The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
General technoeconomic analysis for electrochemical coproduction coupling carbon dioxide reduction with organic oxidation
Open accessAbstract
Electrochemical processes coupling carbon dioxide reduction reactions with organic oxidation reactions are promising techniques for producing clean chemicals and utilizing renewable energy. However, assessments of the economics of the coupling technology remain questionable due to diverse product combinations and significant process design variability. Here, we report a technoeconomic analysis of electrochemical carbon dioxide reduction reaction–organic oxidation reaction coproduction via conceptual process design and thereby propose potential economic combinations. We first develop a fully automated process synthesis framework to guide process simulations, which are then employed to predict the levelized costs of chemicals. We then identify the global sensitivity of current density, Faraday efficiency, and overpotential across 295 electrochemical coproduction processes to both understand and predict the levelized costs of chemicals at various technology levels. The analysis highlights the promise that coupling the carbon dioxide reduction reaction with the value-added organic oxidation reaction can secure significant economic feasibility.
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Cites
Carbon capture and storage (CCS): the way forward
Bui, M., Adjiman, C. S., Bardow, A., Anthony, E. J., Boston, A., Brown, S., Fennell, P. S., Fuss, S., Galindo, A., Hackett, L. A., et al. (2018) · Energy & Environmental Science · doi:10.1039/c7ee02342a · Cited by 4,374
CO 2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface
Dinh, C.-T., Burdyny, T., Kibria, M. G., Seifitokaldani, A., Gabardo, C. M., García de Arquer, F. P., Kiani, A., Edwards, J. P., De Luna, P., Bushuyev, O. S., et al. (2018) · Science · doi:10.1126/science.aas9100 · Cited by 2,515
General Techno-Economic Analysis of CO 2 Electrolysis Systems
Jouny, M., Luc, W., & Jiao, F. (2018) · Industrial & Engineering Chemistry Research · doi:10.1021/acs.iecr.7b03514 · Cited by 1,628
What Should We Make with CO2 and How Can We Make It?
Bushuyev, O. S., De Luna, P., Dinh, C. T., Tao, L., Saur, G., van de Lagemaat, J., Kelley, S. O., & Sargent, E. H. (2018) · Joule · doi:10.1016/j.joule.2017.09.003 · Cited by 1,593
Pérez-Fortes, M., Schöneberger, J. C., Boulamanti, A., Harrison, G., & Tzimas, E. (2016) · International Journal of Hydrogen Energy · doi:10.1016/j.ijhydene.2016.05.199 · Cited by 301
Cited by
Electrocatalytic upcycling of polyethylene terephthalate to commodity chemicals and H2 fuel
Zhou, H., Ren, Y., Li, Z., Xu, M., Wang, Y., Ge, R., Kong, X., Zheng, L., & Duan, H. (2021) · Nature Communications · doi:10.1038/s41467-021-25048-x · Cited by 769
Catalyst–electrolyte interface chemistry for electrochemical CO2 reduction
Sa, Y. J., Lee, C. W., Lee, S. Y., Na, J., Lee, U., & Hwang, Y. J. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00030b · Cited by 468
Self-citationLai, W., Qiao, Y., Zhang, J., Lin, Z., & Huang, H. (2022) · Energy & Environmental Science · doi:10.1039/d2ee00472k · Cited by 373
Endrődi, B., Samu, A., Kecsenovity, E., Halmágyi, T., Sebők, D., & Janáky, C. (2021) · Nature Energy · doi:10.1038/s41560-021-00813-w · Cited by 361
Yan, T., Chen, X., Kumari, L., Lin, J., Li, M., Fan, Q., Chi, H., Meyer, T. J., Zhang, S., & Ma, X. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00514 · Cited by 328
Metadata
- Authors
- Na, J., Seo, B., Kim, J., Lee, C. W., Lee, H., Hwang, Y. J., Min, B. K., Lee, D. K., Oh, H.-S., & Lee, U.
- Venue
- Nature Communications
- Published
- 2019-11-15
- Volume
- 10
- Issue
- 1
- Pages
- 5193-5193
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2985173269
- Cited by
- 399
- References
- 5
- FWCI
- 6.96
- Type
- journal article
- Language
- en
- Open access
- gold
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- Na, J., Seo, B., Kim, J., Lee, C. W., Lee, H., Hwang, Y. J., Min, B. K., Lee, D. K., Oh, H.-S., & Lee, U. (2019). General technoeconomic analysis for electrochemical coproduction coupling carbon dioxide reduction with organic oxidation. Nature Communications. https://doi.org/10.1038/s41467-019-12744-y
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