The DOI matches its Crossref record; 7 of the 7 references it cites were found in a registry or an index.
A Cobalt–Iron Double-Atom Catalyst for the Oxygen Evolution Reaction
Open accessAbstract
Single-atom catalysts exhibit well-defined active sites and potentially maximum atomic efficiency. However, they are unsuitable for reactions that benefit from bimetallic promotion such as the oxygen evolution reaction (OER) in an alkaline medium. Here we show that a single-atom Co precatalyst can be in situ transformed into a Co-Fe double-atom catalyst for the OER. This catalyst exhibits one of the highest turnover frequencies among metal oxides. Electrochemical, microscopic, and spectroscopic data, including those from operando X-ray absorption spectroscopy, reveal a dimeric Co-Fe moiety as the active site of the catalyst. This work demonstrates double-atom catalysis as a promising approach for the development of defined and highly active OER catalysts.
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Citations
Cites
Benchmarking Heterogeneous Electrocatalysts for the Oxygen Evolution Reaction
McCrory, C. C. L., Jung, S., Peters, J. C., & Jaramillo, T. F. (2013) · Journal of the American Chemical Society · doi:10.1021/ja407115p · Cited by 7,026
Electrocatalysis for the oxygen evolution reaction: recent development and future perspectives
Suen, N.-T., Hung, S.-F., Quan, Q., Zhang, N., Xu, Y.-J., & Chen, H. M. (2017) · Chemical Society Reviews · doi:10.1039/c6cs00328a · Cited by 6,307
Self-citationFei, H., Dong, J., Feng, Y., Allen, C. S., Wan, C., Volosskiy, B., Li, M., Zhao, Z., Wang, Y., Sun, H., et al. (2018) · Nature Catalysis · doi:10.1038/s41929-017-0008-y · Cited by 1,973
The Mechanism of Water Oxidation: From Electrolysis via Homogeneous to Biological Catalysis
Dau, H., Limberg, C., Reier, T., Risch, M., Roggan, S., & Strasser, P. (2010) · ChemCatChem · doi:10.1002/cctc.201000126 · Cited by 1,783
Atomic cobalt on nitrogen-doped graphene for hydrogen generation
Fei, H., Dong, J., Arellano-Jiménez, M. J., Ye, G., Dong Kim, N., Samuel, E. L. G., Peng, Z., Zhu, Z., Qin, F., Bao, J., et al. (2015) · Nature Communications · doi:10.1038/ncomms9668 · Cited by 1,621
Catalysis by Supported Single Metal Atoms
Liu, J. (2017) · ACS Catalysis · doi:10.1021/acscatal.6b01534 · Cited by 1,331
Impact of nanoparticle size and lattice oxygen on water oxidation on NiFeOxHy
Roy, C., Sebok, B., Scott, S. B., Fiordaliso, E. M., Sørensen, J. E., Bodin, A., Trimarco, D. B., Damsgaard, C. D., Vesborg, P. C. K., Hansen, O., et al. (2018) · Nature Catalysis · doi:10.1038/s41929-018-0162-x · Cited by 480
Cited by
Chen, F.-Y., Wu, Z.-Y., Adler, Z., & Wang, H. (2021) · Joule · doi:10.1016/j.joule.2021.05.005 · Cited by 1,284
Oxygen Evolution Reaction in Alkaline Environment: Material Challenges and Solutions
Xie, X., Du, L., Yan, L., Park, S., Qiu, Y., Sokolowski, J., Wang, W., & Shao, Y. (2022) · Advanced Functional Materials · doi:10.1002/adfm.202110036 · Cited by 792
Electrocatalysis of Single-Atom Sites: Impacts of Atomic Coordination
Lu, B., Liu, Q., & Chen, S. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c01950 · Cited by 394
Pan, Y., Zhang, C., Liu, Z., Chen, C., & Li, Y. (2020) · Matter · doi:10.1016/j.matt.2019.11.014 · Cited by 341
Selvam, N. C. S., Du, L., Xia, B. Y., Yoo, P. J., & You, B. (2021) · Advanced Functional Materials · doi:10.1002/adfm.202008190 · Cited by 289
Metadata
- Authors
- Bai, L., Hsu, C.-S., Alexander, D. T. L., Chen, H. M., & Hu, X.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2019-08-16
- Volume
- 141
- Issue
- 36
- Pages
- 14190-14199
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2969028050
- Cited by
- 548
- References
- 7
- FWCI
- 14.07
- Type
- journal article
- Language
- en
- Open access
- green
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- Bai, L., Hsu, C.-S., Alexander, D. T. L., Chen, H. M., & Hu, X. (2019). A Cobalt–Iron Double-Atom Catalyst for the Oxygen Evolution Reaction. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.9b05268
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