Cited by 320CO2 Reduction Techniques and CatalystsCarbon dioxide utilization in catalysisCatalysts for Methane Reforming

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Electrocatalytic Production of C3‐C4 Compounds by Conversion of CO 2 on a Chloride‐Induced Bi‐Phasic Cu 2 O‐Cu Catalyst

Lee, Seunghwa, Kim, Dahee, Lee, Jaeyoung·2015·Angewandte Chemie International Edition

DOI 10.1002/anie.201505730

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Abstract

Electrocatalytic conversion of carbon dioxide (CO 2 ) has recently received considerable attention as one of the most feasible CO 2 utilization techniques. In particular, copper and copper‐derived catalysts have exhibited the ability to produce a number of organic molecules from CO 2 . Herein, we report a chloride (Cl)‐induced bi‐phasic cuprous oxide (Cu 2 O) and metallic copper (Cu) electrode (Cu 2 O Cl ) as an efficient catalyst for the formation of high‐carbon organic molecules by CO 2 conversion, and identify the origin of electroselectivity toward the formation of high‐carbon organic compounds. The Cu 2 O Cl electrocatalyst results in the preferential formation of multi‐carbon fuels, including n ‐propanol and n ‐butane C3–C4 compounds. We propose that the remarkable electrocatalytic conversion behavior is due to the favorable affinity between the reaction intermediates and the catalytic surface.

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Authors: Lee, S., Kim, D., & Lee, J.
Affiliations: Gwangju Institute of Science and Technology (KR)
Corresponding author: Lee, Jaeyoung
ORCID: Lee, Seunghwa
Kim, Dahee
Lee, Jaeyoung
Venue: Angewandte Chemie International Edition
Publisher: Wiley
Published: 2015-10-16
Volume: 54
Issue: 49
Pages: 14701-14705
ISSN: 1433-7851 (ISSN-L)
1521-3773
DOI: 10.1002/anie.201505730
OpenAlex: W2144904466
Cited by: 320
References: 40
Citations by year: 2026: 14 · 2025: 32 · 2024: 23 · 2023: 29 · 2022: 31 · 2021: 51 · 2020: 40 · 2019: 37 · 2018: 31 · 2017: 21 · 2016: 11
FWCI: 6.22
Type: journal article
Language: en
Open access: closed
Licence: onlinelibrary.wiley.com/termsAndConditions#vor (vor)
Locations: Angewandte Chemie International Edition (publishedVersion)
PubMed (publishedVersion)
Funders: Ministry of Education (NRF2013R1A1A2A10063010)
Topics: Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
Physical Sciences › Chemical Engineering › Process Chemistry and Technology › Carbon dioxide utilization in catalysis
Physical Sciences › Chemical Engineering › Catalysis › Catalysts for Methane Reforming
Keywords: copper oxide, cuprous oxide, 1-propanol, butane, reaction intermediates, copper catalysts

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Electrocatalytic Production of C3‐C4 Compounds by Conversion of CO 2 on a Chloride‐Induced Bi‐Phasic Cu 2 O‐Cu Catalyst

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