The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Electrocatalytic Polysulfide Traps for Controlling Redox Shuttle Process of Li–S Batteries
Abstract
Stabilizing the polysulfide shuttle while ensuring high sulfur loading holds the key to realizing high theoretical energy of lithium-sulfur (Li-S) batteries. Herein, we present an electrocatalysis approach to demonstrate preferential adsorption of a soluble polysulfide species, formed during discharge process, toward the catalyst anchored sites of graphene and their efficient transformation to long-chain polysulfides in the subsequent redox process. Uniform dispersion of catalyst nanoparticles on graphene layers has shown a 40% enhancement in the specific capacity over pristine graphene and stability over 100 cycles with a Coulombic efficiency of 99.3% at a current rate of 0.2 C. Interaction between electrocatalyst and polysulfides has been evaluated by conducting X-ray photoelectron spectroscopy and electron microscopy studies at various electrochemical conditions.
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Citations
Cites
Li-O2 and Li-S batteries with high energy storage
Bruce, P. G., Freunberger, S. A., Hardwick, L. J., & Tarascon, J.-M. (2012) · Nature Materials · doi:10.1038/nmat3191 · Cited by 9,479
Cited by
Review on High‐Loading and High‐Energy Lithium–Sulfur Batteries
Peng, H., Huang, J., Cheng, X., & Zhang, Q. (2017) · Advanced Energy Materials · doi:10.1002/aenm.201700260 · Cited by 1,746
Current Status and Future Prospects of Metal–Sulfur Batteries
Chung, S., & Manthiram, A. (2019) · Advanced Materials · doi:10.1002/adma.201901125 · Cited by 622
A novel synergistic composite with multi-functional effects for high-performance Li–S batteries
Li, Y.-J., Fan, J.-M., Zheng, M.-S., & Dong, Q.-F. (2016) · Energy & Environmental Science · doi:10.1039/c6ee00104a · Cited by 600
Zhang, J., Hu, H., Li, Z., & Lou, X. W. (. (2016) · Angewandte Chemie International Edition · doi:10.1002/anie.201511632 · Cited by 560
Porous membranes in secondary battery technologies
Lu, W., Yuan, Z., Zhao, Y., Zhang, H., Zhang, H., & Li, X. (2017) · Chemical Society Reviews · doi:10.1039/c6cs00823b · Cited by 479
Metadata
- Authors
- Al Salem, H., Babu, G., V. Rao, C., & Arava, L. M. R.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-09-08
- Volume
- 137
- Issue
- 36
- Pages
- 11542-11545
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2272188882
- Cited by
- 753
- References
- 1
- FWCI
- 25.82
- Type
- journal article
- Language
- en
- Open access
- closed
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Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
