The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Healing High-Loading Sulfur Electrodes with Unprecedented Long Cycling Life: Spatial Heterogeneity Control
Abstract
Self-healing capability helps biological systems to maintain their survivability and extend their lifespan. Similarly, self-healing is also beneficial to next-generation secondary batteries because high-capacity electrode materials, especially the cathodes such as oxygen or sulfur, suffer from shortened cycle lives resulting from irreversible and unstable phase transfer. Herein, by mimicking a biological self-healing process, fibrinolysis, we introduced an extrinsic healing agent, polysulfide, to enable the stable operation of sulfur microparticle (SMiP) cathodes. An optimized capacity (∼3.7 mAh cm –2 ) with almost no decay after 2000 cycles at a high sulfur loading of 5.6 mg (S) cm –2 was attained. The inert SMiP is activated by the solubilization effect of polysulfides whereas the unstable phase transfer is mediated by mitigated spatial heterogeneity of polysulfides, which induces uniform nucleation and growth of solid compounds. The comprehensive understanding of the healing process, as well as of the spatial heterogeneity, could further guide the design of novel healing agents (e.g., lithium iodine) toward high-performance rechargeable batteries.
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Li-O2 and Li-S batteries with high energy storage
Bruce, P. G., Freunberger, S. A., Hardwick, L. J., & Tarascon, J.-M. (2012) · Nature Materials · doi:10.1038/nmat3191 · Cited by 9,479
A review on the key issues for lithium-ion battery management in electric vehicles
Lu, L., Han, X., Li, J., Hua, J., & Ouyang, M. (2013) · Journal of Power Sources · doi:10.1016/j.jpowsour.2012.10.060 · Cited by 4,837
Mechanisms linking obesity with cardiovascular disease
Van Gaal, L. F., Mertens, I. L., & De Block, C. E. (2006) · Nature · doi:10.1038/nature05487 · Cited by 2,814
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Cited by
Current Status and Future Prospects of Metal–Sulfur Batteries
Chung, S., & Manthiram, A. (2019) · Advanced Materials · doi:10.1002/adma.201901125 · Cited by 622
Zhang, Z., Peng, H., Zhao, M., & Huang, J. (2018) · Advanced Functional Materials · doi:10.1002/adfm.201707536 · Cited by 357
Self-citationToward Practical High‐Energy‐Density Lithium–Sulfur Pouch Cells: A Review
Chen, Z., Zhao, M., Hou, L., Zhang, X., Li, B., & Huang, J. (2022) · Advanced Materials · doi:10.1002/adma.202201555 · Cited by 282
Self-citationCathode Kinetics Evaluation in Lean-Electrolyte Lithium–Sulfur Batteries
Chen, Z.-X., Cheng, Q., Li, X.-Y., Li, Z., Song, Y.-W., Sun, F., Zhao, M., Zhang, X.-Q., Li, B.-Q., & Huang, J.-Q. (2023) · Journal of the American Chemical Society · doi:10.1021/jacs.3c02786 · Cited by 279
Self-citationEdström, K., Dominko, R., Fichtner, M., & Perraud, S. (2020) · doi:10.33063/diva2-1452023 · Cited by 46
Metadata
- Authors
- Peng, H.-J., Huang, J.-Q., Liu, X.-Y., Cheng, X.-B., Xu, W.-T., Zhao, C.-Z., Wei, F., & Zhang, Q.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-03-28
- Volume
- 139
- Issue
- 25
- Pages
- 8458-8466
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2596235730
- Cited by
- 224
- References
- 4
- FWCI
- 14.43
- Type
- journal article
- Language
- en
- Open access
- closed
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- Peng, H.-J., Huang, J.-Q., Liu, X.-Y., Cheng, X.-B., Xu, W.-T., Zhao, C.-Z., Wei, F., & Zhang, Q. (2017). Healing High-Loading Sulfur Electrodes with Unprecedented Long Cycling Life: Spatial Heterogeneity Control. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.6b12358
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