The DOI matches its Crossref record; 11 of the 11 references it cites were found in a registry or an index.
Electrochemical Reduction of CO2 on Metal-Nitrogen-Doped Carbon Catalysts
Abstract
The electrochemical CO 2 reduction reaction (CO2RR) is a promising technology for converting waste CO 2 into chemicals which could be used as feedstock for the chemical industry or as synthetic fuels. The technological viability of this process, however, is contingent on finding affordable and efficient catalysts. Recently, carbon-based solid state catalyst materials containing small amounts of nitrogen and transition metals (MNC) have emerged as a selective and cost-efficient alternative to noble metal catalysts for the direct electrochemical reduction of CO 2 into CO. In addition, other products have also been reported, including formic acid and methane. In this Perspective, we offer a focused discussion of recent advances in the field of MNC catalysts for the CO2RR. The different factors which control the catalytic performance of MNC toward the CO2RR are discussed in this Perspective. We focus on density functional theory-guided experimental studies aiming to elucidate key experimental parameters and molecular descriptors that control the activity and selectivity of this class of materials. We close addressing the remaining challenges and take a look forward into future studies.
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Cites
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Cited by
Electrocatalysis for CO 2 conversion: from fundamentals to value-added products
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Single atom electrocatalysts supported on graphene or graphene-like carbons
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High‐Entropy Nanomaterials for Advanced Electrocatalysis
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Metadata
- Authors
- Varela, A. S., Ju, W., Bagger, A., Franco, P., Rossmeisl, J., & Strasser, P.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2019-06-28
- Volume
- 9
- Issue
- 8
- Pages
- 7270-7284
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2956042519
- Cited by
- 390
- References
- 11
- FWCI
- 10.05
- Type
- journal article
- Language
- en
- Open access
- closed
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- Varela, A. S., Ju, W., Bagger, A., Franco, P., Rossmeisl, J., & Strasser, P. (2019). Electrochemical Reduction of CO2 on Metal-Nitrogen-Doped Carbon Catalysts. ACS Catalysis. https://doi.org/10.1021/acscatal.9b01405
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