENATE
- Funders
- MEXT | Japan Society for the Promotion of Science (24224009, 16K13705, 17H02914, 16H00981, 18K14155)
- MEXT | Japan Science and Technology Agency (JPMJPR16R5, JPMJPR15R5, JPMJPR17I3)
- Deutsche Forschungsgemeinschaft (SFB1143)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Topological Materials and Phenomena
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Terahertz technology and applications
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Keywords
- shift current, ferroelectric semiconductors, Berry connection, terahertz emission, ultrafast electron dynamics, interband transitions, inversion symmetry breaking, photoexcitation, spectral dynamics
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