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Recycling of spent lithium-ion battery with polyvinyl chloride by mechanochemical process
Open accessAbstract
In the present study, cathode materials (C/LiCoO2) of spent lithium-ion batteries (LIBs) and waste polyvinyl chloride (PVC) were co-processed via an innovative mechanochemical method, i.e. LiCoO2/PVC/Fe was co-grinded followed by water-leaching. This procedure generated recoverable LiCl from Li by the dechlorination of PVC and also generated magnetic CoFe4O6 from Co. The effects of different additives (e.g. alkali metals, non-metal oxides, and zero-valent metals) on (i) the conversion rates of Li and Co and (ii) the dechlorination rate of PVC were investigated, and the reaction mechanisms were explored. It was found that the chlorine atoms in PVC were mechanochemically transformed into chloride ions that bound to the Li in LiCoO2 to form LiCl. This resulted in reorganization of the Co and Fe crystals to form the magnetic material CoFe4O6. This study provides a more environmentally-friendly, economical, and straightforward approach for the recycling of spent LIBs and waste PVC compared to traditional processes.
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Xin, Y., Guo, X., Chen, S., Wang, J., Wu, F., & Xin, B. (2016) · Journal of Cleaner Production · doi:10.1016/j.jclepro.2016.01.001 · Cited by 306
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Harper, G., Sommerville, R., Kendrick, E., Driscoll, L., Slater, P., Stolkin, R., Walton, A., Christensen, P., Heidrich, O., Lambert, S., et al. (2019) · Nature · doi:10.1038/s41586-019-1682-5 · Cited by 3,890
A Critical Review and Analysis on the Recycling of Spent Lithium-Ion Batteries
Lv, W., Wang, Z., Cao, H., Sun, Y., Zhang, Y., & Sun, Z. (2018) · ACS Sustainable Chemistry & Engineering · doi:10.1021/acssuschemeng.7b03811 · Cited by 1,163
Toward sustainable and systematic recycling of spent rechargeable batteries
Zhang, X., Li, L., Fan, E., Xue, Q., Bian, Y., Wu, F., & Chen, R. (2018) · Chemical Society Reviews · doi:10.1039/c8cs00297e · Cited by 1,038
Recycling of spent lithium-ion batteries in view of lithium recovery: A critical review
Liu, C., Lin, J., Cao, H., Zhang, Y., & Sun, Z. (2019) · Journal of Cleaner Production · doi:10.1016/j.jclepro.2019.04.304 · Cited by 789
Mossali, E., Picone, N., Gentilini, L., Rodrìguez, O., Pérez, J. M., & Colledani, M. (2020) · Journal of Environmental Management · doi:10.1016/j.jenvman.2020.110500 · Cited by 574
Metadata
- Authors
- Wang, M.-M., Zhang, C.-C., & Zhang, F.-S.
- Venue
- Waste Management
- Publisher
- Elsevier BV
- Published
- 2017-09
- Volume
- 67
- Pages
- 232-239
- ISSN
- 0956-053X (ISSN-L)
- OpenAlex
- W2619903364
- Cited by
- 167
- References
- 1
- FWCI
- 10.34
- Type
- journal article
- Language
- en
- Open access
- green
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- Wang, M.-M., Zhang, C.-C., & Zhang, F.-S. (2017). Recycling of spent lithium-ion battery with polyvinyl chloride by mechanochemical process. Waste Management. https://doi.org/10.1016/j.wasman.2017.05.013
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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