Phase differences in the photoemission from krypton in the fine-structure-split ionization channelsP3/22andP1/22
Abstract
Using the reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) technique, a nonzero phase difference is observed in the two-photon ionization transition of krypton atoms into the ionization channels $^{2}P_{1/2}$ and $^{2}P_{3/2}$ when an electron is removed from the $4p$ shell. The phase difference is studied for excitation energies ranging from $\ensuremath{\approx}18\phantom{\rule{0.28em}{0ex}}\mathrm{eV}$ up to $\ensuremath{\approx}28\phantom{\rule{0.28em}{0ex}}\mathrm{eV}$. The phase differences are found to depend on the relative directions of linear polarization of the photoionization laser pulses and the pulses inducing the subsequent continuum-continuum transition. The experimental results are compared to phase differences calculated on the basis of dipole matrix elements for photoionization and scattering phases known for krypton from earlier experiments. The results indicate that the RABBITT phase differences do not give an obvious direct access to time-delay differences in the primary photoionization step of the atom.
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Unless one channel is dominant, interpretation of experimental results in terms of photoionization time delays or phase retrieval becomes ambiguous.
“Unless one of the channels is dominant, the interpretation of the experimental results in terms of photoionization time delays (figure 22) [196] or phase retrieval (figure 23) becomes ambiguous.”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [196]
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Roadmap of ultrafast x-ray atomic and molecular physics
Young, L., Ueda, K., Gühr, M., Bucksbaum, P. H., Simon, M., Mukamel, S., Rohringer, N., Prince, K. C., Masciovecchio, C., Meyer, M., et al. (2018) · Journal of Physics B: Atomic, Molecular and Optical Physics · doi:10.1088/1361-6455/aa9735 · Cited by 337 · see citing works
- Authors
- Baggash, M., & Rottke, H.
- Affiliations
- Max-Born-Institute for Nonlinear Optics and Short Pulse Spectroscopy (DE)
- ORCID
- Rottke, H.
- Venue
- Physical Review A
- Publisher
- American Physical Society (APS)
- Published
- 2015-07-27
- Volume
- 92
- Issue
- 1
- ISSN
- 0556-2791 (ISSN-L)
- 1050-2947
- 1094-1622
- OpenAlex
- W2562828702
- Cited by
- 4
- References
- 21
- Citations by year
- 2026: 1 · 2018: 1 · 2017: 2
- FWCI
- 0.51
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Physical Review A (publishedVersion)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Atomic and Molecular Physics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Quantum optics and atomic interactions
- Keywords
- krypton, two-photon ionization, phase difference, RABBITT, fine structure splitting, polarization dependence, dipole matrix elements, photoionization time delay, photoemission
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