Cited by 310CO2 Reduction Techniques and CatalystsElectrocatalysts for Energy ConversionCatalysts for Methane Reforming

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Highly Efficient Electroreduction of CO2 to Methanol on Palladium–Copper Bimetallic Aerogels

Lu, Lu, Sun, Xiaofu, Ma, Jun, Yang, Dexin, Wu, Haihong, Zhang, Bingxing, Zhang, Jianling, Han, Buxing·2018·Angewandte Chemie International Edition

DOI 10.1002/anie.201808964

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Abstract

Electrochemical reduction of CO 2 to CH 3 OH is of great interest. Aerogels have fine inorganic superstructure with high porosity and are known to be exceptional materials. Now a Pd-Cu bimetallic aerogel electrocatalyst has been developed for conversion of CO 2 into CH 3 OH. The current density and Faradaic efficiency of CH 3 OH can be as high as 31.8 mA cm -2 and 80.0 % over the Pd 83 Cu 17 aerogel at a very low overpotential (0.24 V). The superior performance of the electrocatalyst results from efficient adsorption and stabilization of the CO 2 radical anion, high Pd 0 /Pd II and Cu I +Cu 0 /Cu II ratios, and sufficient Pd/Cu grain boundaries of aerogel nanochains.

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Authors: Lu, L., Sun, X., Ma, J., Yang, D., Wu, H., Zhang, B., Zhang, J., & Han, B.
Affiliations: Chinese Academy of Sciences (CN)
East China Normal University (CN)
Corresponding author: Sun, Xiaofu
Han, Buxing
ORCID: Lu, Lu
Sun, Xiaofu
Ma, Jun
Yang, Dexin
Wu, Haihong
Zhang, Bingxing
Zhang, Jianling
Han, Buxing
Venue: Angewandte Chemie International Edition
Publisher: Wiley
Published: 2018-10-02
Volume: 57
Issue: 43
Pages: 14149-14153
ISSN: 1433-7851 (ISSN-L)
1521-3773
DOI: 10.1002/anie.201808964
OpenAlex: W2889349896
Cited by: 310
References: 48
Citations by year: 2026: 16 · 2025: 34 · 2024: 46 · 2023: 34 · 2022: 51 · 2021: 52 · 2020: 48 · 2019: 28 · 2018: 1
FWCI: 7.45
Type: journal article
Language: en
Open access: closed
Licence: onlinelibrary.wiley.com/termsAndConditions#vor (vor)
Locations: Angewandte Chemie International Edition (publishedVersion)
PubMed (publishedVersion)
Funders: National Science Foundation
National Natural Science Foundation of China
National Key Research and Development Program of China
Topics: Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Physical Sciences › Chemical Engineering › Catalysis › Catalysts for Methane Reforming
Keywords: electrochemical CO2 reduction, methanol synthesis, palladium-copper bimetallic catalyst, Faradaic efficiency, grain boundaries

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Highly Efficient Electroreduction of CO2 to Methanol on Palladium–Copper Bimetallic Aerogels

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