Cited by 1,408Battery Modeling and ManagementAdvancements in Battery MaterialsAdvanced Battery Materials and Technologies

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Capacity Fade Mechanisms and Side Reactions in Lithium‐Ion Batteries

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Arora, Pankaj, White, Ralph E., Doyle, Marc·1998·Journal of The Electrochemical Society

DOI 10.1149/1.1838857

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Abstract

The capacity of a lithium‐ion battery decreases during cycling. This capacity loss or fade occurs due to several different mechanisms which are due to or are associated with unwanted side reactions that occur in these batteries. These reactions occur during overcharge or overdischarge and cause electrolyte decomposition, passive film formation, active material dissolution, and other phenomena. These capacity loss mechanisms are not included in the present lithium‐ion battery mathematical models available in the open literature. Consequently, these models cannot be used to predict cell performance during cycling and under abuse conditions. This article presents a review of the current literature on capacity fade mechanisms and attempts to describe the information needed and the directions that may be taken to include these mechanisms in advanced lithium‐ion battery models.

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Authors: Arora, P., White, R. E., & Doyle, M.
Affiliations: DuPont (United States) (US)
ORCID: White, Ralph E.
Venue: Journal of The Electrochemical Society
Publisher: The Electrochemical Society
Published: 1998-10-01
Volume: 145
Issue: 10
Pages: 3647-3667
ISSN: 0013-4651 (ISSN-L)
1945-7111
DOI: 10.1149/1.1838857
OpenAlex: W2014862314
Cited by: 1,408
References: 0
Citations by year: 2026: 43 · 2025: 69 · 2024: 59 · 2023: 75 · 2022: 74 · 2021: 70 · 2020: 89 · 2019: 96 · 2018: 86 · 2017: 117 · 2016: 87 · 2015: 96 · 2014: 92 · 2013: 63 · 2012: 39
FWCI: 47.70
Type: journal article
Language: en
Open access: bronze
doi.org
Licence: iopscience.iop.org/page/copyright (vor, 7736 d)
iopscience.iop.org/info/page/text-and-data-mining (tdm, 7736 d)
Locations: Journal of The Electrochemical Society (publishedVersion)
Scholar Commons (University of South Carolina) (submittedVersion)
Topics: Physical Sciences › Engineering › Automotive Engineering › Battery Modeling and Management
Physical Sciences › Engineering › Electrical and Electronic Engineering › Advancements in Battery Materials
Physical Sciences › Engineering › Electrical and Electronic Engineering › Advanced Battery Materials and Technologies
Keywords: lithium-ion batteries, capacity fade, capacity loss mechanisms, side reactions, overcharging, overdischarge, electrolyte decomposition, passive film formation, active material dissolution, cycling performance

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Capacity Fade Mechanisms and Side Reactions in Lithium‐Ion Batteries

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