Superaerophobic hydrogels for enhanced electrochemical and photoelectrochemical hydrogen production
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A simple modification of electrodes with hydrogel can facilitate hydrogen evolution reactions by readily eliminating gas bubbles.
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Depositing M13 bacteriophages-assembled hydrogel onto a Pt electrode, due to large surface area and high porosity, allows generated H2 bubbles to quickly detach, achieving efficient HER; the number of bubbles generated by the gel-coated electrode with titer 1.5 × 1014 PFU mL−1 is significantly more than pristine Pt electrode.
“Jeon et al. [181] innovatively deposited M13 bacteriophages-assembled hydrogel onto a Pt electrode. Based on the large surface area and high porosity of the hydrogel, the generated H2 bubbles can quickly detach from the electrode surface, thereby achieving efficient HER (Fig. 16b). From the bubble situation during the hydrogen evolution process, it can be found that the number of bubbles generated”
From Advances in Surface/Interface Engineering of Under-Water Superaerophobic Electrodes for Hydrogen Evolution Reaction by Manipulating of Bubbles (2026) · cites this paper as [181]
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- Authors
- Jeon, D., Park, J., Shin, C., Kim, H., Jang, J.-W., Lee, D. W., & Ryu, J.
- Affiliations
- Ulsan National Institute of Science and Technology (KR)
- Corresponding author
- Lee, Dong Woog
- Ryu, Jungki
- Venue
- Science Advances
- Published
- 2020-04-10
- Volume
- 6
- Issue
- 15
- Pages
- eaaz3944-eaaz3944
- ISSN
- 2375-2548 (ISSN-L)
- PMC
- PMC7148083
- OpenAlex
- W3015367981
- Cited by
- 141
- References
- 40
- Citations by year
- 2026: 19 · 2025: 19 · 2024: 33 · 2023: 24 · 2022: 23 · 2021: 17 · 2020: 6
- FWCI
- 3.46
- Type
- journal article
- Language
- en
- Open access
- gold
- doi.org
- Licence
- cc-by-nc
- Locations
- Science Advances (publishedVersion, cc-by-nc)
- PubMed Central (publishedVersion, cc-by-nc)
- PubMed (publishedVersion)
- Scholarworks@UNIST (Ulsan National Institute of Science and Technology) (submittedVersion, cc-by-nc)
- Funders
- National Research Foundation of Korea (2018R1D1A1A02046918, 2019M1A2A2065616, 2019R1A2C2005854)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Advanced Photocatalysis Techniques
- Physical Sciences › Environmental Science › Water Science and Technology › Minerals Flotation and Separation Techniques
- Keywords
- superaerophobic surfaces, hydrogels, hydrogen evolution reaction, photoelectrochemical hydrogen production, bubble removal, transparent hydrogels, electrode modification, gas evolution reactions, concentration overpotential
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