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Band-Selective Measurements of Electron Dynamics inVO2Using Femtosecond Near-Edge X-Ray Absorption
Open accessAbstract
We report on the first demonstration of femtosecond x-ray absorption spectroscopy, made uniquely possible by the use of broadly tunable bending-magnet radiation from "laser-sliced" electron bunches within a synchrotron storage ring. We measure the femtosecond electronic rearrangements that occur during the photoinduced insulator-metal phase transition in VO2. Symmetry- and element-specific x-ray absorption from V2p and O1s core levels (near 500 eV) separately measures the filling dynamics of differently hybridized V3d-O2p electronic bands near the Fermi level.
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Citations
Cited by
Pickett, M. D., & Stanley Williams, R. (2012) · Nanotechnology · doi:10.1088/0957-4484/23/21/215202 · Cited by 385
The ultrafast X-ray spectroscopic revolution in chemical dynamics
Kraus, P. M., Zürch, M., Cushing, S. K., Neumark, D. M., & Leone, S. R. (2018) · Nature Reviews Chemistry · doi:10.1038/s41570-018-0008-8 · Cited by 336
0.5-keV Soft X-ray attosecond continua
Teichmann, S. M., Silva, F., Cousin, S. L., Hemmer, M., & Biegert, J. (2016) · Nature Communications · doi:10.1038/ncomms11493 · Cited by 265
Real-Time Probing of Electron Dynamics Using Attosecond Time-Resolved Spectroscopy
Ramasesha, K., Leone, S. R., & Neumark, D. M. (2016) · Annual Review of Physical Chemistry · doi:10.1146/annurev-physchem-040215-112025 · Cited by 225
Photo-induced superconductivity
Cavalleri, A. (2018) · Contemporary Physics · doi:10.1080/00107514.2017.1406623 · Cited by 169
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Metadata
- Authors
- Cavalleri, A., Rini, M., Chong, H. H. W., Fourmaux, S., Glover, T. E., Heimann, P. A., Kieffer, J. C., & Schoenlein, R. W.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2005-08-05
- Volume
- 95
- Issue
- 6
- Pages
- 067405-067405
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W1981216549
- Cited by
- 280
- References
- 0
- FWCI
- 13.39
- Type
- journal article
- Language
- en
- Open access
- green
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- Cavalleri, A., Rini, M., Chong, H. H. W., Fourmaux, S., Glover, T. E., Heimann, P. A., Kieffer, J. C., & Schoenlein, R. W. (2005). Band-Selective Measurements of Electron Dynamics inVO2Using Femtosecond Near-Edge X-Ray Absorption. Physical Review Letters. https://doi.org/10.1103/physrevlett.95.067405
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