Electrochemical CO2 reduction on a glassy carbon electrode under high pressure
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While the dominant products of CO2RR do not change significantly with temperature on most catalysts, studies on Cu have demonstrated that hydrocarbon selectivity tends to shift from CH4 to C2H4 as temperature increases.
“While the dominant products of CO2RR do not change significantly with temperature on most catalysts, [240] studies on Cu have demonstrated that hydrocarbon selectivity tends to shift from CH4 to C2H4 as temperature increases.[242,[245][246][247]”
From Electrochemical CO <sub>2</sub> Reduction into Chemical Feedstocks: From Mechanistic Electrocatalysis Models to System Design (2019) · cites this paper as [242]
Improved C2H4 selectivity with increasing temperature is attributed to reduced activation energies and enhanced surface diffusion of adsorbed intermediates.
“This improved C2H4 selectivity is attributed to reduced activation energies [240] and enhanced surface diffusion of adsorbed intermediates.[242]”
From Electrochemical CO <sub>2</sub> Reduction into Chemical Feedstocks: From Mechanistic Electrocatalysis Models to System Design (2019) · cites this paper as [242]
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- Authors
- Hara, K., Kudo, A., & Sakata, T.
- Affiliations
- Tokyo Institute of Technology (JP)
- Corresponding author
- Sakata, T.
- Venue
- Journal of Electroanalytical Chemistry
- Publisher
- Elsevier BV
- Published
- 1997-01
- Volume
- 421
- Issue
- 1-2
- Pages
- 1-4
- ISSN
- 1572-6657 (ISSN-L)
- OpenAlex
- W2007661145
- Cited by
- 73
- References
- 25
- Citations by year
- 2026: 5 · 2025: 3 · 2024: 4 · 2023: 3 · 2022: 3 · 2021: 6 · 2020: 8 · 2019: 6 · 2018: 5 · 2017: 3 · 2016: 5 · 2015: 6 · 2014: 2 · 2013: 6 · 2012: 1
- FWCI
- 0.00
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Journal of Electroanalytical Chemistry (publishedVersion)
- Funders
- Japan Society for the Promotion of Science
- Ministry of Education, Culture, Sports, Science and Technology
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
- Physical Sciences › Chemical Engineering › Process Chemistry and Technology › Carbon dioxide utilization in catalysis
- Physical Sciences › Chemical Engineering › Catalysis › Catalysts for Methane Reforming
- Keywords
- electrochemical CO2 reduction, high-pressure electrolysis, glassy carbon electrode, CO2 selectivity, Faradaic efficiency, carbon monoxide, formic acid, hydrocarbon generation, methane, propane, butane, current density dependence
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