Efficient Simulation of Strong System-Environment Interactions
Open accessAbstract
Multicomponent quantum systems in strong interaction with their environment are receiving increasing attention due to their importance in a variety of contexts, ranging from solid state quantum information processing to the quantum dynamics of biomolecular aggregates. Unfortunately, these systems are difficult to simulate as the system-bath interactions cannot be treated perturbatively and standard approaches are invalid or inefficient. Here we combine the time-dependent density matrix renormalization group with techniques from the theory of orthogonal polynomials to provide an efficient method for simulating open quantum systems, including spin-boson models and their generalizations to multicomponent systems.
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Non-equilibrium exchanges between system and environment can influence the direction of energy transfer.
“This and other non-equilibrium exchanges between system and environment can have considerable influence on the system dynamics [28-35], influence the direction of energy transfer [28] and may even lead to the generation of long-lived quantum coherence in the system [28, 36-38].”
From Vibrations, quanta and biology (2013) · cites this paper as [28]
Non-equilibrium exchanges between system and environment may lead to generation of long-lived quantum coherence in the system.
“This and other non-equilibrium exchanges between system and environment can have considerable influence on the system dynamics [28-35], influence the direction of energy transfer [28] and may even lead to the generation of long-lived quantum coherence in the system [28, 36-38].”
From Vibrations, quanta and biology (2013) · cites this paper as [28]
Non-equilibrium exchanges between system and environment can have considerable influence on the system dynamics.
“This and other non-equilibrium exchanges between system and environment can have considerable influence on the system dynamics [28-35], influence the direction of energy transfer [28] and may even lead to the generation of long-lived quantum coherence in the system [28, 36-38].”
From Vibrations, quanta and biology (2013) · cites this paper as [28]
Inclusion of significant coupling of electronic motion to long-lived vibrational modes is capable of explaining the long-lived coherences observed in ultrafast 2-D spectroscopy on photosynthetic complexes.
“In the following we will show that the inclusion of significant coupling of electronic motion to long-lived vibrational modes [28, 34] are capable of explaining the observations [36, 37]”
From Vibrations, quanta and biology (2013) · cites this paper as [28]
Electronic coherence may emerge from transiently exciting robust, weakly dephasing vibrational coherences which then transfer back coherence to those exciton transitions that are well matched to the mode.
“The physical picture presented here illustrates a key point: electronic coherence may emerge from transiently exciting robust, weakly dephasing vibrational coherences which then transfer back coherence to those exciton transitions that are well matched to the mode [28, 36, 37].”
From Vibrations, quanta and biology (2013) · cites this paper as [28]
The method has been essential in accurate numerical modeling of complex environments that explain long-lived quantum coherence in photosynthetic complexes.
“Indeed it has been essential in the accurate numerical modeling dynamics of complex environments which explain the emergence of long-lived quantum coherence in photosynthetic complex [28] as explained earlier.”
From Vibrations, quanta and biology (2013) · cites this paper as [28]
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- Authors
- Prior, J., Chin, A. W., Huelga, S. F., & Plenio, M. B.
- Affiliations
- Universidad Politécnica de Cartagena (ES)
- Universität Ulm (DE)
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2010-07-30
- Volume
- 105
- Issue
- 5
- Pages
- 050404-050404
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2007593774
- Cited by
- 480
- References
- 34
- Citations by year
- 2026: 23 · 2025: 38 · 2024: 40 · 2023: 29 · 2022: 32 · 2021: 42 · 2020: 38 · 2019: 28 · 2018: 27 · 2017: 39 · 2016: 28 · 2015: 25 · 2014: 19 · 2013: 22 · 2012: 23
- FWCI
- 12.33
- Type
- journal article
- Language
- en
- Open access
- green
- arxiv.org
- Locations
- Physical Review Letters (publishedVersion)
- PubMed (publishedVersion)
- arXiv (Cornell University) (submittedVersion)
- arXiv (Cornell University)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Quantum many-body systems
- Physical Sciences › Computer Science › Artificial Intelligence › Quantum Computing Algorithms and Architecture
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Quantum Mechanics and Applications
- Keywords
- open quantum systems, system-bath interaction, time-dependent density matrix renormalization group, orthogonal polynomials, spin-boson model, quantum dynamics
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