Cited by 3,890Extraction and Separation ProcessesAdvanced Battery Technologies ResearchRecycling and Waste Management Techniques

Recycling lithium-ion batteries from electric vehicles

Open access
Harper, Gavin, Sommerville, Roberto, Kendrick, Emma, Driscoll, Laura, Slater, Peter, Stolkin, Rustam, Walton, Allan, Christensen, Paul +6 more·2019·Nature

Abstract

Rapid growth in the market for electric vehicles is imperative, to meet global targets for reducing greenhouse gas emissions, to improve air quality in urban centres and to meet the needs of consumers, with whom electric vehicles are increasingly popular. However, growing numbers of electric vehicles present a serious waste-management challenge for recyclers at end-of-life. Nevertheless, spent batteries may also present an opportunity as manufacturers require access to strategic elements and critical materials for key components in electric-vehicle manufacture: recycled lithium-ion batteries from electric vehicles could provide a valuable secondary source of materials. Here we outline and evaluate the current range of approaches to electric-vehicle lithium-ion battery recycling and re-use, and highlight areas for future progress.

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Crossref · 10.1038/s41586-019-1682-5

Cites

95 of 95 references verified0 citation errors · 0 not checkable

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  • There are a variety of techniques used to recover materials from lithium-ion batteries, with a special focus on lithium and the other critical minerals.

    “There are a variety of techniques used to recover materials from lithium-ion batteries, with a special focus on lithium and the other critical minerals [57].”
  • Among all environmental factors, temperature has the greatest impact on the charge and discharge performance of lithium ion batteries.

    “Among all environmental factors, temperature has the greatest impact on the charge and discharge performance of lithium ion batteries [10].”

    From The Influence of Temperature on the Capacity of Lithium Ion Batteries with Different Anodes (2021) · cites this paper as [10]

    The Stabilization and passivation of end-of-life batteries section says increasing temperature shortens discharge time in a salt solution during recycling. It does not compare environmental factors or discuss temperature’s effect on normal charging and discharging performance. Searches for the claimed comparison and for temperature-related battery performance found no passage addressing it. (LLM, conf=0.77)

    Experimental — accuracy not yet measured
  • Closed-loop recycling will gain importance, depending on EV fleet and battery chemistry developments, second-use, and other factors such as standardization, legislation, business models, eco-design, collection systems, and recycling technology.

    “Closed-loop recycling will gain importance, depending on EV fleet and battery chemistry developments, second-use, and other factors, such as standardization 42 , legislation, business models 43 , eco-design or design for recycling 44 , collection systems, and recycling technology”
  • Direct recycling aims at recovering cathode materials while maintaining their chemical structures, which could be economically and environmentally advantageous, but it is currently still in early development stages.

    “Direct recycling aims at recovering cathode materials while maintaining their chemical structures, which could be economically and environmentally advantageous 28 ; however, it is currently still in early development stages”
  • The difference between recycling technologies is not so much in recycling efficiency for individual materials, but whether materials are recovered and in what chemical form and purity.

    “The difference between the recycling technologies is not so much in the recycling efficiency for individual materials, but whether materials are recovered and in what chemical form and purity”

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Cites

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Research works printed but not linked: 7

  1. Reaugh, L. American Manganese: Virtual Reality International Conference (VRIC) Conversation with President and CEO Larry Reaugh -MoonShot Exec, https:// moonshotexec.com/american-manganese-vric-conversation-with-president-and-ceo- larry-reaugh/ (2018).
  2. Cerdas, F. et al. in Recycling of Lithium-Ion Batteries 83-97 (Springer, 2018).
  3. Arora, S. & Kapoor, A. in Behaviour of Lithium-Ion Batteries in Electric Vehicles (eds Pistoia, G. & Liaw, B.) 175-200 (Springer, 2018).
  4. Advances in Battery Technologies for Electric Vehicles (eds Bruno Scrosati, B., Jürgen Garche, J. & Werner Tillmetz, W.) 245-263 (Elsevier, 2015).
  5. Luca, A., Albu-Schaffer, A., Haddadin, S. & Hirzinger, G. in 2006 IEEE/RSJ Int. Conf. on Intelligent Robots and Systems 1623-1630 (IEEE, 2006).
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Authors
Harper, G., Sommerville, R., Kendrick, E., Driscoll, L., Slater, P., Stolkin, R., Walton, A., Christensen, P., Heidrich, O., Lambert, S., Abbott, A., Ryder, K., Gaines, L., & Anderson, P.
Affiliations
  • University of Birmingham (GB)
  • University of Leicester (GB)
  • Argonne National Laboratory (US)
Corresponding author
Harper, Gavin
Venue
Nature
Published
2019-11-06
Volume
575
Issue
7781
Pages
75-86
ISSN
  • 0028-0836 (ISSN-L)
  • 1476-4687
OpenAlex
W2983762108
Cited by
3,890
References
95
Citations by year
2026: 735 · 2025: 827 · 2024: 702 · 2023: 584 · 2022: 486 · 2021: 371 · 2020: 181 · 2019: 4
FWCI
23.25
Type
journal article
Language
en
Open access
Locations
  • Nature (publishedVersion)
  • PubMed (publishedVersion)
  • RePEc: Research Papers in Economics (submittedVersion)
  • University of Birmingham Research Portal (University of Birmingham) (submittedVersion)
  • Newcastle University ePrints (Newcastle Univesity)
Funders
  • U.S. Department of Energy
  • Faraday Institution (FIRG005, FIRG005 and FIRG006, FIRG006)
  • Engineering and Physical Sciences Research Council (EP/S003053/1)
  • Argonne National Laboratory
Topics
  • Physical Sciences › Engineering › Mechanical Engineering › Extraction and Separation Processes
  • Physical Sciences › Engineering › Automotive Engineering › Advanced Battery Technologies Research
  • Physical Sciences › Environmental Science › Waste Management and Disposal › Recycling and Waste Management Techniques
Keywords
lithium-ion battery recycling, electric vehicles, spent batteries, critical raw materials recovery, end-of-life vehicles, waste management, secondary raw materials

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