The DOI matches its Crossref record; 13 of the 13 references it cites were found in a registry or an index.
Trimetallic NiFeMo for Overall Electrochemical Water Splitting with a Low Cell Voltage
Abstract
We report the development of an efficient and earth-abundant catalyst for electrochemical overall water splitting. Trimetallic NiFeMo alloy is synthesized by hydrothermal deposition from inorganic precursors and subsequent low-temperature thermal annealing. A complete cell made of NiFeMo electrodes on nickel foam exhibits a low voltage of 1.45 V at 10 mA/cm 2 as a result of low overpotentials for both hydrogen evolution reaction (HER) and oxygen evolution reaction (OER). High-resolution transmission electron microscopy reveals that nanometer-sized single-crystal domains of Ni, Fe, and Mo are intimately integrated at the atomic level, which enables a synergistic effect of metallic Ni, Fe, and Mo for efficient HER, while self-formed Ni–Fe–Mo (oxy)hydroxides on the surface of the NiFeMo anode become active sites for OER. Such a multimetallic alloy and its (oxy)hydroxides represent a typical HER/OER catalyst couple, and our method provides a new route to develop efficient low-cost metallic alloys for overall water splitting.
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Cites
Combining theory and experiment in electrocatalysis: Insights into materials design
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Electrocatalysis for the oxygen evolution reaction: recent development and future perspectives
Suen, N.-T., Hung, S.-F., Quan, Q., Zhang, N., Xu, Y.-J., & Chen, H. M. (2017) · Chemical Society Reviews · doi:10.1039/c6cs00328a · Cited by 6,307
Noble metal-free hydrogen evolution catalysts for water splitting
Zou, X., & Zhang, Y. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00448e · Cited by 5,955
McCrory, C. C. L., Jung, S., Ferrer, I. M., Chatman, S. M., Peters, J. C., & Jaramillo, T. F. (2015) · Journal of the American Chemical Society · doi:10.1021/ja510442p · Cited by 4,145
Nanostructured Nickel Phosphide as an Electrocatalyst for the Hydrogen Evolution Reaction
Popczun, E. J., McKone, J. R., Read, C. G., Biacchi, A. J., Wiltrout, A. M., Lewis, N. S., & Schaak, R. E. (2013) · Journal of the American Chemical Society · doi:10.1021/ja403440e · Cited by 2,911
Water photolysis at 12.3% efficiency via perovskite photovoltaics and Earth-abundant catalysts
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Ni–Mo Nanopowders for Efficient Electrochemical Hydrogen Evolution
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Cited by
Chatenet, M., Pollet, B. G., Dekel, D. R., Dionigi, F., Deseure, J., Millet, P., Braatz, R. D., Bazant, M. Z., Eikerling, M., Staffell, I., et al. (2022) · Chemical Society Reviews · doi:10.1039/d0cs01079k · Cited by 2,025
Singh, T. I., Rajeshkhanna, G., Pan, U. N., Kshetri, T., Lin, H., Kim, N. H., & Lee, J. H. (2021) · Small · doi:10.1002/smll.202101312 · Cited by 312
Lian, Y., Sun, H., Wang, X., Qi, P., Mu, Q., Chen, Y., Ye, J., Zhao, X., Deng, Z., & Peng, Y. (2019) · Chemical Science · doi:10.1039/c8sc03877e · Cited by 297
Comprehensive overview of polyoxometalates for electrocatalytic hydrogen evolution reaction
Zeb, Z., Huang, Y., Chen, L., Zhou, W., Liao, M., Jiang, Y., Li, H., Wang, L., Wang, L., Wang, H., et al. (2023) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2023.215058 · Cited by 208
Multicomponent transition metal oxides and (oxy)hydroxides for oxygen evolution
Han, J., & Guan, J. (2023) · Nano Research · doi:10.1007/s12274-022-4874-7 · Cited by 145
Metadata
- Authors
- Qin, F., Zhao, Z., Alam, M. K., Ni, Y., Robles-Hernandez, F., Yu, L., Chen, S., Ren, Z., Wang, Z., & Bao, J.
- Venue
- ACS Energy Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-02-06
- Volume
- 3
- Issue
- 3
- Pages
- 546-554
- ISSN
- 2380-8195 (ISSN-L)
- OpenAlex
- W2785671977
- Cited by
- 277
- References
- 13
- FWCI
- 6.16
- Type
- journal article
- Language
- en
- Open access
- closed
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- Qin, F., Zhao, Z., Alam, M. K., Ni, Y., Robles-Hernandez, F., Yu, L., Chen, S., Ren, Z., Wang, Z., & Bao, J. (2018). Trimetallic NiFeMo for Overall Electrochemical Water Splitting with a Low Cell Voltage. ACS Energy Letters. https://doi.org/10.1021/acsenergylett.7b01335
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