The DOI matches its Crossref record; 31 of the 31 references it cites were found in a registry or an index.
Robust Interface Ru Centers for High‐Performance Acidic Oxygen Evolution
Abstract
RuO 2 is considered as the state‐of‐the‐art electrocatalyst for the oxygen evolution reaction (OER) in acidic media. However, its practical application is largely hindered by both the high reaction overpotential and severe electrochemical corrosion of the active centers. To overcome these limitations, innovative design strategies are necessary, which remains a great challenge. Herein, robust interface Ru centers between RuO 2 and graphene, via a controllable oxidation of graphene encapsulating Ru nanoparticles, are presented to efficiently enhance both the activity and stability of the acidic OER. Through precisely controlling the reaction interface, a much lower OER overpotential of only 227 mV at 10 mA cm−2 in acidic electrolyte, compared with that of 290 mV for commercial RuO 2, but a significantly higher durability than the commercial RuO 2, are achieved. Density functional theory (DFT) calculations reveal that the interface Ru centers between the RuO 2 and the graphene can break the classic scaling relationships between the free energies of HOO* and HO* to reduce the limiting potential, rendering an enhancement in the intrinsic OER activity and the resistance to over‐oxidation and corrosion for RuO 2.
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Cites
Combining theory and experiment in electrocatalysis: Insights into materials design
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A highly active and stable IrO x /SrIrO 3 catalyst for the oxygen evolution reaction
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Self-citationInfluence of iron doping on tetravalent nickel content in catalytic oxygen evolving films
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Cited by
Wu, Z.-Y., Chen, F.-Y., Li, B., Yu, S.-W., Finfrock, Y. Z., Meira, D. M., Yan, Q.-Q., Zhu, P., Chen, M.-X., Song, T.-W., et al. (2023) · Nature Materials · doi:10.1038/s41563-022-01380-5 · Cited by 1,004
Oxygen Evolution Reaction in Alkaline Environment: Material Challenges and Solutions
Xie, X., Du, L., Yan, L., Park, S., Qiu, Y., Sokolowski, J., Wang, W., & Shao, Y. (2022) · Advanced Functional Materials · doi:10.1002/adfm.202110036 · Cited by 792
Sun, Y., Xue, Z., Liu, Q., Jia, Y., Li, Y., Liu, K., Lin, Y., Liu, M., Li, G., & Su, C.-Y. (2021) · Nature Communications · doi:10.1038/s41467-021-21595-5 · Cited by 687
Wang, Y., Yang, R., Ding, Y., Zhang, B., Li, H., Bai, B., Li, M., Cui, Y., Xiao, J., & Wu, Z.-S. (2023) · Nature Communications · doi:10.1038/s41467-023-37008-8 · Cited by 547
Self-citationStability of electrocatalytic OER: from principle to application
Li, H., Lin, Y., Duan, J., Wen, Q., Liu, Y., & Zhai, T. (2024) · Chemical Society Reviews · doi:10.1039/d3cs00010a · Cited by 540
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Metadata
- Authors
- Cui, X., Ren, P., Ma, C., Zhao, J., Chen, R., Chen, S., Rajan, N. P., Li, H., Yu, L., Tian, Z., & Deng, D.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2020-05-17
- Volume
- 32
- Issue
- 25
- Pages
- e1908126-e1908126
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W3024337769
- Cited by
- 264
- References
- 31
- FWCI
- 6.55
- Type
- journal article
- Language
- en
- Open access
- closed
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