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Easy incorporation of single-walled carbon nanotubes into two-dimensional MoS2 for high-performance hydrogen evolution
Abstract
The limited intrinsic conductivity of two-dimensional (2D) MoS₂ nanosheets compromises its high electrocatalytic performance. In this work, we develop a facile method of simply dispersing MoS₂ nanosheets into a water-isopropanol solution of high-conducting single-walled carbon nanotubes (SWCNTs) for preparation of MoS₂/SWCNT composites. The SWCNTs in the hybrid system serve as effective electron transport channels among 2D MoS₂ nanosheets and facilitate charge transfer at the catalyst-electrolyte interface. We investigated the influence of SWCNTs ratios on the catalytic activities and obtained a high-performance hybrid catalyst with a low Tafel slope of 40.82 mV/decade and prominent electrochemical durability. The demonstration of our hybrid electrocatalytic system, with its scalable capacity for facile preparation, provides a new pathway to enhance HER activity.
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“Carbon materials, such as porous carbon, [ 158-161 ] carbon nanofi bers, [ 162 ] carbon nanotubes [ 163-167 ] and graphene, [ 42,43,168-175 ] have shown great potential applications as electrocatalyst supports owing to their high conductivity and stability.”
From 2D Transition‐Metal‐Dichalcogenide‐Nanosheet‐Based Composites for Photocatalytic and Electrocatalytic Hydrogen Evolution Reactions (2016) · cites this paper as [167]
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Metadata
- Authors
- Cai, Y., Yang, X., Liang, T., Dai, L., Ma, L., Huang, G., Chen, W., Chen, H., Su, H., & Xu, M.
- Affiliations
- State Key Laboratory of Silicon Materials (CN)
- Zhejiang University (CN)
- University of Macau (MO)
- ORCID
- Venue
- Nanotechnology
- Publisher
- IOP Publishing
- Published
- 2014-10-31
- Volume
- 25
- Issue
- 46
- Pages
- 465401
- ISSN
- 0957-4484 (ISSN-L)
- 1361-6528
- OpenAlex
- W2049811783
- Cited by
- 71
- References
- 30
- Citations by year
- 2026: 2 · 2025: 5 · 2024: 6 · 2023: 6 · 2022: 5 · 2021: 5 · 2020: 9 · 2019: 4 · 2018: 8 · 2017: 8 · 2016: 8 · 2015: 5
- FWCI
- 2.31
- Type
- journal article
- Language
- en
- Open access
- closed
- Licence
- Locations
- Nanotechnology (publishedVersion)
- PubMed (publishedVersion)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Materials Science › Materials Chemistry › 2D Materials and Applications
- Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Supercapacitor Materials and Fabrication
- Keywords
- single-walled carbon nanotubes, MoS2 nanosheets, hydrogen evolution reaction, electrocatalysis, charge transfer, electron transport channels, Tafel slope, electrochemical durability, two-dimensional materials, hybrid catalysts
- MeSH terms
- Catalysis, Disulfides, Electrochemistry, Humans, Hydrogen, Molybdenum, Nanotubes, Carbon
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