The DOI matches its Crossref record; 57 of the 57 references it cites were found in a registry or an index.
In Situ Grown Bimetallic MOF‐Based Composite as Highly Efficient Bifunctional Electrocatalyst for Overall Water Splitting with Ultrastability at High Current Densities
Abstract
A newly designed water‐stable NH 2‐MIL‐88B(Fe 2 Ni)‐metal–organic framework (MOF), in situ grown on the surface of a highly conducting 3D macroporous nickel foam (NF), termed NFN‐MOF/NF, is demonstrated to be a highly efficient bifunctional electrocatalyst for overall water splitting with ultrastability at high current densities. The NFN‐MOF/NF achieves ultralow overpotentials of 240 and 87 mV at current density of 10 mA cm−2 for the oxygen evolution reaction and hydrogen evolution reaction, respectively, in 1 m KOH. For the overall water splitting, it requires only an ultralow cell voltage of 1.56 V to reach the current density of 10 mA cm−2, outperforming the pairing of Pt/C on NF as the cathode and IrO 2 on NF as the anode at the same catalyst loading. The stability of the NFN‐MOF/NF catalyst is also outstanding, exhibiting only a minor chronopotentiometric decay of 7.8% at 500 mA cm−2 after 30 h. The success of the present NFN‐MOF/NF catalyst is attributed to the abundant active centers, the bimetallic clusters {Fe 2 Ni(µ 3‐O)(COO)6(H 2 O)3}, in the MOF, the positive coupling effect between Ni and Fe metal ions in the MOF, and synergistic effect between the MOF and NF.
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1 retracted
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RetractedThe Chemistry and Applications of Metal-Organic Frameworks
Furukawa, H., Cordova, K. E., O’Keeffe, M., & Yaghi, O. M. (2013) · Science · doi:10.1126/science.1230444 · Cited by 16,945
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Ultrathin metal–organic framework nanosheets for electrocatalytic oxygen evolution
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Water photolysis at 12.3% efficiency via perovskite photovoltaics and Earth-abundant catalysts
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Cited by
Bavykina, A., Kolobov, N., Khan, I. S., Bau, J. A., Ramirez, A., & Gascon, J. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00685 · Cited by 1,754
Precious Metal Free Hydrogen Evolution Catalyst Design and Application
Feidenhans’l, A. A., Regmi, Y. N., Wei, C., Xia, D., Kibsgaard, J., & King, L. A. (2024) · Chemical Reviews · doi:10.1021/acs.chemrev.3c00712 · Cited by 499
Xu, H., Fei, B., Cai, G., Ha, Y., Liu, J., Jia, H., Zhang, J., Liu, M., & Wu, R. (2020) · Advanced Energy Materials · doi:10.1002/aenm.201902714 · Cited by 332
Cheng, W., Zhang, H., Luan, D., & Lou, X. W. (. (2021) · Science Advances · doi:10.1126/sciadv.abg2580 · Cited by 319
Li, C., Wang, Z., Liu, M., Wang, E., Wang, B., Xu, L., Jiang, K., Fan, S., Sun, Y., Li, J., et al. (2022) · Nature Communications · doi:10.1038/s41467-022-31077-x · Cited by 221
Metadata
- Authors
- Senthil Raja, D., Chuah, X., & Lu, S.
- Venue
- Advanced Energy Materials
- Publisher
- Wiley
- Published
- 2018-05-31
- Volume
- 8
- Issue
- 23
- ISSN
- 1614-6832 (ISSN-L)
- 1614-6840
- OpenAlex
- W2805783971
- Cited by
- 384
- References
- 57
- FWCI
- 9.39
- Type
- journal article
- Language
- en
- Open access
- closed
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