The DOI matches its Crossref record; 54 of the 54 references it cites were found in a registry or an index.
Selective CO2 Reduction Catalyzed by Single Cobalt Sites on Carbon Nitride under Visible-Light Irradiation
Open accessAbstract
Framework nitrogen atoms of carbon nitride (C 3 N 4 ) can coordinate with and activate metal sites for catalysis. In this study, C 3 N 4 was employed to harvest visible light and activate Co 2+ sites, without the use of additional ligands, in photochemical CO 2 reduction. Photocatalysts containing single Co 2+ sites on C 3 N 4 were prepared by a simple deposition method and demonstrated excellent activity and product selectivity toward CO formation. A turnover number of more than 200 was obtained for CO production using the synthesized photocatalyst under visible-light irradiation. Inactive cobalt oxides formed at relatively high cobalt loadings but did not alter product selectivity. Further studies with X-ray absorption spectroscopy confirmed the presence of single Co 2+ sites on C 3 N 4 and their important role in achieving selective CO 2 reduction.
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Zhong, W., Sa, R., Li, L., He, Y., Li, L., Bi, J., Zhuang, Z., Yu, Y., & Zou, Z. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.9b02997 · Cited by 769
Metadata
- Authors
- Huang, P., Huang, J., Pantovich, S. A., Carl, A. D., Fenton, T. G., Caputo, C. A., Grimm, R. L., Frenkel, A. I., & Li, G.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-11-10
- Volume
- 140
- Issue
- 47
- Pages
- 16042-16047
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2900060043
- Cited by
- 391
- References
- 54
- FWCI
- 8.71
- Type
- journal article
- Language
- en
- Open access
- green
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- Huang, P., Huang, J., Pantovich, S. A., Carl, A. D., Fenton, T. G., Caputo, C. A., Grimm, R. L., Frenkel, A. I., & Li, G. (2018). Selective CO2 Reduction Catalyzed by Single Cobalt Sites on Carbon Nitride under Visible-Light Irradiation. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.8b10380
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