Cited by 1,470X-ray Spectroscopy and Fluorescence AnalysisLaser-Matter Interactions and ApplicationsAtomic and Molecular Physics

Time-resolved atomic inner-shell spectroscopy

Open access
Drescher, M., Hentschel, M., Kienberger, R., Uiberacker, M., Yakovlev, V., Scrinzi, A., Westerwalbesloh, Th., Kleineberg, U. +2 more·2002·Nature

Abstract

The characteristic time constants of the relaxation dynamics of core-excited atoms have hitherto been inferred from the linewidths of electronic transitions measured by continuous-wave extreme ultraviolet or X-ray spectroscopy. Here we demonstrate that a laser-based sampling system, consisting of a few-femtosecond visible light pulse and a synchronized sub-femtosecond soft X-ray pulse, allows us to trace these dynamics directly in the time domain with attosecond resolution. We have measured a lifetime of 7.9(-0.9)(+1.0) fs of M-shell vacancies of krypton in such a pump-probe experiment.

Integrity signals

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Crossref · 10.1038/nature01143

Cites

23 of 23 references verified0 citation errors · 0 not checkable

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Authors
Drescher, M., Hentschel, M., Kienberger, R., Uiberacker, M., Yakovlev, V., Scrinzi, A., Westerwalbesloh, T., Kleineberg, U., Heinzmann, U., & Krausz, F.
Affiliations
  • TU Wien (AT)
  • Bielefeld University (DE)
Corresponding author
  • Drescher, M.
  • Krausz, F.
Venue
Nature
Published
2002-10
Volume
419
Issue
6909
Pages
803-807
ISSN
  • 0028-0836 (ISSN-L)
  • 1476-4687
OpenAlex
W2058175549
Cited by
1,470
References
23
Citations by year
2026: 25 · 2025: 28 · 2024: 49 · 2023: 29 · 2022: 33 · 2021: 40 · 2020: 62 · 2019: 46 · 2018: 56 · 2017: 52 · 2016: 68 · 2015: 81 · 2014: 64 · 2013: 92 · 2012: 62
FWCI
63.74
Type
journal article
Language
en
Open access
Locations
  • Nature (publishedVersion)
  • PubMed (publishedVersion)
  • RePEc: Research Papers in Economics (submittedVersion)
  • The HKU Scholars Hub (University of Hong Kong) (submittedVersion)
  • mediaTUM – the media and publications repository of the Technical University Munich (Technical University Munich) (submittedVersion, other-oa)
  • PUB – Publications at Bielefeld University (Bielefeld University) (submittedVersion)
  • Publikationen an der Universität Bielefeld (Universität Bielefeld) (submittedVersion)
Topics
  • Physical Sciences › Physics and Astronomy › Radiation › X-ray Spectroscopy and Fluorescence Analysis
  • Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
  • Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Atomic and Molecular Physics
Keywords
relaxation dynamics, krypton, attosecond spectroscopy, pump-probe spectroscopy, soft x-ray spectroscopy

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