Interpretation of ultrafast pump-probe terahertz experiments in the time domain: How to exploit two-dimensional correlations
Open accessAbstract
Optical-pump-terahertz-probe spectroscopy has the potential to distinguish between several classes of carrier motion, among others high-frequency oscillatory motion, free motion, and quasifree motion within bounded domains. We present a simplified formalism, applicable to thin samples, which allows identification of these three classes of photoexcited species on basis of the two-dimensional correlations in the time-domain experimental data.
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The straightforward interpretation of THz-TDS as a snapshot of the optical conductivity spectrum breaks down when characteristic relaxation times are comparable to the photoexcitation delay, because the Fourier transform involves times that precede photoexcitation.
“However, the straightforward interpretation of THz-TDS as a snapshot of the optical conductivity spectrum breaks down when the characteristic relaxation times are comparable to the photoexcitation delay, because the Fourier transform involves times that precede photoexcitation. 1,9-16”
From Terahertz time-domain spectroscopy of transient metallic and superconducting states (2015) · cites this paper as [15]
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Terahertz time-domain spectroscopy of transient metallic and superconducting states
Orenstein, J., & Dodge, J. S. (2015) · Physical Review B · doi:10.1103/physrevb.92.134507 · Cited by 50 · see citing works
Pump-Probe Spectroscopy at Terahertz Frequencies
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Yang, Y., Forno, S. D., & Battiato, M. (2024) · Physical review. B./Physical review. B · doi:10.1103/physrevb.109.024425 · Cited by 8 · see citing works
Schins, J. M. (2011) · Physical Review B · doi:10.1103/physrevb.83.239908
Self-citation
- Authors
- Schins, J. M.
- Affiliations
- Delft University of Technology (NL)
- Corresponding author
- Schins, Juleon M.
- ORCID
- Schins, Juleon M.
- Venue
- Physical Review B
- Publisher
- American Physical Society (APS)
- Published
- 2011-05-17
- Volume
- 83
- Issue
- 20
- ISSN
- 1098-0121 (ISSN-L)
- 1550-235X
- OpenAlex
- W2133794120
- Cited by
- 4
- References
- 47
- Citations by year
- 2024: 1 · 2015: 1 · 2012: 1
- FWCI
- 0.45
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Locations
- Physical Review B (publishedVersion)
- Research Repository (Delft University of Technology) (submittedVersion)
- Data Archiving and Networked Services (DANS) (submittedVersion, other-oa)
- Topics
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Terahertz technology and applications
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Chemistry › Spectroscopy › Spectroscopy and Laser Applications
- Keywords
- optical pump-terahertz probe spectroscopy, ultrafast carrier dynamics, two-dimensional correlation analysis, terahertz time-domain spectroscopy, thin samples
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