Enhanced performance of Li-ion cell with LiBF4-PC based electrolyte by addition of small amount of LiBOB
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A LiBF4:LiBOB (9:1, molar ratio) dual-salt system in PC/EC/EMC ternary solvent enabled a Li-LiFePO4 cell to show enhanced cyclic performance in a wide temperature range from -50 to 90 °C.
“To combine the good ionic conductivity of LiBF 4 and decent SEI formation capability from LiBOB, a LiBF 4 :LiBOB (9:1, molar ratio) dual-salt system was developed by Xu et al. [99,102], in PC/EC/EMC ternary solvent the Li-LiFePO 4 (LFP) cell showed enhanced cyclic performance in a wide-temperature range from -50 to 90 °C.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [99]
1%-5% LiBOB was sufficient to enable graphite anode cycling reversibly in 1.0 M LiBF4 in 1:1:3 PC:EC:EMC and 1.0 M LiBF4 in 1:1 PC:EC while maintaining excellent cycling performance at low temperatures.
“It was demonstrated that 1%-5% (molar percentage) LiBOB was sufficient to enable graphite anode cycling reversibly in 1.0 M LiBF 4 in 1:1:3 PC:EC:EMC and 1.0 M LiBF 4 in 1:1 PC:EC, respectively, while maintaining the excellent cycling performance of LiBF 4 -PC-based electrolytes at LTs.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [99]
The cell using 1.0 M (0.98 M LiBF4 + 0.02 M LiBOB) in 1:1:3 PC:EC:EMC delivered 83% and 63% of RT discharge capacity at -30 and -40 °C, respectively.
“The cell using the electrolyte of 1.0 M (0.98 M LiBF 4 + 0.02 M LiBOB) in 1:1:3 PC:EC:EMC was able to deliver 83% and 63% of RT discharge capacity at -30 and -40 °C, respectively (Fig. 16b).”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [99]
Cells using 1.0 M LiBF4 in 1:1:3 PC:EC:EMC encounter solvent intercalation into graphite anodes because no stable SEI can be formed at insufficient EC content.
“However, the cells using such electrolyte encounter solvent intercalation into graphite anodes because no stable SEI can be formed at an insufficient content of EC.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [99]
LiBOB introduced into the LiBF4-PC:EC:EMC electrolyte forms an SEI with semicarbonate-like products.
“Hence, LiBOB was introduced into this electrolyte system, which forms an SEI with semicarbonate-like products (Fig. 16a) [99].”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [99]
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“For example, to combine the advantage of the excellent LT performance of LiBF 4 and the low melting point of PC, a system of electrolytes using 1.0 M LiBF 4 in 1:1:3 PC:EC:EMC was studied [99].”
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- Authors
- Zhang, S. S., Xu, K., & Jow, T. R.
- Affiliations
- DEVCOM Army Research Laboratory (US)
- Corresponding author
- Zhang, S.S.
- Venue
- Journal of Power Sources
- Publisher
- Elsevier BV
- Published
- 2006-06
- Volume
- 156
- Issue
- 2
- Pages
- 629-633
- ISSN
- 0378-7753 (ISSN-L)
- OpenAlex
- W2084447311
- Cited by
- 108
- References
- 18
- Citations by year
- 2026: 2 · 2025: 6 · 2024: 9 · 2023: 14 · 2022: 7 · 2021: 6 · 2020: 6 · 2019: 7 · 2018: 2 · 2017: 9 · 2016: 4 · 2015: 6 · 2014: 9 · 2013: 5 · 2012: 2
- FWCI
- 1.27
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Journal of Power Sources (publishedVersion)
- Topics
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advancements in Battery Materials
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advanced Battery Materials and Technologies
- Physical Sciences › Engineering › Automotive Engineering › Advanced Battery Technologies Research
- Keywords
- lithium-ion batteries, solid electrolyte interphase, graphite anode, high current density, electrolyte additives, ethylene carbonate, ethyl methyl carbonate
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