3D printing of tunable shape memory polymer blends

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3D Printing of Shape Memory Polymers for Flexible Electronic Devices

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Recent advances in polymer shape memory

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From rapid prototyping to home fabrication: How 3D printing is changing business model innovation

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Shape and temperature memory of nanocomposites with broadened glass transition

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3D Printing Gets a Boost and Opportunities with Polymer Materials

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Combined one-way and two-way shape memory in a glass-forming nematic network

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Strain-Based Temperature Memory Effect for Nafion and Its Molecular Origins

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Shape-memory polymers with multiple transitions: complex actively moving polymers

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Multiple shape-memory behavior and thermal-mechanical properties of peroxide cross-linked blends of linear and short-chain branched polyethylenes

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Recent Trends in the Chemistry of Shape‐Memory Polymers

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Polyolefin thermoplastics for multiple shape and reversible shape memory

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A new strategy to prepare polymer composites with versatile shape memory properties

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Organic–inorganic nanocomposite bilayers with triple shape memory effect

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Selectively actuated multi-shape memory effect of a polymer multicomposite

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Tunable Multiple‐Shape Memory Polyethylene Blends

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The quintuple-shape memory effect in electrospun nanofiber membranes

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Development of zwitterionic copolymers with multi-shape memory effects and moisture-sensitive shape memory effects

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A Facile Strategy to Fabricate Multishape Memory Polymers with Controllable Mechanical Properties

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Ionically Cross-Linked Shape Memory Polypropylene

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Phase-Change Thermoplastic Elastomer Blends for Tunable Shape Memory by Physical Design

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Chemical Cross‐linking of Polypropylenes Towards New Shape Memory Polymers

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Multi-shape memory polymers achieved by the spatio-assembly of 3D printable thermoplastic building blocks

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Triple-Shape Memory Materials Based on Cross-Linked Poly(ethylene vinyl acetate) and Poly(ε-caprolactone)

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Heating Rate Sensitive Multi-Shape Memory Polypropylene: A Predictive Material

Hoeher, R., Raidt, T., Katzenberg, F., & Tiller, J. C. (2016) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.6b04177 · Cited by 25 · see citing works

Recent Progress on Polymer Materials for Additive Manufacturing

Tan, L. J., Zhu, W., & Zhou, K. (2020) · Advanced Functional Materials · doi:10.1002/adfm.202003062 · Cited by 745 · see citing works

Extrusion 3D Printing of Polymeric Materials with Advanced Properties

Jiang, Z., Diggle, B., Tan, M. L., Viktorova, J., Bennett, C. W., & Connal, L. A. (2020) · Advanced Science · doi:10.1002/advs.202001379 · Cited by 417 · see citing works

Thermally-induced two-way shape memory polymers: Mechanisms, structures, and applications

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Stimuli-responsive materials in additive manufacturing

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Two-Way and Multiple-Way Shape Memory Polymers for Soft Robotics: An Overview

Scalet, G. (2020) · Actuators · doi:10.3390/act9010010 · Cited by 209 · see citing works

3D printing of magneto-active smart materials for advanced actuators and soft robotics applications

Khalid, M. Y., Arif, Z. U., Tariq, A., Hossain, M., Khan, K. A., & Umer, R. (2024) · European Polymer Journal · doi:10.1016/j.eurpolymj.2023.112718 · Cited by 192 · see citing works

Untethered soft actuators for soft standalone robotics

Jung, Y., Kwon, K., Lee, J., & Ko, S. H. (2024) · Nature Communications · doi:10.1038/s41467-024-47639-0 · Cited by 182 · see citing works

Active Materials for Functional Origami

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Recent Advances in the Additive Manufacturing of Stimuli‐Responsive Soft Polymers

Tariq, A., Arif, Z. U., Khalid, M. Y., Hossain, M., Rasool, P. I., Umer, R., & Ramakrishna, S. (2023) · Advanced Engineering Materials · doi:10.1002/adem.202301074 · Cited by 149 · see citing works

3D printing of stimuli-responsive hydrogel materials: Literature review and emerging applications

Arif, Z. U., Khalid, M. Y., Tariq, A., Hossain, M., & Umer, R. (2023) · Giant · doi:10.1016/j.giant.2023.100209 · Cited by 136 · see citing works

3D printed biodegradable functional temperature-stimuli shape memory polymer for customized scaffoldings

Pandey, A., Singh, G., Singh, S., Jha, K., & Prakash, C. (2020) · Journal of the mechanical behavior of biomedical materials/Journal of mechanical behavior of biomedical materials · doi:10.1016/j.jmbbm.2020.103781 · Cited by 127 · see citing works

Shape Memory Alloys and Polymers for MEMS/NEMS Applications: Review on Recent Findings and Challenges in Design, Preparation, and Characterization

Stachiv, I., Alarcón, E., & Lamac, M. (2021) · Metals · doi:10.3390/met11030415 · Cited by 126 · see citing works

4D printing of multiple shape memory polymer and nanocomposites with biocompatible, programmable and selectively actuated properties

Wan, X., He, Y., Liu, Y., & Leng, J. (2022) · Additive manufacturing · doi:10.1016/j.addma.2022.102689 · Cited by 117 · see citing works

Additive manufacturing with stimuli-responsive materials

Boydston, A. J., Cao, B., Nelson, A., Ono, R. J., Saha, A., Schwartz, J. J., & Thrasher, C. J. (2018) · Journal of Materials Chemistry A · doi:10.1039/c8ta07716a · Cited by 113 · see citing works

Styrenic block copolymer‐based thermoplastic elastomers in smart applications: Advances in synthesis, microstructure, and structure–property relationships—A review

Maji, P., & Naskar, K. (2022) · Journal of Applied Polymer Science · doi:10.1002/app.52942 · Cited by 114 · see citing works

Advances in 4D Printed Shape Memory Polymers: From 3D Printing, Smart Excitation, and Response to Applications

Zhang, J., Yin, Z., Ren, L., Liu, Q., Ren, L., Yang, X., & Zhou, X. (2022) · Advanced Materials Technologies · doi:10.1002/admt.202101568 · Cited by 110 · see citing works

4D Printing‐Encapsulated Polycaprolactone–Thermoplastic Polyurethane with High Shape Memory Performances

Rahmatabadi, D., Aberoumand, M., Soltanmohammadi, K., Soleyman, E., Ghasemi, I., Baniassadi, M., Abrinia, K., Bodaghi, M., & Baghani, M. (2022) · Advanced Engineering Materials · doi:10.1002/adem.202201309 · Cited by 109 · see citing works

Characterization of three‐dimensional printed thermal‐stimulus polylactic acid‐hydroxyapatite‐based shape memory scaffolds

Singh, G., Singh, S., Prakash, C., Kumar, R., Kumar, R., & Ramakrishna, S. (2020) · Polymer Composites · doi:10.1002/pc.25683 · Cited by 108 · see citing works

Active composites based on shape memory polymers: overview, fabrication methods, applications, and future prospects

Melly, S. K., Liu, L., Liu, Y., & Leng, J. (2020) · Journal of Materials Science · doi:10.1007/s10853-020-04761-w · Cited by 105 · see citing works

Mechanical Reliability and In Vitro Bioactivity of 3D-Printed Porous Polylactic Acid-Hydroxyapatite Scaffold

Prakash, C., Singh, G., Singh, S., Linda, W. L., Zheng, H. Y., Ramakrishna, S., & Narayan, R. J. (2021) · Journal of Materials Engineering and Performance · doi:10.1007/s11665-021-05566-x · Cited by 92 · see citing works

4D Printing via an Unconventional Fused Deposition Modeling Route to High-Performance Thermosets

Chen, Q., Han, L., Ren, J., Rong, L., Cao, P., & Advíncula, R. C. (2020) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.0c13976 · Cited by 90 · see citing works

4D Printing of Shape Memory Polymers, Blends, and Composites and Their Advanced Applications: A Comprehensive Literature Review

Kouka, M. A., Abbassi, F., Habibi, M., Chabert, F., Zghal, A., & Garnier, C. (2022) · Advanced Engineering Materials · doi:10.1002/adem.202200650 · Cited by 91 · see citing works

Dual-method molding of 4D shape memory polyimide ink

Li, X., Yang, Y., Zhang, Y., Wang, T., Yang, Z., Wang, Q., & Zhang, X. (2020) · Materials & Design · doi:10.1016/j.matdes.2020.108606 · Cited by 83 · see citing works

3D printing of multi-material composites with tunable shape memory behavior

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Mechanism and manufacturing of 4D printing: derived and beyond the combination of 3D printing and shape memory material

Feng, P., Yang, F., Jia, J., Zhang, J., Tan, W., & Shuai, C. (2024) · International Journal of Extreme Manufacturing · doi:10.1088/2631-7990/ad7e5f · Cited by 83 · see citing works

Digital Light Processing 3D Printing of Triple Shape Memory Polymer for Sequential Shape Shifting

Peng, B., Yang, Y., Gu, K., Amis, E. J., & Cavicchi, K. A. (2019) · ACS Materials Letters · doi:10.1021/acsmaterialslett.9b00262 · Cited by 79 · see citing works

Three-dimensional printing of cellulose nanofibers reinforced PHB/PCL/Fe3O4 magneto-responsive shape memory polymer composites with excellent mechanical properties

Yue, C., Li, M., Liu, Y., et al. (2021) · Additive manufacturing · doi:10.1016/j.addma.2021.102146 · Cited by 75 · see citing works

Polymer 4D printing: Advanced shape‐change and beyond

Imrie, P., & Jin, J. (2021) · Journal of Polymer Science · doi:10.1002/pol.20210718 · Cited by 67 · see citing works

Shape memory effect of three-dimensional printed products based on polypropylene/nylon 6 alloy

Peng, X., He, H., Jia, Y., Liu, H., Geng, Y., Huang, B., & Luo, C. (2019) · Journal of Materials Science · doi:10.1007/s10853-019-03366-2 · Cited by 64 · see citing works

Design of remotely, locally triggered shape-memory materials based on bicontinuous polylactide/epoxidized natural rubber thermoplastic vulcanizates via regulating the distribution of ferroferric oxide

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Programming Multistage Shape Memory and Variable Recovery Force with 4D Printing Parameters

Wang, J., Wang, Z., Song, Z., Ren, L., Liu, Q., & Ren, L. (2019) · Advanced Materials Technologies · doi:10.1002/admt.201900535 · Cited by 60 · see citing works

Effect of printing speed and part geometry on the self-deformation behaviors of 4D printed shape memory PLA using FDM

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Mass-produced SEBS/graphite nanoplatelet composites with a segregated structure for highly stretchable and recyclable strain sensors

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3D-Printable ABS Blends with Improved Scratch Resistance and Balanced Mechanical Performance

Chen, S., Lu, J., & Feng, J. (2018) · Industrial & Engineering Chemistry Research · doi:10.1021/acs.iecr.7b05074 · Cited by 48 · see citing works

A Review of Multimaterial Additively Manufactured Electronics and 4-D Printing/Origami Shape-Memory Devices: Design, Fabrication, and Implementation

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Shape transformable bifurcated stents

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A high-efficiency way to improve the shape memory property of 4D-printed polyurethane/polylactide composite by forming in situ microfibers during extrusion-based additive manufacturing

Jiang, Y., Leng, J., & Zhang, J. (2020) · Additive manufacturing · doi:10.1016/j.addma.2020.101718 · Cited by 44 · see citing works

Solid‐State Synthesis of Two Different Polymers in a Single Crystal: A Miscible Polymer Blend from a Topochemical Reaction

Hema, K., & Sureshan, K. M. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201813198 · Cited by 43 · see citing works

Preparation of Thermoplastic Polyurethane Parts Reinforced with in Situ Polylactic Acid Microfibers during Fused Deposition Modeling: The Influences of Deposition-Induced Effects

Leng, J., Wu, J., & Zhang, J. (2019) · Industrial & Engineering Chemistry Research · doi:10.1021/acs.iecr.9b04285 · Cited by 36 · see citing works

Preparation of polycarbonate/poly(lactic acid) with improved printability and processability for fused deposition modeling

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3D‐Printed Functional Polymers and Nanocomposites: Defects Characterization and Product Quality Improvement

Alo, O. A., Mauchline, D., & Otunniyi, I. O. (2021) · Advanced Engineering Materials · doi:10.1002/adem.202101219 · Cited by 28 · see citing works

Shape-memory actuators manufactured by dual extrusion multimaterial 3d printing of conductive and non-conductive filaments

Micalizzi, S., Lantada, A. D., & Maria, C. D. (2019) · Smart Materials and Structures · doi:10.1088/1361-665x/ab3b35 · Cited by 26 · see citing works

Triple-shape memory effect in 3D-printed polymers

Dai, L., Song, J., Qu, S., & Xiao, R. (2020) · eXPRESS Polymer Letters · doi:10.3144/expresspolymlett.2020.91 · Cited by 26 · see citing works

Drum Tower‐Inspired Kirigami Structures for Rapid Fabrication of Multifunctional Shape‐Memory Smart Devices with Complex and Rigid 3D Geometry in a Two‐Stage Photopolymer

Li, X., Gai, Y., Sun, M., Li, Y., & Xu, S. (2022) · Advanced Functional Materials · doi:10.1002/adfm.202205842 · Cited by 21 · see citing works

Fabrication of 3D Printed Polylactic Acid/Polycaprolactone Nanocomposites with Favorable Thermo-Responsive Cyclic Shape Memory Effects, and Crystallization and Mechanical Properties

Liu, H., Li, C., Chen, S., Chen, P., Li, J., Jian, H., Guo-yi, G., Chen, X., Zhu, X., & Wu, J. J. (2023) · Polymers · doi:10.3390/polym15061533 · Cited by 22 · see citing works

Comfort fitting shape memory elastomer with constructed strong interface based on amphiphilic hybrid Janus particles

Hu, J., Lv, G., Ning, N., Yu, B., Tian, M., & Zhang, L. (2022) · Composites Part B Engineering · doi:10.1016/j.compositesb.2022.109828 · Cited by 21 · see citing works

Water-responsive actuators based on the solution casted PVA/epoxidized-SBS two-way shape memory bilayer composite film

Ren, S., & Feng, J. (2020) · Journal of Materials Chemistry C · doi:10.1039/d0tc00086h · Cited by 20 · see citing works

Sequential shapeshifting 4D printing: programming the pathway of multi-shape transformation by 3D printing stimuli-responsive polymers

Peng, B., Yang, Y., & Cavicchi, K. A. (2020) · Multifunctional Materials · doi:10.1088/2399-7532/abcbe1 · Cited by 21 · see citing works

Shape memory polymer blends and composites for 3D and 4D printing applications

Salimon, A. I., Senatov, F. S., Kalyaev, V., & Korsunsky, A. M. (2019) · Elsevier eBooks · doi:10.1016/b978-0-12-816805-9.00006-5 · Cited by 19 · see citing works

Influence of Multiple Thermomechanical Processing of 3D Filaments Based on Polylactic Acid and Polyhydroxybutyrate on Their Rheological and Utility Properties

Plavec, R., Horváth, V., Hlaváčiková, S., Omaníková, L., Repiská, M., Medlenová, E., Feranc, J., Kruželák, J., Přikryl, R., Figalla, S., et al. (2022) · Polymers · doi:10.3390/polym14101947 · Cited by 19 · see citing works

4D printable maleated poly(styrene-b-ethylene/butylene-b-styrene) / Poly(ethylene-co-vinyl acetate) thermoplastic elastomer blends; effects of blend composition on shape memory and mechanical properties

Tekay, E., Aybakan, B., & Aslan, V. U. (2023) · Additive manufacturing · doi:10.1016/j.addma.2023.103870 · Cited by 18 · see citing works

Solid‐State Synthesis of Two Different Polymers in a Single Crystal: A Miscible Polymer Blend from a Topochemical Reaction

Hema, K., & Sureshan, K. M. (2019) · Angewandte Chemie · doi:10.1002/ange.201813198 · Cited by 17 · see citing works

4D Printed Bifurcated Stents with Kirigami-Inspired Structures

Kim, D., Kim, T., & Lee, Y. (2019) · Journal of Visualized Experiments · doi:10.3791/59746 · Cited by 17 · see citing works

Characterization of in-House-Developed Mn-ZnO-Reinforced Polyethylene: A Sustainable Approach for Developing Fused Filament Fabrication-Based Filament

Kumar, R., Singh, R., Kumar, V., Kumar, P., Prakesh, C., & Singh, S. (2021) · Journal of Materials Engineering and Performance · doi:10.1007/s11665-021-05801-5 · Cited by 16 · see citing works

Reconfigurable Manipulation of Sound with a Multimaterial 3D Printed Origami Metasurface

Le, D. H., Kronowetter, F., Chiang, Y. K., et al. (2025) · Advanced Materials Technologies · doi:10.1002/admt.202401660 · Cited by 14 · see citing works

Reconfigurable and Reprocessable Thermadapt Stress‐Free Two‐Way Shape Memory Polymers Based on a Dual Crosslinking Network with Outstanding Mechanical Properties

Ren, S., & Feng, J. (2023) · Advanced Materials Technologies · doi:10.1002/admt.202300029 · Cited by 14 · see citing works

Research Status and Potential Direction for Thermoplastic Shape Memory Polymers and Composites: A Review

Yang, S., He, Y., Song, Z., & Li, Y. (2025) · Polymers · doi:10.3390/polym17101360 · Cited by 14 · see citing works

Preparation of Soft Shape Memory Polymer and Its Application as a Compliant Thermal‐Triggered Gripper

Li, H., Luo, Y., & Gao, X. Y. (2019) · Macromolecular Chemistry and Physics · doi:10.1002/macp.201900229 · Cited by 12 · see citing works

Microstructure evolution during cooling and reheating of the physical gel composed of SEBS copolymer and crystallizable paraffin

Zhao, S., Yang, Y., Wang, X., et al. (2021) · Polymer · doi:10.1016/j.polymer.2021.124442 · Cited by 11 · see citing works

Thermally-triggered multi-shape-memory behavior of binary blends of cross-linked EPDM with various thermoplastic polyethylenes and their potential applications as temperature indicators

Pommer, R., Saf, R., Supplit, R., Holzner, A., Plank, H., & Trimmel, G. (2023) · Polymer · doi:10.1016/j.polymer.2023.126302 · Cited by 10 · see citing works

Experimental investigations of temperature-sensitive shape memory polymer composites for 4D printing

Dixit, G., & Pandey, P. M. (2024) · Journal of Thermoplastic Composite Materials · doi:10.1177/08927057241254322 · Cited by 11 · see citing works

Design of thermally triggered triple-shape memory ternary polymer blends for 4D printing applications

Tekay, E., Aybakan, B., & Aslan, V. U. (2025) · Reactive and Functional Polymers · doi:10.1016/j.reactfunctpolym.2025.106188 · Cited by 9 · see citing works

Heterotelechelic poly(propylene oxide) as migration-inhibited toughening agent in hot lithography based additive manufacturing

Grunenberg, D., Ehrmann, K., Gorsche, C., Steyrer, B., Koch, T., Stampfl, J., & Liska, R. (2021) · Polymer Chemistry · doi:10.1039/d0py01746a · Cited by 9 · see citing works

3D printability of highly ductile poly(ethylene glycol‐co‐cyclohexane‐1,4‐dimethanol terephthalate) ‐EMAA blends

Silva, P. A. P., da Silva, A. B., Erbetta, C. D. C., et al. (2021) · Polymer Engineering and Science · doi:10.1002/pen.25693 · Cited by 9 · see citing works

Shape fixing abilities of SEBS/Paraffin blends with different paraffins under conventional and reversible plasticity shape memory programming

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A Novel Multiscale Methodology for Simulating Droplet Morphology Evolution during Injection Molding of Polymer Blends

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