Ultrafast X-Ray Scattering of Xenon Nanoparticles: Imaging Transient States of Matter
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Femtosecond x-ray laser flashes with power densities of up to 10(14) W/cm(2) at 13.7 nm wavelength were scattered by single xenon clusters in the gas phase. Similar to light scattering from atmospheric microparticles, the x-ray diffraction patterns carry information about the optical constants of the objects. However, the high flux of the x-ray laser induces severe transient changes of the electronic configuration, resulting in a tenfold increase of absorption in the developing nanoplasma. The modification in opaqueness can be correlated to strong atomic charging of the particle leading to excitation of Xe(4+). It is shown that single-shot single-particle scattering on femtosecond time scales yields insight into ultrafast processes in highly excited systems where conventional spectroscopy techniques are inherently blind.
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Strong resonances near inner-shell ionization thresholds can leave distinct fingerprints in the x-ray diffraction signal, allowing investigation of electronically excited states.
“For investigating electronically excited states one can exploit that the x-ray scattering signal is generated by the electrons in the sample and that strong resonances near the inner-shell ionization thresholds can leave distinct fingerprints in the diffraction signal [96].”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [96]
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Ziaja, B., Jurek, Z., Medvedev, N. A., Son, S.-K., Thiele, R., & Toleikis, S. (2013) · Journal of Physics B Atomic Molecular and Optical Physics · doi:10.1088/0953-4075/46/16/164009 · Cited by 9 · see citing works
Melting, Bubblelike Expansion, and Explosion of Superheated Plasmonic Nanoparticles
Dold, S., Reichenbach, T., Colombo, A., Jordan, J., Barke, I., Behrens, P., Bernhardt, N., Correa, J., Düsterer, S., Erk, B., et al. (2025) · Physical Review Letters · doi:10.1103/physrevlett.134.136101 · Cited by 10 · see citing works
Self-citationAntonsson, E., Peltz, C., Plenge, J., Langer, B., Fennel, T., & Rühl, E. (2015) · Journal of Electron Spectroscopy and Related Phenomena · doi:10.1016/j.elspec.2015.04.015 · Cited by 8 · see citing works
Ultraintense laser-cluster interactions: Effects of the cluster shape
Barrington, K., Hartwick, Z., Trost, J., Pandit, R. R., Bigaouette, N., Ramunno, L., & Ackad, E. (2016) · Physical Review A · doi:10.1103/physreva.93.013417 · Cited by 8 · see citing works
Sauppe, M., Rompotis, D., Erk, B., Bari, S., Bischoff, T., Boll, R., Bomme, C., Bostedt, C., Dörner, S., Düsterer, S., et al. (2018) · Journal of Synchrotron Radiation · doi:10.1107/s1600577518006094 · Cited by 8 · see citing works
Self-citationNishiyama, T., Niozu, A., Bostedt, C., Ferguson, K., Sato, Y., Hutchison, C. D. M., Nagaya, K., Fukuzawa, H., Motomura, K., Wada, S., et al. (2019) · IUCrJ · doi:10.1107/s2052252519014222 · Cited by 7 · see citing works
Self-citationIntense XUV pulses from a compact HHG setup using a single harmonic
Kretschmar, M., Vrakking, M. J. J., & Schütte, B. (2021) · Journal of Physics B Atomic Molecular and Optical Physics · doi:10.1088/1361-6455/ac3743 · Cited by 7 · see citing works
Bostedt, C., Gorkhover, T., Rupp, D., & Möller, T. B. (2020) · Springer eBooks · doi:10.1007/978-3-030-23201-6_39 · Cited by 7 · see citing works
Self-citationRelation between Inner Structural Dynamics and Ion Dynamics of Laser-Heated Nanoparticles
Niozu, A., Kumagai, Y., Fukuzawa, H., Yokono, N., You, D., Saito, S., Luo, Y., Kukk, E., Cirelli, C., Rist, J., et al. (2021) · Physical Review X · doi:10.1103/physrevx.11.031046 · Cited by 7 · see citing works
Self-citationUltrafast Single-Particle Imaging with Intense X-Ray Pulses
Sun, Z., Haddad, A. A., Augustin, S., Knopp, G., Knurr, J., Schnorr, K., & Bostedt, C. (2022) · CHIMIA International Journal for Chemistry · doi:10.2533/chimia.2022.529 · Cited by 6 · see citing works
Self-citationWhite, J., & Ackad, E. (2015) · Physics of Plasmas · doi:10.1063/1.4908264 · Cited by 6 · see citing works
Gamboa, E. J., Bachmann, B., Kraus, D., MacDonald, M. J., Bucher, M., Carron, S., Coffee, R., Drake, R. P., Emig, J., Ferguson, K., et al. (2016) · Journal of Instrumentation · doi:10.1088/1748-0221/11/08/p08015 · Cited by 5 · see citing works
Self-citationMeasurement of asymmetric electron cloud in cluster nano-plasma
Sarkar, S., Gopal, R., Kundu, M., Gope, K., Anand, M., & Krishnamurthy, M. (2019) · Physics of Plasmas · doi:10.1063/1.5090602 · Cited by 5 · see citing works
Saladrigas, C. A., Feinberg, A. J., Ziemkiewicz, M. P., Bacellar, C., Bucher, M., Bernando, C., Carron, S., Chatterley, A. S., Decker, F.-J., Ferguson, K., et al. (2021) · The European Physical Journal Special Topics · doi:10.1140/epjs/s11734-021-00280-0 · Cited by 5 · see citing works
Self-citationIonization dynamics of Xe nanoplasma formation studied with XUV fluorescence spectroscopy
Przystawik, A., Schroedter, L., Müller, M., Adolph, M., Bostedt, C., Flückiger, L., Gorkhover, T., Kickermann, A., Krikunova, M., Nösel, L., et al. (2015) · Journal of Physics B Atomic Molecular and Optical Physics · doi:10.1088/0953-4075/48/18/184002 · Cited by 3 · see citing works
Self-citationEffect of Rabi dynamics in resonant x-ray scattering of intense attosecond pulses
Venkatesh, A., & Ho, P. J. (2025) · Physical Review A · doi:10.1103/physreva.111.l021101 · Cited by 5 · see citing works
Quantum coherent diffractive imaging
Kruse, B., Liewehr, B., Peltz, C., & Fennel, T. (2020) · Journal of Physics Photonics · doi:10.1088/2515-7647/ab83e4 · Cited by 4 · see citing works
MacDonald, M. J., Gorkhover, T., Bachmann, B., Bucher, M., Carron, S., Coffee, R., Drake, R. P., Ferguson, K., Fletcher, L. B., Gamboa, E. J., et al. (2016) · Review of Scientific Instruments · doi:10.1063/1.4960502 · Cited by 4 · see citing works
Self-citationX-Ray and XUV Imaging of Helium Nanodroplets
Tanyag, R. M. P., Langbehn, B., Möller, T. B., & Rupp, D. (2022) · Topics in applied physics · doi:10.1007/978-3-030-94896-2_7 · Cited by 4 · see citing works
Self-citationMeasurement of a subpicosecond coherence time in a quasi-steady-state XUV laser
Marec, A. L., Meng, L., Klisnick, A., Kozlová, M., Nejdl, J., Tissandier, F., Guilbaud, O., & Calisti, A. (2015) · Physical Review A · doi:10.1103/physreva.92.033852 · Cited by 3 · see citing works
XUV fluorescence as a probe of laser-induced helium nanoplasma dynamics
Sumfleth, M., Przystawik, A., Namboodiri, M. N., & Laarmann, T. (2023) · New Journal of Physics · doi:10.1088/1367-2630/ad02b7 · Cited by 2 · see citing works
Self-citationSimulations of single-particle imaging of hydrated proteins with x-ray free-electron lasers
Jurek, Z., Ziaja, B., Santra, R., Mancuso⋈, A. P., Bielecki, J., & Fortmann-Grote, C. (2017) · Advances in Computational Methods for X-Ray Optics · doi:10.1117/12.2275274 · Cited by 2 · see citing works
Multispectroscopic Study of Single Xe Clusters Using XFEL Pulses
Nishiyama, T., Bostedt, C., Ferguson, K., Hutchison, C. D. M., Nagaya, K., Fukuzawa, H., Motomura, K., Wada, S., Sakai, T., Matsunami, K., et al. (2019) · Applied Sciences · doi:10.3390/app9224932 · Cited by 2 · see citing works
Self-citationFragmentation of clusters and recombination induced by intense and ultrashort x-ray laser pulses
Tı̂mneanu, N., Iwan, B., Andreasson, J., Bergh, M., Seibert, M. M., Bostedt, C., Schorb, S., Thomas, H., Rupp, D., Gorkhover, T., et al. (2013) · Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE · doi:10.1117/12.2019299 · Cited by 1 · see citing works
Self-citationImaging Clusters and Their Dynamics with Single-shot Coherent Diffraction
Colombo, A., & Rupp, D. (2023) · Royal Society of Chemistry eBooks · doi:10.1039/bk9781837671564-00172 · Cited by 1 · see citing works
Self-citationBostedt, C., Gorkhover, T., Rupp, D., & Möller, T. B. (2019) · Springer eBooks · doi:10.1007/978-3-319-04507-8_39-2 · Cited by 1 · see citing works
Self-citationTheoretical Concepts for Single Cluster Imaging
Rupp, D. (2016) · Springer theses · doi:10.1007/978-3-319-28649-5_1 · Cited by 1 · see citing works
Self-citationTracing Nonlinear Cluster Dynamics Induced by Intense XUV, NIR and MIR Laser Pulses
Schütte, B. (2017) · Springer series in chemical physics · doi:10.1007/978-3-319-64840-8_5 · Cited by 1 · see citing works
Ultrafast Nanoscale 3D Coherent X-ray Imaging
De, J. C. M. R. D. (2019) · doi:10.70675/8fba07e1z9be1z48fcz8adbzac1c5033283a · Cited by 1 · see citing works
Ultrafast laser studies of molecules in helium clusters
Galinis, G. (2015) · Leicester Research Archive (University of Leicester)
Mid-infrared strong-field ionization of clusters using two-cycle pulsesPreprint
Schütte, B., Ye, P., Patchkovskii, S., Austin, D. R., Brahms, C., Strüber, C., Witting, T., Ivanov, M., Tisch, J. W. G., & Marangos, J. P. (2016) · arXiv (Cornell University)
Results and Discussion: Imaging and Ion Spectroscopy of Single Large Xenon Clusters
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Self-citationTime-Resolved Measurements of Shock-Compressed Matter using X-rays.
MacDonald, M. J. (2016) · Deep Blue (University of Michigan)
Bucher, M., Ho, P. J., Ferguson, K., Gorkhover, T., Marinelli, A., Rupp, D., Geßner, O., Vilesov, A. F., Rolles, D., Rudenko, A., et al. (2017) · Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC) · doi:10.1109/cleoe-eqec.2017.8087754
Self-citationBostedt, C., Gorkhover, T., Rupp, D., & Möller, T. B. (2015) · Springer eBooks · doi:10.1007/978-3-319-04507-8_39-1
Self-citationBostedt, C., Gorkhover, T., Rupp, D., & Möller, T. B. (2016) · Springer eBooks · doi:10.1007/978-3-319-14394-1_39
Self-citationRupp, D. (2016) · Springer theses · doi:10.1007/978-3-319-28649-5_2
Self-citationXUV fluorescence as a probe of laser-induced helium nanoplasma dynamicsPreprint
Sumfleth, M., Przystawik, A., Namboodiri, M., & Laarmann, T. (2023) · arXiv (Cornell University) · doi:10.48550/arxiv.2305.10031
Self-citationImaging Ultrafast Electron Dynamics in Isolated Nanoparticles
Senfftleben, B., Zimmermann, J., Colombo, A., Hassanpour, E., Hecht, L., Hoffmann, A., Kretschmar, M., Kolatzki, K., Kruse, B., Langbehn, B., et al. (2023) · Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC) · doi:10.1109/cleo/europe-eqec57999.2023.10231805
Self-citationDouble diffraction imaging of x-ray induced structural dynamics in single free nanoparticles
Sauppe, M., Bischoff, T., Bomme, C., Bostedt, C., Colombo, A., Erk, B., Feigl, T., Flückiger, L., Gorkhover, T., Heilrath, A., et al. (2024) · New Journal of Physics · doi:10.1088/1367-2630/ad5d84
Self-citationQuantum interference in two-atom resonant x-ray scattering of an intense attosecond pulse
Venkatesh, A., & Ho, P. J. (2026) · Physical Review A · doi:10.1103/97ss-g7lp
Laser-Induced Transient Opacity in Helium Nanodroplets Probed by Single-Shot Coherent Diffraction
Zimmermann, J., von Scheven, T., Colombo, A., Kolatzki, K., Kruse, B., Langbehn, B., Möller, T., Monserud, N., Sauppe, M., Schütte, B., et al. (2026) · Ultrafast Science · doi:10.34133/ultrafastscience.0146
Self-citation
- Authors
- Bostedt, C., Eremina, E., Rupp, D., Adolph, M., Thomas, H., Hoener, M., de Castro, A. R. B., Tiggesbäumker, J., Meiwes-Broer, K.-H., Laarmann, T., Wabnitz, H., Plönjes, E., Treusch, R., Schneider, J. R., & Möller, T.
- Affiliations
- SLAC National Accelerator Laboratory (US)
- Technische Universität Berlin (DE)
- University of Rostock (DE)
- Deutsches Elektronen-Synchrotron DESY (DE)
- ORCID
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2012-02-29
- Volume
- 108
- Issue
- 9
- Pages
- 093401-093401
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2032211165
- Cited by
- 100
- References
- 21
- Citations by year
- 2026: 2 · 2025: 3 · 2024: 1 · 2023: 6 · 2022: 4 · 2021: 5 · 2020: 6 · 2019: 6 · 2018: 7 · 2017: 6 · 2016: 17 · 2015: 13 · 2014: 7 · 2013: 9 · 2012: 8
- FWCI
- 6.12
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Locations
- Physical Review Letters (publishedVersion)
- PubMed (publishedVersion)
- LA Referencia (Red Federada de Repositorios Institucionales de Publicaciones Científicas) (publishedVersion)
- Desy publication database (The Deutsches Elektronen-Synchrotron) (submittedVersion, other-oa)
- Americanae (AECID Library) (submittedVersion)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Physics and Astronomy › Nuclear and High Energy Physics › Laser-Plasma Interactions and Diagnostics
- Physical Sciences › Physics and Astronomy › Radiation › Advanced X-ray Imaging Techniques
- Keywords
- single-particle scattering, nanoplasma, optical constants, single-shot imaging, ultrafast dynamics
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