The DOI matches its Crossref record; 16 of the 16 references it cites were found in a registry or an index.
Continuous Carbon Dioxide Electroreduction to Concentrated Multi-carbon Products Using a Membrane Electrode Assembly
Open accessAbstract
Summary Electrochemical carbon dioxide (CO2) reduction is a promising strategy to synthesize valuable multi-carbon products (C2+) while sequestering CO2 and utilizing intermittent renewable electricity. For industrial deployment, CO2 electrolyzers must remain stable while selectively producing concentrated C2+ products at high rates with modest cell voltages. Here, we present a membrane electrode assembly (MEA) electrolyzer that converts CO2 to C2+ products. We perform side-by-side comparisons of state-of-the-art electrolyzer systems and find that the MEA provides the most stable cell voltage and product selectivity. We then demonstrate an approach to release concentrated gas and liquid products from the cathode outlet. This strategy achieves ∼50% and ∼80% Faradaic efficiency for ethylene and C2+ products, respectively, with cathode outlet concentrations of ∼30% ethylene and the direct production of ∼4 wt % ethanol. We characterize stability by operating continuously for 100 h, the longest stable ethylene production at current densities >100 mA cm−2 among reported CO2 electrolyzers.
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Cites
How copper catalyzes the electroreduction of carbon dioxide into hydrocarbon fuels
Peterson, A. A., Abild-Pedersen, F., Studt, F., Rossmeisl, J., & Nørskov, J. K. (2010) · Energy & Environmental Science · doi:10.1039/c0ee00071j · Cited by 3,784
CO 2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface
Dinh, C.-T., Burdyny, T., Kibria, M. G., Seifitokaldani, A., Gabardo, C. M., García de Arquer, F. P., Kiani, A., Edwards, J. P., De Luna, P., Bushuyev, O. S., et al. (2018) · Science · doi:10.1126/science.aas9100 · Cited by 2,515
Self-citationLi, C. W., & Kanan, M. W. (2012) · Journal of the American Chemical Society · doi:10.1021/ja3010978 · Cited by 2,000
General Techno-Economic Analysis of CO 2 Electrolysis Systems
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What Should We Make with CO2 and How Can We Make It?
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Self-citationDe Luna, P., Quintero-Bermudez, R., Dinh, C.-T., Ross, M. B., Bushuyev, O. S., Todorović, P., Regier, T., Kelley, S. O., Yang, P., & Sargent, E. H. (2018) · Nature Catalysis · doi:10.1038/s41929-017-0018-9 · Cited by 1,046
Self-citationLarge-Scale and Highly Selective CO2 Electrocatalytic Reduction on Nickel Single-Atom Catalyst
Zheng, T., Jiang, K., Ta, N., Hu, Y., Zeng, J., Liu, J., & Wang, H. (2019) · Joule · doi:10.1016/j.joule.2018.10.015 · Cited by 887
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Technical photosynthesis involving CO2 electrolysis and fermentation
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One-step electrosynthesis of ethylene and ethanol from CO2 in an alkaline electrolyzer
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Cited by
CO 2 electrolysis to multicarbon products in strong acid
Huang, J. E., Li, F., Ozden, A., Sedighian Rasouli, A., García de Arquer, F. P., Liu, S., Zhang, S., Luo, M., Wang, X., Lum, Y., et al. (2021) · Science · doi:10.1126/science.abg6582 · Cited by 1,359
Self-citationYang, K., Kas, R., Smith, W. A., & Burdyny, T. (2021) · ACS Energy Letters · doi:10.1021/acsenergylett.0c02184 · Cited by 474
Bipolar membrane electrolyzers enable high single-pass CO2 electroreduction to multicarbon products
Xie, K., Miao, R. K., Ozden, A., Liu, S., Chen, Z., Dinh, C.-T., Huang, J. E., Xu, Q., Gabardo, C. M., Lee, G., et al. (2022) · Nature Communications · doi:10.1038/s41467-022-31295-3 · Cited by 270
Self-citationSisler, J., Khan, S., Ip, A. H., Schreiber, M. W., Jaffer, S. A., Bobicki, E. R., Dinh, C.-T., & Sargent, E. H. (2021) · ACS Energy Letters · doi:10.1021/acsenergylett.0c02633 · Cited by 259
Self-citationAdvanced manufacturing for electrosynthesis of fuels and chemicals from CO 2
Corral, D., Feaster, J. T., Sobhani, S., DeOtte, J. R., Lee, D. U., Wong, A. A., Hamilton, J., Beck, V. A., Sarkar, A., Hahn, C., et al. (2021) · Energy & Environmental Science · doi:10.1039/d0ee03679j · Cited by 98
Metadata
- Authors
- Gabardo, C. M., O’Brien, C. P., Edwards, J. P., McCallum, C., Xu, Y., Dinh, C.-T., Li, J., Sargent, E. H., & Sinton, D.
- Venue
- Joule
- Publisher
- Elsevier BV
- Published
- 2019-11
- Volume
- 3
- Issue
- 11
- Pages
- 2777-2791
- ISSN
- 2542-4351 (ISSN-L)
- OpenAlex
- W2969819714
- Cited by
- 611
- References
- 16
- FWCI
- 11.49
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Gabardo, C. M., O’Brien, C. P., Edwards, J. P., McCallum, C., Xu, Y., Dinh, C.-T., Li, J., Sargent, E. H., & Sinton, D. (2019). Continuous Carbon Dioxide Electroreduction to Concentrated Multi-carbon Products Using a Membrane Electrode Assembly. Joule. https://doi.org/10.1016/j.joule.2019.07.021
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
