Cited by 455Thermal properties of materialsThermography and Photoacoustic TechniquesHeat Transfer and Boiling Studies

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Thermal Conductance of Hydrophilic and Hydrophobic Interfaces

Ge, Zhenbin, Cahill, David G., Braun, Paul V.·2006·Physical Review Letters

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Abstract

Using time-domain thermoreflectance, we have measured the transport of thermally excited vibrational energy across planar interfaces between water and solids that have been chemically functionalized with a self-assembled monolayer (SAM). The Kapitza length--i.e., the thermal conductivity of water divided by the thermal conductance per unit area of the interface--is analogous to the "slip length" for water flowing tangentially past a solid surface. We find that the Kapitza length at hydrophobic interfaces (10-12 nm) is a factor of 2-3 larger than the Kapitza length at hydrophilic interfaces (3-6 nm). If a vapor layer is present at the hydrophobic interface, and this vapor layer has a thermal conductivity that is comparable to bulk water vapor, then our experimental results constrain the thickness of the vapor layer to be less than 0.25 nm.

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Authors: Ge, Z., Cahill, D. G., & Braun, P. V.
Affiliations: University of Illinois Urbana-Champaign (US)
ORCID: Cahill, David G.
Braun, Paul V.
Venue: Physical Review Letters
Publisher: American Physical Society (APS)
Published: 2006-05-08
Volume: 96
Issue: 18
Pages: 186101-186101
ISSN: 0031-9007 (ISSN-L)
1079-7114
DOI: 10.1103/physrevlett.96.186101
OpenAlex: W1996203962
Cited by: 455
References: 34
Citations by year: 2026: 19 · 2025: 26 · 2024: 17 · 2023: 24 · 2022: 27 · 2021: 29 · 2020: 30 · 2019: 29 · 2018: 23 · 2017: 43 · 2016: 37 · 2015: 17 · 2014: 20 · 2013: 20 · 2012: 16
FWCI: 10.04
Type: journal article
Language: en
Open access: closed
Licence: link.aps.org/licenses/aps-default-license (vor)
Locations: Physical Review Letters (publishedVersion)
PubMed (publishedVersion)
Bulletin of the American Physical Society
Topics: Physical Sciences › Materials Science › Materials Chemistry › Thermal properties of materials
Physical Sciences › Engineering › Mechanics of Materials › Thermography and Photoacoustic Techniques
Physical Sciences › Engineering › Mechanical Engineering › Heat Transfer and Boiling Studies
Keywords: thermal conductance, hydrophobic interface, hydrophilic interfaces, self-assembled monolayers, solid-water interface, vibrational energy transport, time-domain thermoreflectance, interfacial thermal resistance

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Thermal Conductance of Hydrophilic and Hydrophobic Interfaces

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