Coherent spin transfer between molecularly bridged quantum dots
Abstract
Femtosecond time-resolved Faraday rotation spectroscopy reveals the instantaneous transfer of spin coherence through conjugated molecular bridges spanning quantum dots of different size over a broad range of temperature. The room-temperature spin-transfer efficiency is approximately 20%, showing that conjugated molecules can be used not only as interconnections for the hierarchical assembly of functional networks but also as efficient spin channels. The results suggest that this class of structures may be useful as two-spin quantum devices operating at ambient temperatures and may offer promising opportunities for future versatile molecule-based spintronic technologies.
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Spin is inherently quantum in nature, and quantum spin transfer through aromatic rings is enhanced at warm temperature.
“Spin is inherently quantum in nature, and quantum spin transfer through aromatic rings is enhanced at warm temperature [87].”
From Consciousness in the universe (2014) · cites this paper as [87]
Ouyang and Awschalom (2003) showed that quantum spin transfer through phenyl ring π orbital resonance clouds is enhanced at increasingly warm temperatures.
“In 2003, Ouyang and Awschalom [87] showed that quantum spin transfer through phenyl ring π orbital resonance clouds (the same as those in protein hydrophobic regions, as illustrated in Figs.567) are enhanced at increasingly warm temperatures.”
From Consciousness in the universe (2014) · cites this paper as [87]
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- Authors
- Ouyang, M., & Awschalom, D. D.
- Affiliations
- University of California, Santa Barbara (US)
- Venue
- Science
- Published
- 2003-08-22
- Volume
- 301
- Issue
- 5636
- Pages
- 1074-1078
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2021819750
- Cited by
- 254
- References
- 21
- Citations by year
- 2026: 2 · 2025: 4 · 2024: 7 · 2023: 9 · 2022: 7 · 2021: 8 · 2020: 10 · 2019: 5 · 2018: 5 · 2017: 5 · 2016: 6 · 2015: 10 · 2014: 10 · 2013: 13 · 2012: 10
- FWCI
- 13.25
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Science (publishedVersion)
- PubMed (publishedVersion)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Quantum and electron transport phenomena
- Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Magnetism in coordination complexes
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Molecular Junctions and Nanostructures
- Keywords
- spin channels, quantum dot size dependence, temperature dependence
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