Approaching well-dispersed MoS2 assisted with cellulose nanofiber for highly durable hydrogen evolution reaction
Abstract
The agglomeration and low conductivity of molybdenum disulfide (MoS 2) electrocatalysts restrict the presentation of its real intrinsic reaction activity, which leads to challenges for the high-performance hydrogen evolution reaction (HER). Herein, a well-dispersed and superhydrophilic/superaerophobic MoS 2 catalyst with uniform three-dimensional conductive networks have been prepared assisted with cellulose nanofiber (CNF) and carboxylated multi-walled carbon nanotubes (cMWCNT). The resulted CNF/cMWCNT/MoS 2 catalysts present a superhydrophilic/superaerophobic state with contact angles for water and bubble of 0° and 154.1° respectively. This structure effectively disperses MoS 2 nanoparticles through uniform embeddedness and promotes gas-liquid mass transfer via wettability. Benefiting from these optimizations, the CNF/cMWCNT/MoS 2 exhibits better HER performance and a low overpotential (154 mV @ 10 mA/cm 2). Encourangingly, CNF/cMWCNT/MoS 2 catalysts have a slight decay of 6.99 % at 10 mA/cm 2 after 100 h, while the cMWCNT/MoS 2 shows a decay of 35.83 %. This approach using natural CNF for well-dispersed catalysts provides a potential for high-performance HER electrode design.
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A gel-skeleton electrode using cellulose nanofibers, carboxylated multi-walled carbon nanotubes, and hydrothermally synthesized MoS2 particles is superaerophobic with bubble contact angle 154.1°, and its catalyst performance is superior to MoS2 supported by carbon cloth and an electrode without CNF skeleton at the same loading.
“Chen et al. [178] prepared the catalytic electrode with a gel skeleton using cellulose nanofibers (CNFs) as the gel skeleton, carboxylated multi-walled carbon nanotubes (cMWCNTs) as the conductive medium, and hydrothermally synthesized MoS2 particles as the catalyst (Fig. 16a). The hydrophilic CNF gel makes the electrode superaerophobic, with a bubble contact angle as high as 154.1°. The catalyst”
From Advances in Surface/Interface Engineering of Under-Water Superaerophobic Electrodes for Hydrogen Evolution Reaction by Manipulating of Bubbles (2026) · cites this paper as [178]
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- Authors
- Chen, M., Deng, S., Qing, Y., Xu, H., Liao, Y., Li, L., Zhang, Z., Yan, N., Tian, C., Wu, Y., & Wu, Y.
- Affiliations
- Central South University of Forestry and Technology (CN)
- Corresponding author
- Qing, Yan
- Wu, Yiqiang
- Venue
- Carbohydrate Polymers
- Publisher
- Elsevier BV
- Published
- 2022-10
- Volume
- 294
- Pages
- 119754
- ISSN
- 0144-8617 (ISSN-L)
- OpenAlex
- W4283168119
- Cited by
- 20
- References
- 71
- Citations by year
- 2026: 5 · 2025: 4 · 2024: 5 · 2023: 5 · 2022: 1
- FWCI
- 0.68
- Type
- journal article
- Language
- en
- Open access
- closed
- Licence
- Locations
- Carbohydrate Polymers (publishedVersion)
- PubMed (publishedVersion)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Supercapacitor Materials and Fabrication
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Fuel Cells and Related Materials
- Keywords
- MoS2, hydrogen evolution reaction, cellulose nanofibers, carboxylated multi-walled carbon nanotubes, catalyst dispersion, gas-liquid mass transfer, wettability, electrocatalyst durability, 3D conductive network
- MeSH terms
- Cellulose, Hydrogen, Molybdenum, Nanotubes, Carbon, Nanofibers
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