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Kirigami-Inspired Highly Stretchable, Conductive, and Hierarchical Ti3C2Tx MXene Films for Efficient Electromagnetic Interference Shielding and Pressure Sensing
Abstract
Although Ti 3 C 2 T x MXene sheets are highly conductive, it is still a challenge to design highly stretchable MXene electrodes for flexible electronic devices. Inspired by the high stretchability of kirigami patterns, we demonstrate a bottom-up methodology to design highly stretchable and conductive polydimethylsiloxane (PDMS)/Ti 3 C 2 T x MXene films for electromagnetic interference (EMI) shielding and pressure sensing applications by constructing wrinkled MXene patterns on a flexible PDMS substrate to create a hierarchical surface with primary and secondary surface wrinkles. The self-controlled microcracks created in the valley domains of the hierarchical film via a nonuniform deformation during prestretching/releasing cycles endow the hierarchical PDMS/MXene film with a high stretchability (100%), strain-invariant conductivity in a strain range of 0%–100%, and stable conductivities over an 1000-cycle fatigue measurement. The stretchable film exhibits a highly stable EMI shielding performance of ≈30 dB at a tensile strain of 50%, and its EMI shielding efficiency increases further to 103 dB by constructing a two-film structure. Furthermore, a highly stretchable and sensitive iontronic sensor array with integrated MXene-based electrodes and circuits is fabricated by a stencil printing process, exhibiting high sensitivity (66.3 nF kPa –1 ), excellent dynamic cycle stability over 1000 cycles under different frequencies, and sensitive pressure monitoring capability under a tensile strain of 50%.
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Metadata
- Authors
- Chen, W., Liu, L.-X., Zhang, H.-B., & Yu, Z.-Z.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2021-04-16
- Volume
- 15
- Issue
- 4
- Pages
- 7668-7681
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W3153530198
- Cited by
- 293
- References
- 64
- FWCI
- 16.13
- Type
- journal article
- Language
- en
- Open access
- closed
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