The DOI matches its Crossref record; 89 of the 89 references it cites were found in a registry or an index.
Active Sites and Mechanism of Oxygen Reduction Reaction Electrocatalysis on Nitrogen‐Doped Carbon Materials
Abstract
The oxygen reduction reaction (ORR) is a core reaction for electrochemical energy technologies such as fuel cells and metal–air batteries. ORR catalysts have been limited to platinum, which meets the requirements of high activity and durability. Over the last few decades, a variety of materials have been tested as non‐Pt catalysts, from metal–organic complex molecules to metal‐free catalysts. In particular, nitrogen‐doped graphitic carbon materials, including N‐doped graphene and N‐doped carbon nanotubes, have been extensively studied. However, due to the lack of understanding of the reaction mechanism and conflicting knowledge of the catalytic active sites, carbon‐based catalysts are still under the development stage of achieving a performance similar to Pt‐based catalysts. In addition to the catalytic viewpoint, designing mass transport pathways is required for O 2. Recently, the importance of pyridinic N for the creation of active sites for ORR and the requirement of hydrophobicity near the active sites have been reported. Based on the increased knowledge in controlling ORR performances, bottom‐up preparation of N‐doped carbon catalysts, using N‐containing conjugative molecules as the assemblies of the catalysts, is promising. Here, the recent understanding of the active sites and the mechanism of ORRs on N‐doped carbon catalysts are reviewed.
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Cited by
Diao, J., Qiu, Y., Liu, S., Wang, W., Chen, K., Li, H., Yuan, W., Qu, Y., & Guo, X. (2020) · Advanced Materials · doi:10.1002/adma.201905679 · Cited by 555
Application of Biochar-Based Materials for Effective Pollutant Removal in Wastewater Treatment
Han, M., Liu, Z., Huang, S., Zhang, H., Yang, H., Liu, Y., Zhang, K., & Zeng, Y. (2024) · Nanomaterials · doi:10.3390/nano14231933 · Cited by 37
Maliutina, K. M., Omoriyekomwan, J. E., He, C., Fan, L., & Folli, A. (2023) · Frontiers in Environmental Engineering · doi:10.3389/fenve.2023.1228992 · Cited by 35
Moghaddam, M. S., Bahari, A., & Litkohi, H. R. (2023) · International Journal of Hydrogen Energy · doi:10.1016/j.ijhydene.2023.05.070 · Cited by 34
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Metadata
- Authors
- Singh, S. K., Takeyasu, K., & Nakamura, J.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2018-10-22
- Volume
- 31
- Issue
- 13
- Pages
- e1804297-e1804297
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2897996971
- Cited by
- 733
- References
- 89
- FWCI
- 12.67
- Type
- journal article
- Language
- en
- Open access
- closed
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