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Core–Shell Layered Double Hydroxide Microspheres with Tunable Interior Architecture for Supercapacitors
Abstract
Core–shell layered double hydroxide microspheres with tunable interior architecture have been synthesized by a facile and cost-effective in situ growth method. The SEM and TEM images revealed that the obtained microspheres display a three-dimensional architecture with core–shell, yolk–shell, and hollow interior structure respectively, with continuous changes in specific surface area and pore-size distribution. Moreover, the hollow NiAl-LDH microspheres exhibit excellent pseudocapacitance performance, including high specific capacitance and rate capability, good charge/discharge stability and long-term cycling life, owing to the greatly improved faradaic redox reaction and mass transfer. Therefore, this work provides a promising approach for the design and synthesis of structure tunable materials with largely enhanced supercapacitor behavior, which can be potentially applied in energy storage/conversion devices.
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Self-citation
Metadata
- Authors
- Shao, M., Ning, F., Zhao, Y., Zhao, J., Wei, M., Evans, D. G., & Duan, X.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-03-13
- Volume
- 24
- Issue
- 6
- Pages
- 1192-1197
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2335113428
- Cited by
- 384
- References
- 31
- FWCI
- 12.99
- Type
- journal article
- Language
- en
- Open access
- closed
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