Cited by 499Groundwater and Isotope GeochemistryPaleontology and Stratigraphy of FossilsGeochemistry and Elemental Analysis

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Oxygen isotope behavior in the Sulfate-Water System

Lloyd, R. M.·1968·Journal of Geophysical Research

DOI 10.1029/jb073i018p06099

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Abstract

Fundamental data on oxygen isotope behavior in the sulfate-water system are given. Oxygen exchange rates between sulfate ions and water are very slow and show a marked pH dependence. Of the order of 10/sup +3/ to 10/sup +5/ years are required to closely approach isotopic equilibrium at earth surface conditions. Oxygen isotope fractionation experiments yielded the following relationships: Ln alpha = 3878/(t+2) -0.0034 anhydrite water (and) Ln alpha = 3251/(t+2) -0.0056 dissolved sulfate water. During progressive evaporation of saturated CaSO/sub 4/ solution the gypsum formed tends to concentrate oxygen-18 relative to dissolved sulfate by 2%. Sulfate reducing bacteria preferentially metabolize oxygen-16 by about 4.6% in both pure and natural cultures. Oxidation of sulfide to sulfate in natural environments is a complex process making use of both water oxygen and molecular oxygen.

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Authors: Lloyd, R. M.
Corresponding author: Lloyd, R. M.
Venue: Journal of Geophysical Research
Publisher: American Geophysical Union (AGU)
Published: 1968-09-15
Volume: 73
Issue: 18
Pages: 6099-6110
ISSN: 0148-0227 (ISSN-L)
DOI: 10.1029/jb073i018p06099
OpenAlex: W2112478326
Cited by: 499
References: 13
Citations by year: 2026: 8 · 2025: 18 · 2024: 10 · 2023: 8 · 2022: 8 · 2021: 27 · 2020: 14 · 2019: 15 · 2018: 11 · 2017: 17 · 2016: 19 · 2015: 16 · 2014: 16 · 2013: 15 · 2012: 15
FWCI: 12.57
Type: journal article
Language: en
Open access: closed
Licence: doi.wiley.com/10.1002/tdm_license_1.1 (tdm, 17152 d)
Locations: Journal of Geophysical Research Atmospheres (publishedVersion)
Topics: Physical Sciences › Earth and Planetary Sciences › Geochemistry and Petrology › Groundwater and Isotope Geochemistry
Physical Sciences › Earth and Planetary Sciences › Paleontology › Paleontology and Stratigraphy of Fossils
Physical Sciences › Earth and Planetary Sciences › Geochemistry and Petrology › Geochemistry and Elemental Analysis
Keywords: oxygen isotopes, oxygen exchange kinetics, isotope fractionation, anhydrite, gypsum, evaporation, pH dependence, sulfate-reducing bacteria, oxygen-16, sulfide oxidation, molecular oxygen, dissolved sulfate

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Oxygen isotope behavior in the Sulfate-Water System

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