Holistic utilization of waste plastics through a tandem process
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In tandem catalytic pyrolysis-CVD over Ni foam, polyolefin plastics (HDPE/LDPE/PP) yield highly crystalline carbon nanomaterials, high hydrogen selectivity, and low-impurity liquid oil due to their single-stage decomposition behavior and high alkane content.
“Results showed that polyolefin plastics (HDPE/LDPE/PP), due to their single-stage decomposition behavior and high alkane content, yielded highly crystalline carbon nanomaterials on the Ni foam, simultaneously achieving high hydrogen selectivity and low-impurity liquid oil production.”
From Functional carbon materials from waste plastics: synthesis and applications (2025) · cites this paper as [66]
PET led to 42% amorphous carbon deposition and suppressed hydrogen yield due to oxygen-containing COx byproducts.
“PET, however, led to 42% amorphous carbon deposition and suppressed hydrogen yield due to oxygen-containing CO x byproducts.”
From Functional carbon materials from waste plastics: synthesis and applications (2025) · cites this paper as [66]
In the same process, PS generated 84 wt% high-value aromatic oil.
“In contrast, PS, dominated by aromatic hydrocarbons in its pyrolysis products, generated 84 wt% high-value aromatic oil.”
From Functional carbon materials from waste plastics: synthesis and applications (2025) · cites this paper as [66]
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- Authors
- Dai, L., Karakas, O., Lata, S., Cobb, K., Lei, H., He, C., Cheng, Y., Chen, P., & Ruan, R.
- Affiliations
- University of Minnesota (US)
- Washington State University Tri-Cities (US)
- Tampere University (FI)
- Beijing Union University (CN)
- Corresponding author
- Ruan, Roger
- Venue
- Journal of Environmental Chemical Engineering
- Publisher
- Elsevier BV
- Published
- 2023-10
- Volume
- 11
- Issue
- 5
- Pages
- 110547
- ISSN
- 2213-2929 (ISSN-L)
- 2213-3437
- OpenAlex
- W4383645952
- Cited by
- 12
- References
- 60
- Citations by year
- 2026: 4 · 2025: 5 · 2024: 2 · 2023: 1
- FWCI
- 0.95
- Type
- journal article
- Language
- en
- Open access
- green
- trepo.tuni.fi
- Licence
- Locations
- Journal of environmental chemical engineering (publishedVersion)
- Tampere University Institutional Repository (Tampere University) (submittedVersion, cc-by-nc-nd)
- Funders
- University of Minnesota
- Topics
- Physical Sciences › Engineering › Biomedical Engineering › Thermochemical Biomass Conversion Processes
- Physical Sciences › Chemical Engineering › Catalysis › Catalysts for Methane Reforming
- Physical Sciences › Environmental Science › Pollution › Microplastics and Plastic Pollution
- Keywords
- plastic waste, catalytic pyrolysis, catalytic chemical vapor deposition, carbon nanomaterials, hydrogen production, plastic oil, nickel foam, high-density polyethylene, low-density polyethylene, polypropylene, polystyrene, polyethylene terephthalate, graphitic carbon, amorphous carbon, plastic waste upcycling
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