The DOI matches its Crossref record; 45 of the 45 references it cites were found in a registry or an index.
Exciton diamagnetic shifts and valley Zeeman effects in monolayer WS2 and MoS2 to 65 Tesla
Open accessAbstract
In bulk and quantum-confined semiconductors, magneto-optical studies have historically played an essential role in determining the fundamental parameters of excitons (size, binding energy, spin, dimensionality and so on). Here we report low-temperature polarized reflection spectroscopy of atomically thin WS 2 and MoS 2 in high magnetic fields to 65 T. Both the A and B excitons exhibit similar Zeeman splittings of approximately −230 μeV T−1(g-factor ≃−4), thereby quantifying the valley Zeeman effect in monolayer transition-metal disulphides. Crucially, these large fields also allow observation of the small quadratic diamagnetic shifts of both A and B excitons in monolayer WS 2, from which radii of ∼1.53 and ∼1.16 nm are calculated. Further, when analysed within a model of non-local dielectric screening, these diamagnetic shifts also constrain estimates of the A and B exciton binding energies (410 and 470 meV, respectively, using a reduced A exciton mass of 0.16 times the free electron mass). These results highlight the utility of high magnetic fields for understanding new two-dimensional materials.
Overview
The claims and statistics of this paper haven’t been checked yet.
Run the check — free, no account needed. It reads the open-access text and checks the sources it cites.
Integrity signals
Registry
Cites
Statistics
Verification
Claims the paper makes
The claims and statistics of this paper haven’t been checked yet.
Run the check — free, no account needed. It reads the open-access text and checks the sources it cites.
Self-check
Percentages, sums and reported differences re-computed from the paper’s own numbers.
The self-check needs the paper’s full text.
Citations
Cites
Atomically Thin MoS 2 : A New Direct-Gap Semiconductor
Mak, K. F., Lee, C., Hone, J., Shan, J., & Heinz, T. F. (2010) · Physical Review Letters · doi:10.1103/physrevlett.105.136805 · Cited by 15,586
Emerging Photoluminescence in Monolayer MoS2
Splendiani, A., Sun, L., Zhang, Y., Li, T., Kim, J., Chim, C.-Y., Galli, G., & Wang, F. (2010) · Nano Letters · doi:10.1021/nl903868w · Cited by 9,501
Coupled Spin and Valley Physics in Monolayers ofMoS2and Other Group-VI Dichalcogenides
Xiao, D., Liu, G.-B., Feng, W., Xu, X., & Yao, W. (2012) · Physical Review Letters · doi:10.1103/physrevlett.108.196802 · Cited by 5,152
Control of valley polarization in monolayer MoS2 by optical helicity
Mak, K. F., He, K., Shan, J., & Heinz, T. F. (2012) · Nature Nanotechnology · doi:10.1038/nnano.2012.96 · Cited by 4,034
Valley polarization in MoS2 monolayers by optical pumping
Zeng, H., Dai, J., Yao, W., Xiao, D., & Cui, X. (2012) · Nature Nanotechnology · doi:10.1038/nnano.2012.95 · Cited by 3,693
Diluted magnetic semiconductors
Furdyna, J. K. (1988) · Journal of Applied Physics · doi:10.1063/1.341700 · Cited by 3,487
Spin and pseudospins in layered transition metal dichalcogenides
Xu, X., Yao, W., Xiao, D., & Heinz, T. F. (2014) · Nature Physics · doi:10.1038/nphys2942 · Cited by 2,855
Valley-selective circular dichroism of monolayer molybdenum disulphide
Cao, T., Wang, G., Han, W., Ye, H., Zhu, C., Shi, J., Niu, Q., Tan, P., Wang, E., Liu, B., et al. (2012) · Nature Communications · doi:10.1038/ncomms1882 · Cited by 2,605
Exciton Binding Energy and Nonhydrogenic Rydberg Series in Monolayer WS2
Chernikov, A., Berkelbach, T. C., Hill, H. M., Rigosi, A., Li, Y., Aslan, B., Reichman, D. R., Hybertsen, M. S., & Heinz, T. F. (2014) · Physical Review Letters · doi:10.1103/physrevlett.113.076802 · Cited by 2,546
Valley-Contrasting Physics in Graphene: Magnetic Moment and Topological Transport
Xiao, D., Yao, W., & Niu, Q. (2007) · Physical Review Letters · doi:10.1103/physrevlett.99.236809 · Cited by 2,296
Ugeda, M. M., Bradley, A. J., Shi, S.-F., da Jornada, F. H., Zhang, Y., Qiu, D. Y., Ruan, W., Mo, S.-K., Hussain, Z., Shen, Z.-X., et al. (2014) · Nature Materials · doi:10.1038/nmat4061 · Cited by 1,866
Large excitonic effects in monolayers of molybdenum and tungsten dichalcogenides
Ramasubramaniam, A. (2012) · Physical Review B · doi:10.1103/physrevb.86.115409 · Cited by 1,566
Tightly Bound Excitons in MonolayerWSe2
He, K., Kumar, N., Zhao, L., Wang, Z., Mak, K. F., Zhao, H., & Shan, J. (2014) · Physical Review Letters · doi:10.1103/physrevlett.113.026803 · Cited by 1,243
Valley-dependent optoelectronics from inversion symmetry breaking
Yao, W., Xiao, D., & Niu, Q. (2008) · Physical Review B · doi:10.1103/physrevb.77.235406 · Cited by 1,152
k · p theory for two-dimensional transition metal dichalcogenide semiconductors
Kormányos, A., Burkard, G., Gmitra, M., Fabian, J., Zólyomi, V., Drummond, N. D., & Fal’ko, V. (2015) · 2D Materials · doi:10.1088/2053-1583/2/2/022001 · Cited by 1,076
Probing excitonic dark states in single-layer tungsten disulphide
Ye, Z., Cao, T., O’Brien, K., Zhu, H., Yin, X., Wang, Y., Louie, S. G., & Zhang, X. (2014) · Nature · doi:10.1038/nature13734 · Cited by 1,025
Three-band tight-binding model for monolayers of group-VIB transition metal dichalcogenides
Liu, G.-B., Shan, W.-Y., Yao, Y., Yao, W., & Xiao, D. (2013) · Physical Review B · doi:10.1103/physrevb.88.085433 · Cited by 1,012
Theory of neutral and charged excitons in monolayer transition metal dichalcogenides
Berkelbach, T. C., Hybertsen, M. S., & Reichman, D. R. (2013) · Physical Review B · doi:10.1103/physrevb.88.045318 · Cited by 955
Magnetic control of valley pseudospin in monolayer WSe2
Aivazian, G., Gong, Z., Jones, A. M., Chu, R.-L., Yan, J., Mandrus, D. G., Zhang, C., Cobden, D., Yao, W., & Xu, X. (2015) · Nature Physics · doi:10.1038/nphys3201 · Cited by 951
Quasiparticle band structures and optical properties of strained monolayer MoS2and WS2
Shi, H., Pan, H., Zhang, Y.-W., & Yakobson, B. I. (2013) · Physical Review B · doi:10.1103/physrevb.87.155304 · Cited by 911
Valley Zeeman effect in elementary optical excitations of monolayer WSe2
Srivastava, A., Sidler, M., Allain, A. V., Lembke, D. S., Kis, A., & Imamoğlu, A. (2015) · Nature Physics · doi:10.1038/nphys3203 · Cited by 837
Breaking of Valley Degeneracy by Magnetic Field in MonolayerMoSe2
MacNeill, D., Heikes, C., Mak, K. F., Anderson, Z., Kormányos, A., Zólyomi, V., Park, J., & Ralph, D. C. (2015) · Physical Review Letters · doi:10.1103/physrevlett.114.037401 · Cited by 764
Exciton Binding Energy of Monolayer WS2
Zhu, B., Chen, X., & Cui, X. (2015) · Scientific Reports · doi:10.1038/srep09218 · Cited by 753
Role of the Seeding Promoter in MoS2 Growth by Chemical Vapor Deposition
Ling, X., Lee, Y.-H., Lin, Y., Fang, W., Yu, L., Dresselhaus, M. S., & Kong, J. (2014) · Nano Letters · doi:10.1021/nl4033704 · Cited by 694
Cudazzo, P., Tokatly, I. V., & Rubio, A. (2011) · Physical Review B · doi:10.1103/physrevb.84.085406 · Cited by 687
Komsa, H.-P., & Krasheninnikov, A. V. (2012) · Physical Review B · doi:10.1103/physrevb.86.241201 · Cited by 674
Dielectric Screening of Excitons and Trions in Single-Layer MoS2
Lin, Y., Ling, X., Yu, L., Huang, S., Hsu, A. L., Lee, Y.-H., Kong, J., Dresselhaus, M. S., & Palacios, T. (2014) · Nano Letters · doi:10.1021/nl501988y · Cited by 644
Wang, G., Marie, X., Gerber, I., Amand, T., Lagarde, D., Bouet, L., Vidal, M., Balocchi, A., & Urbaszek, B. (2015) · Physical Review Letters · doi:10.1103/physrevlett.114.097403 · Cited by 640
Valley Splitting and Polarization by the Zeeman Effect in MonolayerMoSe2
Li, Y., Ludwig, J., Low, T., Chernikov, A., Cui, X., Arefe, G., Kim, Y. D., van der Zande, A. M., Rigosi, A., Hill, H. M., et al. (2014) · Physical Review Letters · doi:10.1103/physrevlett.113.266804 · Cited by 514
Robust optical emission polarization in MoS2monolayers through selective valley excitation
Sallen, G., Bouet, L., Marie, X., Wang, G., Zhu, C. R., Han, W. P., Lu, Y., Tan, P. H., Amand, T., Liu, B. L., et al. (2012) · Physical Review B · doi:10.1103/physrevb.86.081301 · Cited by 452
Electronic structure ofMoSe2,MoS2, andWSe2. II. The nature of the optical band gaps
Coehoorn, R., Haas, C., & de Groot, R. A. (1987) · Physical Review B · doi:10.1103/physrevb.35.6203 · Cited by 416
Valley Susceptibility of an Interacting Two-Dimensional Electron System
Gunawan, O., Shkolnikov, Y. P., Vakili, K., Gokmen, T., De Poortere, E. P., & Shayegan, M. (2006) · Physical Review Letters · doi:10.1103/physrevlett.97.186404 · Cited by 341
Hanbicki, A. T., Currie, M., Kioseoglou, G., Friedman, A. L., & Jonker, B. T. (2015) · Solid State Communications · doi:10.1016/j.ssc.2014.11.005 · Cited by 331
Self-citationBeal, A. R., Knights, J. C., & Liang, W. Y. (1972) · Journal of Physics C: Solid State Physics · doi:10.1088/0022-3719/5/24/016 · Cited by 309
Synthesis of Large-Area WS2 monolayers with Exceptional Photoluminescence
McCreary, K. M., Hanbicki, A. T., Jernigan, G. G., Culbertson, J. C., & Jonker, B. T. (2016) · Scientific Reports · doi:10.1038/srep19159 · Cited by 212
Self-citationSpin-Orbit Coupling, Quantum Dots, and Qubits in Monolayer Transition Metal Dichalcogenides
Kormányos, A., Zólyomi, V., Drummond, N., & Burkard, G. (2014) · Lancaster EPrints (Lancaster University) · Cited by 192
Magneto-optics in transition metal diselenide monolayers
Wang, G., Bouet, L., Глазов, М. М., Amand, T., Ivchenko, E. L., Palleau, É., Marie, X., & Urbaszek, B. (2015) · 2D Materials · doi:10.1088/2053-1583/2/3/034002 · Cited by 177
Large‐Area Synthesis of Continuous and Uniform MoS2 Monolayer Films on Graphene
McCreary, K. M., Hanbicki, A. T., Robinson, J. T., Cobas, E., Culbertson, J. C., Friedman, A. L., Jernigan, G. G., & Jonker, B. T. (2014) · Advanced Functional Materials · doi:10.1002/adfm.201401511 · Cited by 175
Self-citationBerry Phase Modification to the Energy Spectrum of Excitons
Zhou, J., Shan, W.-Y., Yao, W., & Xiao, D. (2015) · Physical Review Letters · doi:10.1103/physrevlett.115.166803 · Cited by 142
Magneto-optics in transition metal diselenide monolayers
Wang, G., Bouet, L., Глазов, М. М., Amand, T., Ivchenko, E., Palleau, É., Marie, X., Urbaszek, B., et al. (2015) · HAL (Le Centre pour la Communication Scientifique Directe) · Cited by 140
Optical Investigation of Monolayer and Bulk Tungsten Diselenide (WSe2) in High Magnetic Fields
Mitioglu, A., Płochocka, P., del Águila, A. G., Christianen, P. C. M., Deligeorgis, G., Anghel, S., Kulyuk, L. L., & Maude, D. K. (2015) · Nano Letters · doi:10.1021/acs.nanolett.5b00626 · Cited by 139
Valley-Valley Splitting in Inversion Layers on a High-Index Surface of Silicon
Sham, L. J., Allen, S. J., Kamgar, A., & Tsui, D. C. (1978) · Physical Review Letters · doi:10.1103/physrevlett.40.472 · Cited by 129
The Band Edge Excitons in 2HMoS2
Neville, R. A., & Evans, B. L. (1976) · physica status solidi (b) · doi:10.1002/pssb.2220730227 · Cited by 82
Excitonic effects in two-dimensional semiconductors: Path integral Monte Carlo approach
Velizhanin, K. A., & Saxena, A. (2015) · Physical Review B · doi:10.1103/physrevb.92.195305 · Cited by 57
Valley Splitting and Polarization by Zeeman Effect in Monolayer MoSe2
Li, Y. (2015) · Springer theses · doi:10.1007/978-3-319-25376-3_7 · Cited by 40
Cited by
Schaibley, J. R., Yu, H., Clark, G., Rivera, P., Ross, J. S., Seyler, K. L., Yao, W., & Xu, X. (2016) · Nature Reviews Materials · doi:10.1038/natrevmats.2016.55 · Cited by 2,652
Light–valley interactions in 2D semiconductors
Mak, K. F., Xiao, D., & Shan, J. (2018) · Nature Photonics · doi:10.1038/s41566-018-0204-6 · Cited by 502
Excitons and emergent quantum phenomena in stacked 2D semiconductors
Wilson, N. P., Yao, W., Shan, J., & Xu, X. (2021) · Nature · doi:10.1038/s41586-021-03979-1 · Cited by 319
Excitonic devices with van der Waals heterostructures: valleytronics meets twistronics
Ciarrocchi, A., Tagarelli, F., Avsar, A., & Kis, A. (2022) · Nature Reviews Materials · doi:10.1038/s41578-021-00408-7 · Cited by 291
Valleytronics in transition metal dichalcogenides materials
Liu, Y., Gao, Y., Zhang, S., He, J., Yu, J., & Liu, Z. (2019) · Nano Research · doi:10.1007/s12274-019-2497-2 · Cited by 285
Metadata
- Authors
- Stier, A. V., McCreary, K. M., Jonker, B. T., Kono, J., & Crooker, S. A.
- Venue
- Nature Communications
- Published
- 2016-02-09
- Volume
- 7
- Issue
- 1
- Pages
- 10643-10643
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W1850053210
- Cited by
- 352
- References
- 45
- FWCI
- 18.34
- Type
- journal article
- Language
- en
- Open access
- gold
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
Are you an author, or do you see a problem with this page? Request a review
Data sources
Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
