Lithium difluorophosphate as an additive to improve the low temperature performance of LiNi0.5Co0.2Mn0.3O2/graphite cells

Yang, Bowen; Zhang, Hong; Yu, Le; Fan, WeiZhen; Huang, Donghai

doi:10.1016/j.electacta.2016.10.037

Cited by 156Advancements in Battery MaterialsAdvanced Battery Technologies ResearchAdvanced Battery Materials and Technologies

Lithium difluorophosphate as an additive to improve the low temperature performance of LiNi0.5Co0.2Mn0.3O2/graphite cells

Yang, Bowen, Zhang, Hong, Yu, Le, Fan, WeiZhen, Huang, Donghai·2016·Electrochimica Acta

DOI 10.1016/j.electacta.2016.10.037

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The LiPO2F2-derived SEI has much lower ionic resistance than baseline electrolyte at 0 °C.
“This SEI with rich inorganic species has much lower ionic resistance compared to that of baseline electrolyte at 0 °C (Fig. 18a).”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [142]
At -20 °C, graphite||NMC532 cells using LiPO2F2 additive retained 71.9% of RT capacity, better than 49.4% for baseline electrolyte.
“At -20 °C, the retention of RT capacity of graphite||NMC532 cells using LiPO 2 F 2 additive was 71.9%, much better than the 49.4% for the baseline electrolyte.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [142]
LiPO2F2 additive forms a thin, dense, smooth SEI containing more inorganic components such as LiF and Li2CO3 on graphite anodes, protecting graphite through 100 cycles at 0 °C.
“According to the morphology and composition characterization results, a thin, dense and smooth SEI layer containing more inorganic components such as LiF and Li 2 CO 3 was formed on graphite anodes, showing the capability to protect the graphite anode through 100 cycles at 0 °C.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [142]

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Authors: Yang, B., Zhang, H., Yu, L., Fan, W., & Huang, D.
Affiliations: Shaanxi University of Science and Technology (CN)
Corresponding author: Zhang, Hong
ORCID: Yang, Bowen
Yu, Le
Venue: Electrochimica Acta
Publisher: Elsevier BV
Published: 2016-12
Volume: 221
Pages: 107-114
ISSN: 0013-4686 (ISSN-L)
DOI: 10.1016/j.electacta.2016.10.037
OpenAlex: W2527729130
Cited by: 156
References: 23
Citations by year: 2026: 7 · 2025: 10 · 2024: 12 · 2023: 25 · 2022: 17 · 2021: 30 · 2020: 18 · 2019: 18 · 2018: 17 · 2017: 2
FWCI: 5.12
Type: journal article
Language: en
Open access: closed
Licence: www.elsevier.com/tdm/userlicense/1.0/ (tdm)
Locations: Electrochimica Acta (publishedVersion)
Funders: Guangdong Province (2014B010123002)
science and technology projects of Guangzhou (2014Y2-00012)
Topics: Physical Sciences › Engineering › Electrical and Electronic Engineering › Advancements in Battery Materials
Physical Sciences › Engineering › Automotive Engineering › Advanced Battery Technologies Research
Physical Sciences › Engineering › Electrical and Electronic Engineering › Advanced Battery Materials and Technologies
Keywords: lithium difluorophosphate, electrolyte additives, low-temperature performance, LiNi0.5Co0.2Mn0.3O2, NCM cathode, graphite anode, solid electrolyte interphase, lithium fluoride, lithium carbonate, lithium-ion batteries, capacity retention

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