Cited by 261Per- and polyfluoroalkyl substances researchFluoride Effects and RemovalAdsorption and biosorption for pollutant removal

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Adsorption behavior of perfluorooctanesulfonate (PFOS) and perfluorooctanoate (PFOA) on boehmite

Wang, Fei, Liu, Chengshuai, Shih, Kaimin·2012·Chemosphere

DOI 10.1016/j.chemosphere.2012.06.071

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Abstract

Understanding the interaction of perfluorochemicals, persistent pollutants with known human health effects, with mineral compounds in surface water and groundwater environments is essential to determining their fate and transport. Kinetic experiments showed that adsorption equilibrium can be achieved within 48 h and the boehmite (AlOOH) surface is receptive to perfluorooctanesulfonate (PFOS) and perfluorooctanoate (PFOA) adsorption. The adsorption isotherms estimated the maximum adsorption capacities of PFOS and PFOA on boehmite as 0.877 μg m(-2) and 0.633 μg m(-2), respectively. Compared to the adsorption capacity on γ-alumina, the abundant hydroxyl groups on boehmite surfaces resulted in the 2-3 times higher adsorption of PFOS and PFOA. Increasing solution pH led to a moderate decrease in PFOS and PFOA adsorption, owing to an increase in ligand exchange reactions and the decrease of electrostatic interactions. The presence of NaCl and CaCl(2) in solution demonstrated negative effects for PFOS and PFOA adsorption on boehmite surfaces, with potential mechanisms being electrical double layer compression, competitive adsorption of chloride, and the Ca(2+) bridging effect between perfluorochemicals.

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Authors: Wang, F., Liu, C., & Shih, K.
Affiliations: University of Hong Kong (HK)
Corresponding author: Shih, Kaimin
ORCID: Wang, Fei
Liu, Chengshuai
Shih, Kaimin
Venue: Chemosphere
Publisher: Elsevier BV
Published: 2012-11
Volume: 89
Issue: 8
Pages: 1009-1014
ISSN: 0045-6535 (ISSN-L)
DOI: 10.1016/j.chemosphere.2012.06.071
OpenAlex: W2144867616
Cited by: 260
References: 41
Citations by year: 2026: 27 · 2025: 23 · 2024: 32 · 2023: 17 · 2022: 28 · 2021: 22 · 2020: 25 · 2019: 19 · 2018: 13 · 2017: 11 · 2016: 15 · 2015: 8 · 2014: 12 · 2013: 7 · 2012: 1
FWCI: 7.15
Type: journal article
Language: en
Open access: closed
Licence: www.elsevier.com/tdm/userlicense/1.0/ (tdm)
Locations: Chemosphere (publishedVersion)
PubMed (publishedVersion)
The HKU Scholars Hub (University of Hong Kong) (submittedVersion)
Topics: Physical Sciences › Environmental Science › Environmental Chemistry › Per- and polyfluoroalkyl substances research
Physical Sciences › Environmental Science › Water Science and Technology › Fluoride Effects and Removal
Physical Sciences › Environmental Science › Water Science and Technology › Adsorption and biosorption for pollutant removal
Keywords: PFOS, perfluorooctanoic acid, boehmite, adsorption, perfluorinated compounds, adsorption isotherms, pH effect, chloride interference, calcium interference, electrostatic interactions, ligand exchange, adsorption kinetics, gamma-alumina, groundwater contamination, fate and transport
MeSH terms: Adsorption, Aluminum Hydroxide, Aluminum Oxide, Calcium Chloride, Caprylates, Chlorates, Fluorocarbons, Hydrogen-Ion Concentration, Kinetics, Surface Properties, Water Pollutants, Chemical, Alkanesulfonic Acids, Static Electricity

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Adsorption behavior of perfluorooctanesulfonate (PFOS) and perfluorooctanoate (PFOA) on boehmite

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