The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Perspective—Towards Establishing Apparent Hydrogen Binding Energy as the Descriptor for Hydrogen Oxidation/Evolution Reactions
Open accessAbstract
This perspective article formalizes our proposal that the apparent hydrogen binding energy (HBE app ), which takes into account of the water adsorption energy as well as the intrinsic hydrogen binding energy (HBE) on metal surfaces, is the descriptor for hydrogen oxidation/evolution reactions (HOR/HERs). We show that the HBE app , not HBE, is pH dependent and can be determined from the underpotential-deposited hydrogen peaks in cyclic voltammograms for platinum group metals including Pt, Ir, Pd, and Rh, and the decrease of their HOR/HER activities with pH is the result of a strengthened HBE app due to a weakened water adsorption. Also discussed are the needs of further experimental and theoretical work to prove this hypothesis.
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Cites
Hydrogen Oxidation and Evolution Reaction Kinetics on Platinum: Acid vs Alkaline Electrolytes
Sheng, W., Gasteiger, H. A., & Shao-Horn, Y. (2010) · Journal of The Electrochemical Society · doi:10.1149/1.3483106 · Cited by 1,829
Improving the hydrogen oxidation reaction rate by promotion of hydroxyl adsorption
Strmcnik, D., Uchimura, M., Wang, C., Subbaraman, R., Danilovic, N., van der Vliet, D., Paulikas, A. P., Stamenkovic, V. R., & Markovic, N. M. (2013) · Nature Chemistry · doi:10.1038/nchem.1574 · Cited by 1,426
Sheng, W., Myint, M., Chen, J. G., & Yan, Y. (2013) · Energy & Environmental Science · doi:10.1039/c3ee00045a · Cited by 1,202
Self-citationSheng, W., Zhuang, Z., Gao, M., Zheng, J., Chen, J. G., & Yan, Y. (2015) · Nature Communications · doi:10.1038/ncomms6848 · Cited by 1,136
Self-citation
Cited by
Li, P., Jiang, Y., Hu, Y., Men, Y., Liu, Y., Cai, W., & Chen, S. (2022) · Nature Catalysis · doi:10.1038/s41929-022-00846-8 · Cited by 852
Liu, Y., Ding, J., Li, F., Su, X., Zhang, Q., Guan, G., Hu, F., Zhang, J., Wang, Q., Jiang, Y., et al. (2023) · Advanced Materials · doi:10.1002/adma.202207114 · Cited by 193
Pu, Z., Zhang, G., Hassanpour, A., Zheng, D., Wang, S., Liao, S., Chen, Z., & Sun, S. (2021) · Applied Energy · doi:10.1016/j.apenergy.2020.116376 · Cited by 148
Development of Anion Exchange Membrane Water Electrolysis and the Associated Challenges: A Review
Hua, D., Huang, J., Fabbri, E., Rafique, M., & Song, B. (2023) · ChemElectroChem · doi:10.1002/celc.202200999 · Cited by 148
Kim, J., Kim, H., Lee, W.-J., Ruqia, B., Baik, H., Oh, H.-S., Paek, S.-M., Lim, H.-K., Choi, C. H., & Choi, S.-I. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.9b09229 · Cited by 129
Metadata
- Authors
- Zheng, J., Nash, J., Xu, B., & Yan, Y.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 2018
- Volume
- 165
- Issue
- 2
- Pages
- H27-H29
- ISSN
- 0013-4651 (ISSN-L)
- 1945-7111
- OpenAlex
- W2794335936
- Cited by
- 188
- References
- 4
- FWCI
- 3.05
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Zheng, J., Nash, J., Xu, B., & Yan, Y. (2018). Perspective—Towards Establishing Apparent Hydrogen Binding Energy as the Descriptor for Hydrogen Oxidation/Evolution Reactions. Journal of The Electrochemical Society. https://doi.org/10.1149/2.0881802jes
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