Efficient and mechanically robust stretchable organic light-emitting devices by a laser-programmable buckling process
Open accessAbstract
Stretchable organic light-emitting devices are becoming increasingly important in the fast-growing fields of wearable displays, biomedical devices and health-monitoring technology. Although highly stretchable devices have been demonstrated, their luminous efficiency and mechanical stability remain impractical for the purposes of real-life applications. This is due to significant challenges arising from the high strain-induced limitations on the structure design of the device, the materials used and the difficulty of controlling the stretch-release process. Here we have developed a laser-programmable buckling process to overcome these obstacles and realize a highly stretchable organic light-emitting diode with unprecedented efficiency and mechanical robustness. The strained device luminous efficiency -70 cd A(-1) under 70% strain - is the largest to date and the device can accommodate 100% strain while exhibiting only small fluctuations in performance over 15,000 stretch-release cycles. This work paves the way towards fully stretchable organic light-emitting diodes that can be used in wearable electronic devices.
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Microelectronic technologies may ultimately reach their limits inherent in low-frequency electromagnetic fields.
“As microelectronic technologies are driven by requirements for wearable devices towards higher sensitivity, faster response, better robustness, and higher integration, they may ultimately reach their limits, which are inherent in the very nature of low-frequency electromagnetic fields [26,27,28,29,30,31].”
From The Current State of Optical Sensors in Medical Wearables (2022) · cites this paper as [27]
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Cites
Materials and Mechanics for Stretchable Electronics
Rogers, J. A., Someya, T., & Huang, Y. Y. (2010) · Science · doi:10.1126/science.1182383 · Cited by 5,071 · see citing works
Femtosecond, picosecond and nanosecond laser ablation of solids
Chichkov, B. N., Momma, C., Nolte, S., Alvensleben, F., & Tünnermann, A. (1996) · Applied Physics A Materials Science & Processing · doi:10.1007/bf01567637 · Cited by 3,066 · see citing works
An ultra-lightweight design for imperceptible plastic electronics
Kaltenbrunner, M., Sekitani, T., Reeder, J., Yokota, T., Kuribara, K., Tokuhara, T., Drack, M., Schwödiauer, R., Graz, I., Bauer-Gogonea, S., et al. (2013) · Nature · doi:10.1038/nature12314 · Cited by 2,485 · see citing works
Stretchable active-matrix organic light-emitting diode display using printable elastic conductors
Sekitani, T., Nakajima, H., Maeda, H., Fukushima, T., Aida, T., Hata, K., & Someya, T. (2009) · Nature Materials · doi:10.1038/nmat2459 · Cited by 1,769 · see citing works
Ultrathin and lightweight organic solar cells with high flexibility
Kaltenbrunner, M., White, M. S., Głowacki, E. D., Sekitani, T., Someya, T., Sariçiftçi, N. S., & Bauer, S. (2012) · Nature Communications · doi:10.1038/ncomms1772 · Cited by 1,763 · see citing works
A hemispherical electronic eye camera based on compressible silicon optoelectronics
Ko, H. C., Stoykovich, M. P., Song, J., Malyarchuk, V., Choi, W. M., Yu, C., Geddes, J. B., Xiao, J., Wang, S., Huang, Y. Y., et al. (2008) · Nature · doi:10.1038/nature07113 · Cited by 1,352 · see citing works
Flexible organic transistors and circuits with extreme bending stability
Sekitani, T., Zschieschang, U., Klauk, H., & Someya, T. (2010) · Nature Materials · doi:10.1038/nmat2896 · Cited by 1,253 · see citing works
Elastomeric polymer light-emitting devices and displays
Liang, J., Li, L., Niu, X., Yu, Z., & Pei, Q. (2013) · Nature Photonics · doi:10.1038/nphoton.2013.242 · Cited by 973 · see citing works
Ultrathin, highly flexible and stretchable PLEDs
White, M. S., Kaltenbrunner, M., Głowacki, E. D., Gutnichenko, K., Kettlgruber, G., Graz, I. M., Aazou, S., Ulbricht, C., Egbe, D. A. M., Miron, M. C., et al. (2013) · Nature Photonics · doi:10.1038/nphoton.2013.188 · Cited by 940 · see citing works
Controlled buckling of semiconductor nanoribbons for stretchable electronics
Sun, Y., Choi, W. M., Jiang, H., Huang, Y. Y., & Rogers, J. A. (2006) · Nature Nanotechnology · doi:10.1038/nnano.2006.131 · Cited by 935 · see citing works
Chiechi, R. C., Weiss, E. A., Dickey, M. D., & Whitesides, G. M. (2007) · Angewandte Chemie International Edition · doi:10.1002/anie.200703642 · Cited by 722 · see citing works
Choi, M. K., Yang, J., Kang, K., Kim, D. C., Choi, C., Park, C., Kim, S. J., Chae, S. I., Kim, J. H., Kim, J. H., et al. (2015) · Nature Communications · doi:10.1038/ncomms8149 · Cited by 706 · see citing works
Liang, J., Li, L., Tong, K., Ren, Z. F., Hu, W., Niu, X., Chen, Y., & Pei, Q. (2014) · ACS Nano · doi:10.1021/nn405887k · Cited by 674 · see citing works
Stretchable Electronics: Materials Strategies and Devices
Kim, D., & Rogers, J. A. (2008) · Advanced Materials · doi:10.1002/adma.200801788 · Cited by 651 · see citing works
Kim, R.-H., Kim, D.-H., Xiao, J., Kim, B. H., Park, S.-I., Panilaitis, B., Ghaffari, R., Yao, J., Li, M., Liu, Z., et al. (2010) · Nature Materials · doi:10.1038/nmat2879 · Cited by 637 · see citing works
Yu, Z., Niu, X., Liu, Z., & Pei, Q. (2011) · Advanced Materials · doi:10.1002/adma.201101986 · Cited by 537 · see citing works
Fukuda, K., Takeda, Y., Yoshimura, Y., Shiwaku, R., Tran, L. T., Sekine, T., Mizukami, M., Kumaki, D., & Tokito, S. (2014) · Nature Communications · doi:10.1038/ncomms5147 · Cited by 407 · see citing works
Stretchable, elastic materials and devices for solar energy conversion
Lipomi, D. J., & Bao, Z. (2011) · Energy & Environmental Science · doi:10.1039/c1ee01881g · Cited by 394 · see citing works
Wafer-scale design of lightweight and transparent electronics that wraps around hairs
Salvatore, G. A., Munzenrieder, N. S., Kinkeldei, T., Petti, L., Zysset, C., Strebel, I., Büthe, L., & Tröster, G. (2014) · Nature Communications · doi:10.1038/ncomms3982 · Cited by 317 · see citing works
Ultra-flexible solution-processed organic field-effect transistors
Yi, H. T., Payne, M. M., Anthony, J. E., et al. (2012) · Nature Communications · doi:10.1038/ncomms2263 · Cited by 302 · see citing works
On the resistivity and surface tension of the eutectic alloy of gallium and indium
Zrnić, D., & Swatik, D. S. (1969) · Journal of the Less Common Metals · doi:10.1016/0022-5088(69)90121-0 · Cited by 233 · see citing works
Stretchable Light‐Emitting Electrochemical Cells Using an Elastomeric Emissive Material
Filiatrault, H. L., Porteous, G. C., Carmichael, R. S., Davidson, G. J. E., & Carmichael, T. B. (2012) · Advanced Materials · doi:10.1002/adma.201200448 · Cited by 148 · see citing works
French, S. J., Saunders, D. J., & Ingle, G. W. (1938) · The Journal of Physical Chemistry · doi:10.1021/j100897a011 · Cited by 91 · see citing works
Light-emitting electronic skin
Vosgueritchian, M., Tok, J. B. ‐., & Bao, Z. (2013) · Nature Photonics · doi:10.1038/nphoton.2013.251 · Cited by 87 · see citing works
Highly flexible and efficient top-emitting organic light-emitting devices with ultrasmooth Ag anode
Liu, Y.-F., Feng, J., Yin, D., et al. (2012) · Optics Letters · doi:10.1364/ol.37.001796 · Cited by 32 · see citing works
Self-citationLiu, Y., Feng, J., Cui, H.-F., et al. (2013) · Nanoscale · doi:10.1039/c3nr04276f · Cited by 25 · see citing works
Self-citationStability Improved Stretchable Metallic Gratings With Tunable Grating Period in Submicron Scale
Yin, D., Feng, J., Ma, R., et al. (2015) · Journal of Lightwave Technology · doi:10.1109/jlt.2015.2430878 · Cited by 15 · see citing works
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Wearable and flexible sensors for user-interactive health-monitoring devices
Ha, M., Lim, S., & Ko, H. (2018) · Journal of Materials Chemistry B · doi:10.1039/c8tb01063c · Cited by 352 · see citing works
Jinno, H., Yokota, T., Koizumi, M., Yukita, W., Saito, M., Osaka, I., Fukuda, K., & Someya, T. (2021) · Nature Communications · doi:10.1038/s41467-021-22558-6 · Cited by 253 · see citing works
Ultrasensitive skin-like wearable optical sensors based on glass micro/nanofibers
Zhang, L., Pan, J., Zhang, Z., Wu, H., Yao, N., Cai, D., Xu, Y., Zhang, J., Sun, G., Wang, L., et al. (2020) · Opto-Electronic Advances · doi:10.29026/oea.2020.190022 · Cited by 186 · see citing works
The Current State of Optical Sensors in Medical Wearables
Vavrinsky, E., Esfahani, N. E., Hausner, M., Kuzma, A., Rezo, V., Donoval, M., & Kosnacova, H. (2022) · Biosensors · doi:10.3390/bios12040217 · Cited by 103 · see citing works
Photonic skins based on flexible organic microlaser arrays
Zhang, C., Dong, H., Zhang, C., Fan, Y., Yao, J., & Zhao, Y. S. (2021) · Science Advances · doi:10.1126/sciadv.abh3530 · Cited by 98 · see citing works
- Authors
- Yin, D., Feng, J., Ma, R., Liu, Y.-F., Zhang, Y.-L., Zhang, X.-L., Bi, Y.-G., Chen, Q.-D., & Sun, H.-B.
- Affiliations
- Jilin University (CN)
- Corresponding author
- Feng, Jing
- Sun, Hong-Bo
- ORCID
- Venue
- Nature Communications
- Published
- 2016-05-17
- Volume
- 7
- Issue
- 1
- Pages
- 11573-11573
- ISSN
- 2041-1723 (ISSN-L)
- PMC
- PMC4873666
- OpenAlex
- W2401852898
- Cited by
- 236
- References
- 27
- Citations by year
- 2026: 17 · 2025: 16 · 2024: 29 · 2023: 16 · 2022: 30 · 2021: 25 · 2020: 32 · 2019: 31 · 2018: 21 · 2017: 15 · 2016: 4
- FWCI
- 10.90
- Type
- journal article
- Language
- en
- Open access
- gold
- doi.org
- Locations
- Nature Communications (publishedVersion, cc-by)
- Europe PMC (PubMed Central) (publishedVersion, cc-by)
- PubMed Central (publishedVersion, cc-by)
- PubMed (publishedVersion)
- RePEc: Research Papers in Economics (submittedVersion)
- DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion, cc-by-sa)
- Funders
- National Natural Science Foundation of China (2011CB013000, 61590930, #61322402, 2013CBA01700, 61435005)
- National Key Research and Development Program of China (61435005, 2011CB013000, 2013CBA01700, 61590930)
- Topics
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Organic Light-Emitting Diodes Research
- Physical Sciences › Engineering › Biomedical Engineering › Advanced Sensor and Energy Harvesting Materials
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Organic Electronics and Photovoltaics
- Keywords
- mechanical robustness, luminous efficiency, wearable displays, stretchable electronics
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