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Fluorine-Free Oil Absorbents Made from Cellulose Nanofibril Aerogels
Abstract
Aerogels based on cellulose nanofibrils (CNFs) have been of great interest as absorbents due to their high absorption capacity, low density, biodegradability, and large surface area. Hydrophobic aerogels have been designed to give excellent oil absorption tendency from water. Herein, we present an in situ method for CNF surface modification and hydrophobic aerogel preparation. Neither solvent exchange nor fluorine chemical is used in aerogel preparations. The as-prepared hydrophobic aerogels exhibit low density (23.2 mg/cm(-3)), high porosity (98.5%), good flexibility, and solvent-induced shape recovery property. Successful surface modification was confirmed through field emission scanning electron microscopy (FE-SEM), Fourier transform infrared spectroscopy (FTIR), thermogravimetric analysis (TGA), and water contact angle measurements. The hydrophobic aerogels show high absorption capacities for various oils, depending on liquid density, up to 47× their original weight but with low water uptake (<0.5 g/g aerogel).
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Cites
Silica Aerogel: Synthesis and Applications
Gurav, J. L., Jung, I.-K., Park, H.-H., Kang, E. S., & Nadargi, D. Y. (2010) · Journal of Nanomaterials · doi:10.1155/2010/409310 · Cited by 756
Cited by
Chen, Y., Zhang, L., Yang, Y., Pang, B., Xu, W., Duan, G., Jiang, S., & Zhang, K. (2021) · Advanced Materials · doi:10.1002/adma.202005569 · Cited by 721
Ferroelectric Hf0.5Zr0.5O2 Thin Films: A Review of Recent Advances
Kim, S. J., Mohan, J., Summerfelt, S. R., & Kim, J. (2019) · JOM · doi:10.1007/s11837-018-3140-5 · Cited by 363
3D printing to innovate biopolymer materials for demanding applications: A review
Li, N., Qiao, D., Zhao, S., Lin, Q., Zhang, B., & Xie, F. (2021) · Materials Today Chemistry · doi:10.1016/j.mtchem.2021.100459 · Cited by 142
Hierarchical Design of 1D Building Blocks for Anisotropic Aerogel
Long, X., Qin, J., Tang, J., Xue, J., Wang, Y., Zhou, L., Wang, S., Wei, X., Lin, Y., & Liao, J. (2025) · Advanced Functional Materials · doi:10.1002/adfm.202413018 · Cited by 25
Metadata
- Authors
- Mulyadi, A., Zhang, Z., & Deng, Y.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-01-22
- Volume
- 8
- Issue
- 4
- Pages
- 2732-2740
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2233316567
- Cited by
- 225
- References
- 1
- FWCI
- 10.78
- Type
- journal article
- Language
- en
- Open access
- closed
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- Mulyadi, A., Zhang, Z., & Deng, Y. (2016). Fluorine-Free Oil Absorbents Made from Cellulose Nanofibril Aerogels. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.5b10985
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
