Liquid-phase laser ablation
Open accessAbstract
The irradiation of an intense laser pulse onto a solid target immersed in liquid produces dense plasma. The plasma produced by liquid-phase laser ablation has unique features at high pressure and temperature, which are never realized by liquid-phase discharges. Another unique characteristic of liquid-phase laser ablation is the formation of a cavitation bubble. This article reports the fundamental aspects of liquid-phase laser-ablation plasmas, cavitation bubbles, and the formation processes of nanoparticles, together with some applications of liquid-phase laser ablation.
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When laser-induced photonic energy strikes metal surface, inverse bremsstrahlung occurs, where radiation absorption results in vibration of electrons, which are ejected because of formation of superheated plasma at temperatures of 4000-6000 K and explosive solid-vapor phase transition.
“When laser-induced photonic energy strikes the metal surface, inverse bremsstrahlung (IB) [78] occurs, where radiation absorption results in the vibration of the electrons, which are ejected because of the formation of superheated plasma at temperatures of 4000–6000 K [79] and explosive solid–vapor phase transition.”
From Influence of Laser Process Parameters, Liquid Medium, and External Field on the Synthesis of Colloidal Metal Nanoparticles Using Pulsed Laser Ablation in Liquid: A Review (2022) · cites this paper as [79]
Split into 2 atoms — 0 confirmed, 1 partially supported, 0 disputed, 0 misattributed, 1 unverifiable. Expand the claim to see per-atom verdicts.
Experimental — accuracy not yet measuredRecently, research has applied external magnetic, electric, and temperature fields to examine impact of light-matter interaction and achieve shape control on various types of nanocrystals.
“Recently [73,74,75,76,77,78,79,80,81,82,83,84,85,86,87,88,89,90,91,92,93,94,95,96], research has taken a further step, which involved the application of external magnetic, electric, and temperature fields to examine the impact of light–matter interaction and to achieve shape control on various types of nanocrystals.”
From Influence of Laser Process Parameters, Liquid Medium, and External Field on the Synthesis of Colloidal Metal Nanoparticles Using Pulsed Laser Ablation in Liquid: A Review (2022) · cites this paper as [79]
The Control of Liquid-Phase Laser Ablation section (pp. 1324–1325) describes investigating pressure and temperature as physical controls, but reports results for changing water pressure. It does not report applying magnetic or electric fields, or achieving nanocrystal shape control with those fields. (LLM, conf=0.84)
Experimental — accuracy not yet measuredAblation of materials in water generates plasma plumes with a temperature in the range of 4000-8000 K.
“The ablation of materials in water is reported to generate plasma plumes with a temperature in the range of 4000-8000 K. 132,133,135,137”
From Green nanoparticle synthesis at scale: a perspective on overcoming the limits of pulsed laser ablation in liquids for high-throughput production (2023) · cites this paper as [135]
The “Estimations of Plasma Pressure and Temperature” section describes laser ablation of a graphite target in water producing plasma, and the Figure 2 caption says its temperature was evaluated from emission spectra. However, the Conclusions report a temperature of 10⁴ K, not the attributed range of 4000–8000 K. The cited paper supports plasma generation in water but not that numerical range. (LLM, conf=0.88)
Experimental — accuracy not yet measuredA cavitation bubble lifetime is approximately 0.1-1 ms, while persistent microbubbles can stay as long as seconds.
“While a cavitation bubble lifetime is approximately 0.1-1 ms, 145 persistent microbubbles can stay even as long as seconds.135”
From Green nanoparticle synthesis at scale: a perspective on overcoming the limits of pulsed laser ablation in liquids for high-throughput production (2023) · cites this paper as [135]
The citation to this source follows the claim that persistent microbubbles can last for seconds. The Dynamics of Cavitation Bubble section describes a bubble observed at 2.4 ms that then remained stationary, but gives no duration in seconds. Searches for persistent microbubbles and seconds found no passage establishing the claimed lifetime. (LLM, conf=0.72)
Experimental — accuracy not yet measured
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“When laser-induced photonic energy strikes the metal surface, inverse bremsstrahlung (IB) [78] occurs, where radiation absorption results in the vibration of the electrons, which are ejected because of the formation of superheated plasma at temperatures of 4000–6000 K [79] and explosive solid–vapor phase transition.”
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Nguyen, T. T. P., Tanabe-Yamagishi, R., & Ito, Y. (2019) · Applied Surface Science · doi:10.1016/j.apsusc.2018.10.160 · Cited by 44 · see citing works
Nucleation and growth of nanoparticles in a plasma by laser ablation in liquid
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Al-Mamun, S. A., Nakajima, R., & Ishigaki, T. (2012) · Thin Solid Films · doi:10.1016/j.tsf.2012.06.011 · Cited by 29 · see citing works
- Authors
- Sasaki, K., & Takada, N.
- Affiliations
- Hokkaido University (JP)
- Nagoya University (JP)
- ORCID
- Sasaki, Koichi
- Venue
- Pure and Applied Chemistry
- Publisher
- Walter de Gruyter GmbH
- Published
- 2010-05-02
- Volume
- 82
- Issue
- 6
- Pages
- 1317-1327
- ISSN
- 0033-4545 (ISSN-L)
- 1365-3075
- OpenAlex
- W2150997291
- Cited by
- 111
- References
- 18
- Citations by year
- 2026: 1 · 2024: 5 · 2023: 5 · 2022: 10 · 2021: 7 · 2020: 5 · 2019: 7 · 2018: 6 · 2017: 11 · 2016: 8 · 2015: 4 · 2014: 5 · 2013: 13 · 2012: 17
- FWCI
- 6.99
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Locations
- Pure and Applied Chemistry (publishedVersion)
- Funders
- Ministry of Education, Culture, Sports, Science and Technology
- Japan Society for the Promotion of Science (21510114)
- Topics
- Physical Sciences › Engineering › Biomedical Engineering › Laser-Ablation Synthesis of Nanoparticles
- Physical Sciences › Engineering › Mechanics of Materials › Laser-induced spectroscopy and plasma
- Physical Sciences › Engineering › Computational Mechanics › Laser Material Processing Techniques
- Keywords
- laser-produced plasma, cavitation bubbles, nanoparticle formation, high-pressure plasma, laser-matter interaction
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