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Doping Monolayer Graphene with Single Atom Substitutions

Wang, Hongtao, Wang, Qingxiao, Cheng, Yingchun, Li, Kun, Yao, Yingbang, Zhang, Qiang, Dong, Cezhou, Wang, Peng, Schwingenschlögl, Udo, Yang, Wei, Zhang, X. X.·2012·Nano Letters

Abstract

Functionalized graphene has been extensively studied with the aim of tailoring properties for gas sensors, superconductors, supercapacitors, nanoelectronics, and spintronics. A bottleneck is the capability to control the carrier type and density by doping. We demonstrate that a two-step process is an efficient way to dope graphene: create vacancies by high-energy atom/ion bombardment and fill these vacancies with desired dopants. Different elements (Pt, Co, and In) have been successfully doped in the single-atom form. The high binding energy of the metal-vacancy complex ensures its stability and is consistent with in situ observation by an aberration-corrected and monochromated transmission electron microscope.

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Metadata

Authors
Wang, H., Wang, Q., Cheng, Y., Li, K., Yao, Y., Zhang, Q., Dong, C., Wang, P., Schwingenschlögl, U., Yang, W., & Zhang, X. X.
Venue
Nano Letters
Published
2011-12-07
Volume
12
Issue
1
Pages
141-144
ISSN
  • 1530-6984 (ISSN-L)
  • 1530-6992
OpenAlex
W2312413687
Cited by
590
References
0
FWCI
14.10
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Doping Monolayer Graphene with Single Atom Substitutions. https://app.cochat.ai/papers/10.1021/nl2031629
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Wang, H., Wang, Q., Cheng, Y., Li, K., Yao, Y., Zhang, Q., Dong, C., Wang, P., Schwingenschlögl, U., Yang, W., & Zhang, X. X. (2012). Doping Monolayer Graphene with Single Atom Substitutions. Nano Letters. https://doi.org/10.1021/nl2031629

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