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Development of high harmonic generation spectroscopy of organic molecules and biomolecules
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In this review we will discuss the topic of high order harmonic generation (HHG) from samples of organic and bio-molecules. The possibility to extract useful dynamical and structural information from the measurement of the HHG emission, a technique termed high harmonic generation spectroscopy (HHGS), will be the special focus of our discussions. We will begin by introducing the salient facts of HHG from atoms and simple molecules and explaining the principles behind HHGS. Next the technical difficulties associated with HHG from samples of organic molecules and biomolecules, principally the low sample density and the low ionization potential, will be examined. Then we will present some recent experiments where HHG spectra from samples of these molecules have been measured and discuss what has been learned from these measurements. Finally we will look at the future prospects for HHG spectroscopy of organic molecules, discussing some of the technical and in principle limits of the technique and methods that may ameliorate these limits.
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Lappas, D. G., & Marangos, J. P. (2000) · Journal of Physics B Atomic Molecular and Optical Physics · doi:10.1088/0953-4075/33/21/313 · Cited by 70
Self-citationNiikura, H., Wörner, H. J., Villeneuve, D. M., & Corkum, P. B. (2011) · Physical Review Letters · doi:10.1103/physrevlett.107.093004 · Cited by 69
Extension of high harmonic spectroscopy in molecules by a 1300 nm laser field
Torres, R., Siegel, T., Brugnera, L., Procino, I., Underwood, J. G., Altucci, C., Velotta, R., Springate, E., Froud, C. A., Turcu, I. C. E., et al. (2010) · Optics Express · doi:10.1364/oe.18.003174 · Cited by 66
Self-citationOpportunities for chiral discrimination using high harmonic generation in tailored laser fields
Smirnova, O. V., Mairesse, Y., & Patchkovskii, S. (2015) · Journal of Physics B Atomic Molecular and Optical Physics · doi:10.1088/0953-4075/48/23/234005 · Cited by 65
Enhanced high-order-harmonic generation in a carbon ablation plume
Ganeev, R. A., Witting, T., Hutchison, C. D. M., Frank, F., Redkin, P. V., Okell, W. A., Lei, D., Roschuk, T. R., Maier, S. A., Marangos, J. P., et al. (2012) · Physical Review A · doi:10.1103/physreva.85.015807 · Cited by 65
Self-citationSynchronized pulses generated at 20 eV and 90 eV for attosecond pump–probe experiments
Fabris, D., Witting, T., Okell, W. A., Walke, D., Matía-Hernando, P., Henkel, J., Barillot, T. R., Lein, M., Marangos, J. P., & Tisch, J. W. G. (2015) · Nature Photonics · doi:10.1038/nphoton.2015.77 · Cited by 63
Self-citationHigh-Order Harmonic Transient Grating Spectroscopy in a Molecular Jet
Mairesse, Y., Zeidler, D., Dudovich, N., Spanner, M., Levesque, J., Villeneuve, D. M., & Corkum, P. B. (2008) · Physical Review Letters · doi:10.1103/physrevlett.100.143903 · Cited by 63
Nuclear Dynamics in Polyatomic Molecules and High-Order Harmonic Generation
Patchkovskii, S. (2009) · Physical Review Letters · doi:10.1103/physrevlett.102.253602 · Cited by 62
Absolute Ionization Rates of Multielectron Transition Metal Atoms in Strong Infrared Laser Fields
Smits, M., de Lange, C. A., Stolow, A., & Rayner, D. M. (2004) · Physical Review Letters · doi:10.1103/physrevlett.93.213003 · Cited by 57
High-Order Harmonic Generation Spectroscopy of Correlation-Driven Electron Hole Dynamics
Leeuwenburgh, J., Cooper, B., Averbukh, V., Marangos, J. P., & Ivanov, M. (2013) · Physical Review Letters · doi:10.1103/physrevlett.111.123002 · Cited by 54
Self-citationCEP-stable, sub-6 fs, 300-kHz OPCPA system with more than 15 W of average power
Prinz, S., Haefner, M., Teisset, C. Y., Bessing, R., Michel, K., Lee, Y., Geng, X., Kim, S., Kim, D. E., Metzger, T., et al. (2015) · Optics Express · doi:10.1364/oe.23.001388 · Cited by 53
Single-Photon Laser-Enabled Auger Spectroscopy for Measuring Attosecond Electron-Hole Dynamics
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High harmonic generation spectroscopy of hydrocarbons
Vozzi, C., Torres, R., Negro, M., Brugnera, L., Siegel, T., Altucci, C., Velotta, R., Frassetto, F., Poletto, L., Villoresi, P., et al. (2010) · Applied Physics Letters · doi:10.1063/1.3526752 · Cited by 52
Self-citationAttosecond and XUV Physics: Ultrafast Dynamics and Spectroscopy
Vrakking, M. J. J. (2014) · Wiley eBooks · doi:10.1002/9783527677689.ch1 · Cited by 51
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Walters, Z. B., & Smirnova, O. V. (2010) · Journal of Physics B Atomic Molecular and Optical Physics · doi:10.1088/0953-4075/43/16/161002 · Cited by 50
Attosecond control of electron–ion recollision in high harmonic generation
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Vapour pressures and sublimation enthalpies of thymine and cytosine
Ferro, D., Bencivenni, L., Teghil, R., & Mastromarino, R. (1980) · Thermochimica Acta · doi:10.1016/0040-6031(80)87117-6 · Cited by 44
Pulse-length dependence of high-order harmonic generation in dissociating cyclic organic molecules
Hay, N., de Nalda, R., Halfmann, T., Mendham, K. J., Mason, M. B., Castillejo, M., & Marangos, J. P. (2000) · Physical Review A · doi:10.1103/physreva.62.041803 · Cited by 40
Self-citationHigh harmonic generation in butane and butadiene
Fraser, D. J., Hutchinson, M. H. R., Marangos, J. P., Shao, Y., Tisch, J. W. G., & Castillejo, M. (1995) · Journal of Physics B Atomic Molecular and Optical Physics · doi:10.1088/0953-4075/28/23/006 · Cited by 40
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Wörner, H. J., Bertrand, J. B., Corkum, P. B., & Villeneuve, D. M. (2010) · Physical Review Letters · doi:10.1103/physrevlett.105.103002 · Cited by 40
Kraus, P. M., & Wörner, H. J. (2013) · ChemPhysChem · doi:10.1002/cphc.201201022 · Cited by 37
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High-order harmonic generation in cyclic organic molecules
Hay, N., Castillejo, M., de Nalda, R., Springate, E., Mendham, K. J., & Marangos, J. P. (2000) · Physical Review A · doi:10.1103/physreva.61.053810 · Cited by 35
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Electron diffraction studies of supersonic jets. I. Apparatus and methods
Bartell, L. S., Heenan, R. K., & Nagashima, M. (1983) · The Journal of Chemical Physics · doi:10.1063/1.444546 · Cited by 30
Cooper, B., Kolorenč, P., Frasinski, L. J., Averbukh, V., & Marangos, J. P. (2014) · Faraday Discussions · doi:10.1039/c4fd00051j · Cited by 29
Self-citationElectron diffraction studies of supersonic jets. II. Formation of benzene clusters
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Comparison of high-order harmonic generation in uracil and thymine ablation plumes
Hutchison, C. D. M., Ganeev, R. A., Castillejo, M., Lopez-Quintas, I., Zaïr, A., Weber, S. J., McGrath, F., Abdelrahman, Z., Oppermann, M., Martı́n, M., et al. (2013) · Physical Chemistry Chemical Physics · doi:10.1039/c3cp00004d · Cited by 29
Self-citationDynamic Polarization in the Strong-Field Ionization of Small Metal Clusters
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Kajumba, N., Torres, R., Underwood, J. G., Robinson, J. S., Baker, S., Tisch, J. W. G., de Nalda, R., Bryan, W. A., Velotta, R., Altucci, C., et al. (2008) · New Journal of Physics · doi:10.1088/1367-2630/10/2/025008 · Cited by 28
Self-citationHigh-order harmonic generation from organic molecules in ultra-short pulses
Hay, N., de Nalda, R., Halfmann, T., Mendham, K. J., Mason, M. B., Castillejo, M., & Marangos, J. P. (2001) · The European Physical Journal D · doi:10.1007/s100530170221 · Cited by 28
Self-citationMeasuring the intensity and phase of high-order harmonic emission from aligned molecules
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Wong, M. C. H., Brichta, J.-P., & Bhardwaj, V. R. (2010) · Physical Review A · doi:10.1103/physreva.81.061402 · Cited by 24
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Altucci, C., Velotta, R., Marangos, J. P., Heesel, E., Springate, E., Pascolini, M., Poletto, L., Villoresi, P., Vozzi, C., Sansone, G., et al. (2005) · Physical Review A · doi:10.1103/physreva.71.013409 · Cited by 20
Self-citationEnhancement of high-order harmonic emission using attosecond pulse trains
Biegert, J., Heinrich, A., Hauri, C. P., Kornelis, W., Schlup, P., Anscombe, M., Schäfer, K. J., Gaarde, M. B., & Keller, U. (2005) · Civil War Book Review · Cited by 20
High-harmonic generation in H_2O
Wong, M., Brichta, J.-P., & Bhardwaj, V. R. (2010) · Optics Letters · doi:10.1364/ol.35.001947 · Cited by 18
Explosion of irradiated with a high-intensity femtosecond laser pulse
Hay, N., Springate, E., Mason, M. B., Tisch, J. W. G., Castillejo, M., & Marangos, J. P. (1999) · Journal of Physics B Atomic Molecular and Optical Physics · doi:10.1088/0953-4075/32/2/033 · Cited by 17
Self-citationLiu, B., He, Y., Malomed, B. A., Wang, X.-S., Kevrekidis, P. G., Wang, T., Leng, F.-C., Qiu, Z., & Wang, H. (2010) · Optics Letters · doi:10.1364/ol.35.001974 · Cited by 17
High-order harmonic generation in alkanes
Altucci, C., Velotta, R., Heesel, E., Springate, E., Marangos, J. P., Vozzi, C., Benedetti, E., Calegari, F., Sansone, G., Stagira, S., et al. (2006) · Physical Review A · doi:10.1103/physreva.73.043411 · Cited by 16
Self-citationSub-laser-cycle control of coupled electron–nuclear dynamics at a conical intersection
Richter, M., Bouakline, F., González‐Vázquez, J., Martínez‐Fernández, L., Corral, I., Patchkovskii, S., Morales, F., Ivanov, M., Martı́n, F., & Smirnova, O. V. (2015) · New Journal of Physics · doi:10.1088/1367-2630/17/11/113023 · Cited by 15
Short-Time Dynamics at a Conical Intersection in High-Harmonic Spectroscopy
Patchkovskii, S., & Schuurman, M. S. (2014) · The Journal of Physical Chemistry A · doi:10.1021/jp5090444 · Cited by 13
Transient Impulsive Electronic Raman Redistribution
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Sensitivity of high-order-harmonic generation to aromaticity
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Erratum: High-harmonic spectroscopy of molecular isomers [Phys. Rev. A84, 051403(R) (2011)]
Wong, M. C. H., Brichta, J.-P., Spanner, M., Patchkovskii, S., & Bhardwaj, V. R. (2012) · Physical Review A · doi:10.1103/physreva.85.049901 · Cited by 2
High-order harmonic generation in alkanes (9 pages)
Velotta, R., & Altucci, C. (2006) · Physical Review A · Cited by 1
Attosecond Generation and High Field Physics
Marangos, J. P., & Oppermann, M. (2013) · Springer eBooks · doi:10.1007/978-3-319-00017-6_3 · Cited by 1
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Metadata
- Authors
- Marangos, J. P.
- Affiliations
- Imperial College London (GB)
- Corresponding author
- Marangos, J P
- ORCID
- Marangos, J P
- Venue
- Journal of Physics B: Atomic, Molecular and Optical Physics
- Publisher
- IOP Publishing
- Published
- 2016-05-31
- Volume
- 49
- Issue
- 13
- Pages
- 132001
- ISSN
- 0953-4075 (ISSN-L)
- 1361-6455
- OpenAlex
- W2529289822
- Cited by
- 111
- References
- 147
- Citations by year
- 2026: 7 · 2025: 13 · 2024: 9 · 2023: 3 · 2022: 12 · 2021: 16 · 2020: 9 · 2019: 16 · 2018: 12 · 2017: 8 · 2016: 6
- FWCI
- 6.62
- Type
- journal article
- Language
- en
- Open access
- hybrid
- doi.org
- Licence
- Locations
- Journal of Physics B Atomic Molecular and Optical Physics (publishedVersion, cc-by)
- Funders
- European Research Council (ASTEX 290467)
- Engineering and Physical Sciences Research Council (EP/I032517/1)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Spectroscopy and Quantum Chemical Studies
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Terahertz technology and applications
- Keywords
- high harmonic generation, organic compounds, biomolecules, molecular dynamics, molecular structure, attosecond spectroscopy
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