The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Surface Modification of Nano‐Cu2O for Controlling CO2 Electrochemical Reduction to Ethylene and Syngas
Abstract
In the surroundings of carbon neutrality, nano‐Cu 2 O is considered a promising catalyst for the electrochemical CO 2 reduction reaction (ECO 2 RR), whose improvements in product selectivity still require considerable efforts. Here, we present an efficient strategy for controlling the ECO 2 RR product by modifying the surface of nano‐Cu 2 O, i.e., by controlling the exposed facets via a reductant‐controlled method to achieve the highest C 2 H 4 selectivity (Faradic efficiency=74.1 %) for Cu 2 O‐based catalysts in neutral electrolytes, and introducing a well‐suited metal–organic framework (MOF) coating on the surface of nano‐Cu 2 O to obtain syngas completely with an appropriate H 2:CO ratio. Detailed mechanism and key intermediate have been illustrated by DFT calculations. Our systematic strategy is expected to control the ECO 2 RR product, improve the selectivity, and provide a reliable method for CO 2 management and the green production of important carbon resources.
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Cites
Progress and perspectives of electrochemical CO2 reduction on copper in aqueous electrolyte
Nitopi, S., Bertheussen, E., Scott, S. B., Liu, X., Engstfeld, A. K., Horch, S., Seger, B., Stephens, I. E. L., Chan, K., Hahn, C., et al. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00705 · Cited by 5,223
Lee, S., Kim, D., & Lee, J. (2015) · Angewandte Chemie International Edition · doi:10.1002/anie.201505730 · Cited by 320
Highly Efficient Electroreduction of CO2 to Methanol on Palladium–Copper Bimetallic Aerogels
Lu, L., Sun, X., Ma, J., Yang, D., Wu, H., Zhang, B., Zhang, J., & Han, B. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201808964 · Cited by 310
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Cited by
Yan, T., Chen, X., Kumari, L., Lin, J., Li, M., Fan, Q., Chi, H., Meyer, T. J., Zhang, S., & Ma, X. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00514 · Cited by 328
Jiang, M., Wang, H., Zhu, M., Luo, X., He, Y., Wang, M., Wu, C., Zhang, L., Li, X., Liao, X., et al. (2024) · Chemical Society Reviews · doi:10.1039/d3cs00857f · Cited by 299
Metadata
- Authors
- Luo, H., Li, B., Ma, J., & Cheng, P.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2022-01-27
- Volume
- 61
- Issue
- 11
- Pages
- e202116736-e202116736
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W4206631307
- Cited by
- 160
- References
- 3
- FWCI
- 6.22
- Type
- journal article
- Language
- en
- Open access
- closed
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- Luo, H., Li, B., Ma, J., & Cheng, P. (2022). Surface Modification of Nano‐Cu2O for Controlling CO2 Electrochemical Reduction to Ethylene and Syngas. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202116736
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