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The Chemical Recycling of PLA: A Review
Open accessAbstract
Plastics are an indispensable material with numerous benefits and advantages compared to traditional materials, such as glass and paper. However, their widespread use has caused significant environmental pollution and most plastics are currently nonrenewable. Biobased polymers represent an important step for tackling these issues, however, the end-of-life disposal of such materials needs to be critically considered to allow for a transition to a circular economy for plastics. Poly(lactic acid) (PLA) is an important example of a biobased polymer, which is also biodegradable. However, industrial composting of PLA affords water and carbon dioxide only and in the natural environment, PLA has a slow biodegradation rate. Therefore, recycling processes are important for PLA, particularly chemical recycling, which affords monomers and useful platform chemicals, maintaining the usefulness and value of the material. This review covers the different methods of PLA chemical recycling, highlighting recent trends and advances in the area.
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“LL, GG and Cap are all lactones but they show very different reactivities in the ring‐opening polymerization. [16]”
From Master of Chaos and Order: Opposite Microstructures of PCL‐co‐PGA‐co‐PLA Accessible by a Single Catalyst** (2022) · cites this paper as [16]
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Metadata
- Authors
- McKeown, P., & Jones, M. D.
- Affiliations
- University of Bath (GB)
- Corresponding author
- McKeown, Paul
- Jones, Matthew D.
- Venue
- Sustainable Chemistry
- Publisher
- MDPI AG
- Published
- 2020-05-02
- Volume
- 1
- Issue
- 1
- Pages
- 1-22
- ISSN
- 2673-4079 (ISSN-L)
- OpenAlex
- W3021978864
- Cited by
- 294
- References
- 150
- Citations by year
- 2026: 41 · 2025: 66 · 2024: 49 · 2023: 67 · 2022: 49 · 2021: 19 · 2020: 3
- FWCI
- 2.31
- Type
- journal article
- Language
- en
- Open access
- gold
- dx.doi.org
- Licence
- Locations
- Sustainable Chemistry (publishedVersion, cc-by)
- Funders
- Engineering and Physical Sciences Research Council (EP/P016405/1)
- Topics
- Physical Sciences › Materials Science › Biomaterials › biodegradable polymer synthesis and properties
- Physical Sciences › Materials Science › Polymers and Plastics › Polymer crystallization and properties
- Physical Sciences › Environmental Science › Waste Management and Disposal › Waste Management and Recycling
- Keywords
- polylactic acid, chemical recycling, bio-based polymers, biodegradable plastics, monomer recovery, circular economy, plastic waste, end-of-life plastics, composting, biodegradation
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
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