Using phenyl methanesulfonate as an electrolyte additive to improve performance of LiNi0.5Co0.2Mn0.3O2/graphite cells at low temperature
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Less inorganic species (LiF, Li2CO3) were observed on graphite surface while using PhMs additive, thereby decreasing resistance.
“According to the XPS results of graphite after 100 cycles shown in Fig. 15e, less inorganic species (LiF, Li 2 CO 3 ) were observed on graphite surface while using PhMs additive, thereby decreasing the resistance.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [131]
The improved low-temperature electrochemical performance by using PhMs additive was ascribed to decreased interphase impedance.
“Recently, the improved LT electrochemical performance by using phenyl methanesulfonate (PhMs) additive [131] was ascribed to the decreased interphase impedance as well.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [131]
There are competing arguments in the literature that improved battery performance at low temperatures was obtained by decreasing inorganic species including LiF in SEIs.
“there are competing arguments regarding the effects of inorganic components of SEIs in the literature claiming that improved battery performance was obtained at LTs by decreasing inorganic species including LiF in SEIs.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [131]
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Lithium-ion batteries for low-temperature applications: Limiting factors and solutions
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“Recently, the improved LT electrochemical performance by using phenyl methanesul-fonate (PhMs) additive [131] was ascribed to the decreased interphase impedance as well.”
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“[205] Alternatively, phenyl methanesulfonate,([206]) butyl sultone,([54]) allyl sulfide,([207]) DTD, PS, and ethylene sulfite([208]) are applied in different systems for obtaining satisfied low‐temperature performance.”
BackgroundAlternative anodes for low temperature lithium-ion batteries
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Recent Progress on the Low‐Temperature Lithium Metal Batteries and Electrolytes
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“Furthermore, three characteristic peaks assigned to LiF, LiP x F y , and LiP x O y F z can be seen, which are related to the decomposition products of LiPF 6 [63].”
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“The reduction in the PMS additive can produce Li2SO4, ROSO2Li, and LiS2 [25].”
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Research Status of Low-Temperature Electrolyte Additives for Lithium-ion Batteries
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“1 XPS spectra for (a) C 1s; (b) O 1s; (c) F 1s; (d) P 2p and (e) S 2p measured from the graphite anode after 100 cycles at -10°C without and with 1 wt % PhMS[10]”
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Low-Temperature All-Solid-State Batteries
Lee, H., Suh, J. H., Kim, J., Pang, W. K., Konstantinov, K., Mun, J., Song, T., & Kim, J. H. (2026) · Nano-Micro Letters · doi:10.1007/s40820-026-02270-0
- Authors
- Lin, Y., Yue, X., Zhang, H., Yu, L., Fan, W., & Xie, T.
- Affiliations
- Shaanxi University of Science and Technology (CN)
- Corresponding author
- Yue, Xiaopeng
- Venue
- Electrochimica Acta
- Publisher
- Elsevier BV
- Published
- 2019-03
- Volume
- 300
- Pages
- 202-207
- ISSN
- 0013-4686 (ISSN-L)
- OpenAlex
- W2913725482
- Cited by
- 33
- References
- 0
- Citations by year
- 2026: 2 · 2025: 3 · 2024: 2 · 2023: 12 · 2022: 4 · 2021: 6 · 2020: 4
- FWCI
- 1.26
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Electrochimica Acta (publishedVersion)
- Funders
- science and technology projects of Guangdong Province (2015B010135008)
- science and technology projects of Guangzhou (201604016131; 201704030020)
- Topics
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advancements in Battery Materials
- Physical Sciences › Engineering › Automotive Engineering › Advanced Battery Technologies Research
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advanced Battery Materials and Technologies
- Keywords
- electrolyte additives, film-forming additives, low-temperature performance, LiNi0.5Co0.2Mn0.3O2, NCM cathode, graphite anode, solid electrolyte interphase, lithium dendrites, capacity retention, interfacial performance, lithium-ion batteries
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