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RuO2–CeO2 Lattice Matching Strategy Enables Robust Water Oxidation Electrocatalysis in Acidic Media via Two Distinct Oxygen Evolution Mechanisms
Abstract
The discovery of acid-stable and highly active electrocatalysts for the oxygen evolution reaction (OER) is crucial in the quest for high-performance water-splitting technologies. Herein, a heterostructured RuO 2 –CeO 2 electrocatalyst was constructed by using a lattice-matching strategy. The interfacial Ru–O–Ce bridge structure provided a channel for electron transfer between Ru and Ce, creating a lattice stress that distorts the local structure of RuO 2 . The resulting RuO 2 –CeO 2 catalyst exhibited attractive stability with negligible decay after 1000 h of the OER in 0.5 M H 2 SO 4, along with high activity with an overpotential of only 180 mV at 10 mA cm –2 . In situ attenuated total reflectance surface-enhanced infrared absorption spectroscopy (ATR-SEIRAS), in situ differential electrochemical mass spectrometry (DEMS), and density functional theory (DFT) calculations were used to reveal that the interface and noninterface RuO 2 sites enabled an oxide path mechanism (OPM) and the enhanced adsorbate evolution mechanism (AEM-plus), respectively, during the OER. The simultaneous and independent OER pathways accessible by lattice matching guides improved electrocatalyst design for the OER in acidic media.
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Self-citation
Cited by
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Metadata
- Authors
- Song, H., Yong, X., Waterhouse, G. I. N., Yu, J., Wang, H., Cai, J., Tang, Z., Yang, B., Chang, J., & Lu, S.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2024-02-15
- Volume
- 14
- Issue
- 5
- Pages
- 3298-3307
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W4391836369
- Cited by
- 280
- References
- 45
- FWCI
- 18.50
- Type
- journal article
- Language
- en
- Open access
- closed
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