Identification of twinned gas phase clusters by single-shot scattering with intense soft x-ray pulses
Open accessAbstract
Scattering experiments on xenon nanoclusters with high-intensity soft x-ray laser pulses from the F ree-Electron LAS er in H amburg (FLASH) are performed to investigate different cluster morphologies in the gas phase. Three different types of scattering patterns can be identified. The most frequent pattern of concentric rings reflects the event of a single spherical cluster in focus. Fine interference rings similar to Newton rings appear when two clusters are illuminated at μ m distance, revealing three-dimensional information about the location of the clusters. Between 10 and 30% of all hits show a previously unknown twin cluster configuration with two clusters in direct contact. Simulations of scattering patterns for twin clusters with different sizes of the two particles, degree of fusion and orientation in space allow us to explain all the observed patterns.
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The first proof-of-principle experiments for single-shot imaging of single nanometer-sized samples in the gas phase targeted cluster shapes and sizes, morphologies of cluster assemblies, and imaging biological specimens.
“The first proof-of-principle experiments for single-shot imaging of single nanometer-sized samples in the gas phase (figure 15) were targeted at determining cluster shapes and sizes [92], the morphologies of cluster assemblies [93], and imaging biological specimens [94].”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [93]
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Roadmap of ultrafast x-ray atomic and molecular physics
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- Authors
- Rupp, D., Adolph, M., Gorkhover, T., Schorb, S., Wolter, D., Hartmann, R., Kimmel, N., Reich, C., Feigl, T., de Castro, A. R. B., Treusch, R., Strüder, L., Möller, T., & Bostedt, C.
- Affiliations
- Technische Universität Berlin (DE)
- SLAC National Accelerator Laboratory (US)
- PNSensor (Germany) (DE)
- Max Planck Society (DE)
- Fraunhofer Institute for Applied Optics and Precision Engineering (DE)
- Deutsches Elektronen-Synchrotron DESY (DE)
- Corresponding author
- Rupp, D
- Venue
- New Journal of Physics
- Publisher
- IOP Publishing
- Published
- 2012-05-16
- Volume
- 14
- Issue
- 5
- Pages
- 055016
- ISSN
- 1367-2630 (ISSN-L)
- OpenAlex
- W2009201928
- Cited by
- 54
- References
- 25
- Citations by year
- 2026: 1 · 2024: 1 · 2023: 3 · 2022: 6 · 2021: 4 · 2020: 4 · 2019: 6 · 2018: 5 · 2017: 1 · 2016: 8 · 2015: 6 · 2014: 6 · 2013: 3
- FWCI
- 4.62
- Type
- journal article
- Language
- en
- Open access
- gold
- doi.org
- Licence
- cc-by
- Locations
- New Journal of Physics (publishedVersion, cc-by)
- LA Referencia (Red Federada de Repositorios Institucionales de Publicaciones Científicas) (publishedVersion)
- Americanae (AECID Library) (submittedVersion)
- Desy Publications Database (Deutsches Elektronen-Synchrotron DESY) (submittedVersion, other-oa)
- Fraunhofer-Publica (Fraunhofer-Gesellschaft) (submittedVersion)
- MPG.PuRe (Max Planck Society) (submittedVersion)
- Repository for Publications and Research Data (ETH Zurich) (submittedVersion, other-oa)
- ETH Zürich Research Collection
- Greater South Information System
- Funders
- Deutsche Forschungsgemeinschaft
- Bundesministerium für Bildung und Forschung
- Deutsches Elektronen-Synchrotron
- Topics
- Physical Sciences › Physics and Astronomy › Radiation › Advanced X-ray Imaging Techniques
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Earth and Planetary Sciences › Atmospheric Science › nanoparticles nucleation surface interactions
- Keywords
- FLASH free-electron laser, interference rings, Newton rings, cluster fusion
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