Cited by 963High Entropy Alloys StudiesElectrocatalysts for Energy ConversionMachine Learning in Materials Science

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High-entropy energy materials: challenges and new opportunities

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Ma, Yanjiao, Ma, Yuan, Wang, Qingsong, Schweidler, Simon, Botros, Miriam, Fu, Tongtong, Hahn, Horst, Brezesinski, Torsten, Breitung, Ben·2021·Energy & Environmental Science

DOI 10.1039/d1ee00505g

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Abstract

An overview of high-entropy materials for energy applications, including H 2 catalysis and storage, CO 2 conversion, O 2 catalysis and electrochemical energy storage, is given and the challenges and opportunities within this field are discussed.

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“High-entropy materials have been regarded as rising stars in renewable energy technology owing to their unpredicted physical, chemical and mechanical properties22–25.”
High-entropy oxides for catalysis: A diamond in the rough
Pan, Y., Liu, J., Tianzhe, T., Wang, W., & Zhang, G. (2022) · Chemical Engineering Journal · doi:10.1016/j.cej.2022.138659 · Cited by 234
Recent advances in Ru/Ir-based electrocatalysts for acidic oxygen evolution reaction
Gao, G., Sun, Z., Chen, X., Zhu, G., Sun, B., Yamauchi, Y., & Liu, S. (2023) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2023.123584 · Cited by 196
High-entropy alloy electrocatalysts go to (sub-)nanoscale
Li, M., Lin, F., Zhang, S., Zhao, R., Tao, L., Li, L., Li, J., Zeng, L., Luo, M., & Guo, S. (2024) · Science Advances · doi:10.1126/sciadv.adn2877 · Cited by 177
Biohydrogen production from microalgae for environmental sustainability
Li, S., Li, F., Zhu, X., Liao, Q., Chang, J., & Ho, S. (2021) · Chemosphere · doi:10.1016/j.chemosphere.2021.132717 · Cited by 223
A map of single-phase high-entropy alloys
Chen, W., Hilhorst, A., Bokas, G., Gorsse, S., Jacques, P., & Hautier, G. (2022) · Nature Communications · doi:10.1038/s41467-023-38423-7 · Cited by 150
Recent status and challenging perspective of high entropy oxides for chemical catalysis
Wang, Y., Mi, J., & Wu, Z. (2022) · Chem Catalysis · doi:10.1016/j.checat.2022.05.003 · Cited by 135
Advances in high entropy oxides: synthesis, structure, properties and beyond
Liu, C., Li, S.-P., Zheng, Y., Xu, M., Su, H.-Y., Miao, X., Liu, Y., Zhou, Z.-F., Qi, J., Yang, B., et al. (2024) · Progress in Materials Science · doi:10.1016/j.pmatsci.2024.101385 · Cited by 134
High-entropy oxides for catalysis: status and perspectives
Gao, Y., Liu, Y.-Z., Yu, H., & Zou, D.-L. (2022) · Applied Catalysis A : General · doi:10.1016/j.apcata.2022.118478 · Cited by 126
Synthetic methods for high-entropy nanomaterials
Kar, N., & Skrabalak, S. E. (2025) · Nature Reviews Materials · doi:10.1038/s41578-025-00829-8 · Cited by 147
“The atomic-scale mixing of elements within a nanomaterial is key to its properties, including catalytic performance, durability, plasmonic properties and more 33–36 .”
Achieving high energy storage properties in perovskite oxide via high-entropy design
Ning, Y., Pu, Y., Zhang, Q., Zhou, S., Wu, C., Zhang, L., Shi, Y. J., & Sun, Z. (2022) · Ceramics International · doi:10.1016/j.ceramint.2022.12.073 · Cited by 118
Porous Nanoarchitectures of Nonprecious Metal Borides: From Controlled Synthesis to Heterogeneous Catalyst Applications
Kang, Y., Tang, Y., Zhu, L., Jiang, B., Xu, X., Guselnikova, O., Li, H., Asahi, T., & Yamauchi, Y. (2022) · ACS Catalysis · doi:10.1021/acscatal.2c03480 · Cited by 107
Review on electrospinning anode and separators for lithium ion batteries
Liu, J.-H., Wang, P., Gao, Z., Li, X.-H., Cui, W., Li, R., Ramakrishna, S., Zhang, J., & Long, Y.-Z. (2024) · Renewable & Sustainable Energy Reviews · doi:10.1016/j.rser.2023.113939 · Cited by 102
General synthesis of high-entropy single-atom nanocages for electrosynthesis of ammonia from nitrate
Tang, S., Xie, M., Yu, S., Zhan, X., Wei, R., Wang, M., Guan, W., Zhang, B., Wang, Y., Zhou, H., et al. (2024) · Nature Communications · doi:10.1038/s41467-024-51112-3 · Cited by 128
“The emerging methodology of advanced materials design, harnessing con ﬁ gurational entropy to prompt diverse interactions among incorporated elements (known as the “ cocktail effect ” ), often imparts these materials with unparalleled properties 17,18,20,23 .”
Emerging high-entropy compounds for electrochemical energy storage and conversion
Liu, D., Guo, P., Pan, H., & Wu, R. (2024) · Progress in Materials Science · doi:10.1016/j.pmatsci.2024.101300 · Cited by 114
High Entropy Activated and Stabilized Nickel-based Prussian Blue Analogue for High-performance Aqueous Sodium-ion Batteries
Ran, B., Cheng, R.-Q., Zhong, Y., Zhang, X., Zhao, T.-S., Yang, Z., Yang, C., Zhang, J., & Fu, C.-P. (2024) · Energy Storage Materials · doi:10.1016/j.ensm.2024.103583 · Cited by 91
High-entropy alloys in catalyses and supercapacitors: Progress, prospects
Wang, Y., & Wang, Y. (2022) · Nano Energy · doi:10.1016/j.nanoen.2022.107958 · Cited by 104
High-entropy engineering with regulated defect structure and electron interaction tuning active sites for trifunctional electrocatalysis
Zou, X.-X., Xie, J., Mei, Z.-J., Jing, Q., Sheng, X.-L., Zhang, C., Yang, Y.-X., Sun, M., Ren, F., Wang, L., et al. (2024) · Proceedings of the National Academy of Sciences of the United States of America · doi:10.1073/pnas.2313239121 · Cited by 87
“…each element has different atomic radii, chemical bonding, and crystal structure, mixing so many elements increases lattice distortion, so the flexibility for crystallographic defect optimizes the electronic structure of HEANs allowing catalytic activity and selectivity to be fine - tuned (5–9).”
Background
High‐performance ferroelectric based materials via high‐entropy strategy: Design, properties, and mechanism
Zhang, Y.-Y., Chen, L., Liu, H., Deng, S., Qi, H., & Chen, J. (2023) · InfoMat · doi:10.1002/inf2.12488 · Cited by 87
Surface-engineered nanostructured high-entropy alloys for advanced electrocatalysis
Cai, J. R., & Zhu, H. (2025) · Communications Materials · doi:10.1038/s43246-025-00838-8 · Cited by 96
A High-Entropy Multicationic Substituted Lithium Argyrodite Superionic Solid Electrolyte
Lin, J. C., Cherkashinin, G., Schaller, M., Melinte, G. A., Indris, S., Kondrakov, A., Janek, J., Brezesinski, T., & Strauss, F. (2022) · ACS Materials Letters · doi:10.1021/acsmaterialslett.2c00667 · Cited by 109
Self-citation
High-Entropy Approach vs. Traditional Doping Strategy for Layered Oxide Cathodes in Alkali-Metal-Ion Batteries: A Comparative Study
Ma, Y., Du, H., Zheng, S., Zhou, Z., Zhang, H., Ma, Y., Passerini, S., & Wu, Y. (2025) · Energy storage materials · doi:10.1016/j.ensm.2025.104295 · Cited by 75
“The synergistic effects of multiple elements, arising from their subtle interactions during mixing, are one of the key factors contributing to the overall performance enhancement of HE-TMLO [180,190].”
InfluentialSelf-citation
Lignin-Based Carbon Dots as High-Performance Support of Pt Single Atoms for Photocatalytic H2 Evolution
Zhuang, J.-D., Ren, S.-M., Zhu, B., Han, C., Li, Y., Zhang, X.-X., Gao, H.-L., Fan, M., & Tian, Q.-F. (2022) · Social Science Research Network · doi:10.2139/ssrn.4065675 · Cited by 83
P2-type layered high-entropy oxides as sodium-ion cathode materials
Wang, J., Dreyer, S. L., Wang, K., Ding, Z., Diemant, T., Karkera, G., Ma, Y.-J., Sarkar, A., Zhou, B., Gorbunov, M., et al. (2022) · Materials Futures · doi:10.1088/2752-5724/ac8ab9 · Cited by 81
Self-citation
Plasmon Assisted Highly Efficient Visible Light Catalytic CO2 Reduction Over the Noble Metal Decorated Sr-Incorporated g-C3N4
Humayun, M., Ullah, H., Shu, L., Ao, X., Tahir, A., Wang, C.-P., & Luo, W. (2021) · Nano-Micro Letters · doi:10.1007/s40820-021-00736-x · Cited by 79
Entropy engineering activation of UiO-66 for boosting catalytic transfer hydrogenation
Ma, M.-S., Chen, E.-P., Yue, H.-J., Tian, G., & Feng, S.-H. (2025) · Nature Communications · doi:10.1038/s41467-024-52225-5 · Cited by 76
“The unique composition provides not only a wide range of combinations for materials discovery, but also a distinctive microstructure for property optimization 3 .”
High-entropy electromagnetic functional materials: From electromagnetic genes to materials design
Liu, T., Li, L.-Y., Gao, P., Li, L., & Cao, M.-S. (2025) · Materials science & engineering. R, Reports · doi:10.1016/j.mser.2025.100982 · Cited by 74
A review on the rational design and fabrication of nanosized high-entropy materials
Zhou, Y., Shen, X., Qian, T., Yan, C., & Lu, J. (2023) · Nano Research · doi:10.1007/s12274-023-5419-2 · Cited by 103
Layered Oxygen-Deficient Double Perovskites as Promising Cathode Materials for Solid Oxide Fuel Cells
Klyndyuk, A., Chizhova, E., Kharytonau, D., & Medvedev, D. (2021) · Materials · doi:10.3390/ma15010141 · Cited by 74
“(or occasionally four) constituting elements [49,50].”
Background
High-entropy FeCoNiMn (oxy)hydroxide as high-performance electrocatalyst for OER and boosting clean carrier production under quasi-industrial condition
He, L., Wang, N., Sun, B., Li, Z., Yao, M., Hu, W., & Komarneni, S. (2022) · Journal of Cleaner Production · doi:10.1016/j.jclepro.2022.131680 · Cited by 85
Two-dimensional single-crystalline mesoporous high-entropy oxide nanoplates for efficient electrochemical biomass upgrading
Wang, Y., He, H., Lv, H., Jia, F., & Liu, B. (2024) · Nature Communications · doi:10.1038/s41467-024-50721-2 · Cited by 82
“On the other hand, high-entropy oxides (HEOs), which are composed of at least ﬁ ve transition metals arranged in a single-phase solid solution with homogeneous yet random distributions, have received more attention than ever compared to their monometallic counterparts 35 – 41 .”
High entropy energy storage materials: Synthesis and application
Ma, J., & Huang, C. (2023) · Journal of Energy Storage · doi:10.1016/j.est.2023.107419 · Cited by 87
High-entropy doping strategy towards reinforced Mn-O bond for durable aqueous zinc ion batteries
Jia, H., Li, Y.-X., Ali, U., Liu, B.-Q., Jin, Z., Li, L., Chen, Y.-N., Zhang, L.-Y., Wang, T.-T., & Wang, C.-G. (2024) · Nano Energy · doi:10.1016/j.nanoen.2024.109348 · Cited by 66
Structurally ordered high‐entropy intermetallic nanoparticles with enhanced C–C bond cleavage for ethanol oxidation
Wang, D., Chen, Z., Wu, Y., Huang, Y.-C., Tao, L., Chen, J., Dong, C.-L., Singh, C., & Wang, S.-Y. (2022) · SmartMat · doi:10.1002/smm2.1117 · Cited by 65
“High‐entropy alloys (HEAs), as the most representative high‐entropy materials (HEMs), have become a research hotspot in the field of metallic materials and catalysis due to their unprecedented composition and unique physical and chemical properties.(15,16) HEAs usually contain five or more principal elements, which pr…”
Background
Phase transformations in an Aurivillius layer structured ferroelectric designed using the high entropy concept
Zhang, M., Xu, X.-Z., Ahmed, S., Yue, Y., Palma, M., Švec, P., Gao, F., Abrahams, I., Reece, M., & Yan, H.-X. (2022) · Acta Materialia · doi:10.1016/j.actamat.2022.117815 · Cited by 65
Multi-elemental doping modulated P2-type layered cathodes for high performance sodium-ion batteries
Feng, G.-S., Gao, L., Li, J., Zhang, C.-K., Wu, Y., Tan, M., Wang, Q., Lv, F., Tao, L.-J., & Cao, M.-L. (2025) · Journal of Alloys and Compounds · doi:10.1016/j.jallcom.2025.179926 · Cited by 61
Self-citation
Generative learning facilitated discovery of high-entropy ceramic dielectrics for capacitive energy storage
Li, W., Shen, Z., Liu, R., Chen, X., Guo, M., Guo, J.-M., Hao, H., Shen, Y., Liu, H., Chen, L., et al. (2024) · Nature Communications · doi:10.1038/s41467-024-49170-8 · Cited by 73
“Recently, high-entropy strategy 10,11 with local disorder have been proposed to enhance energy storage performance by modulating the mutual constraints among P m , P r, and E b 10,12 .”
High-entropy spinel (FeCoNiMnAl)3O4 with three-dimensional microflower structure for stable seawater oxidation
Feng, C., Zhou, Y., Chen, M., Zou, L., Li, X., An, X., Zhao, Q., Xiaokaiti, P., Abudula, A., Yan, K., et al. (2024) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2024.123875 · Cited by 71
Solid-state hydrogen storage alloys for production-storage and transportation-application coupling at ambient temperature: A review
Tu, J., Zhou, P., Chen, S., Shen, S., Liu, X., Xiao, X., Li, Z., & Ouyang, L. (2025) · Materials Science and Engineering R Reports · doi:10.1016/j.mser.2025.101089 · Cited by 57
Coupling high entropy oxide with hollow carbon spheres by rapid microwave solvothermal strategy for boosting oxygen evolution reaction
He, H., Kou, P., Zhang, Z., Wang, D., Zheng, R., Sun, H., Liu, Y., & Wang, Z. (2023) · Journal of Colloid and Interface Science · doi:10.1016/j.jcis.2023.09.063 · Cited by 73
Active cation-integration high-entropy Prussian blue analogues cathodes for efficient Zn storage
Xing, J., Zhang, Y., Jin, Y., & Jin, Q. (2022) · Nano Reseach · doi:10.1007/s12274-022-5020-0 · Cited by 57
Review: High-Entropy Materials for Lithium-Ion Battery Electrodes
Sturman, J. W., Baranova, E., & Abu-Lebdeh, Y. (2022) · Frontiers in Energy Research · doi:10.3389/fenrg.2022.862551 · Cited by 57
Improved tribological behavior of plasma-nitrided AlCrTiV and AlCrTiVSi high-entropy alloy films
Cai, Z.-B., Wang, Z.-Y., Hong, Y., Lu, B.-W., Liu, J., Li, Y., & Pu, J. (2021) · doi:10.1016/j.triboint.2021.107195 · Cited by 57
Maximizing interface stability in all-solid-state lithium batteries through entropy stabilization and fast kinetics
Kong, X., Gu, R., Jin, Z., Zhang, L., Zhang, C., Xiang, W., Li, C., Zhu, K., Xu, Y., Huang, H., et al. (2024) · Nature Communications · doi:10.1038/s41467-024-51123-0 · Cited by 62
“Due to the unique entropy effects 30 – 32 , high-entropy materials have the potential to achieve a balance between chemical stability (high T stable ) and wettability (low T wetting ).”
High-Entropy Polyanionic Lithium Superionic Conductors
Strauss, F., Lin, J., Duffiet, M., Wang, K., Zinkevich, T., Hansen, A.-L., Indris, S., & Brezesinski, T. (2022) · ACS Materials Letters · doi:10.1021/acsmaterialslett.1c00817 · Cited by 56
Self-citation
Compositionally Complex Perovskite Oxides for Solar Thermochemical Water Splitting
Zhang, D., Santiago, H. A. D., Xu, B., Liu, C., Trindell, J. A., Li, W., Park, J., Rodriguez, M. A., Coker, E. N., Sugar, J. D., et al. (2023) · Chemistry of Materials · doi:10.1021/acs.chemmater.2c03054 · Cited by 68
Engineering high-entropy materials for electrocatalytic water splitting
Yang, X., Guo, R., Cai, R., Ouyang, Y., Yang, P., & Xiao, J. (2022) · International Journal of Hydrogen Energy · doi:10.1016/j.ijhydene.2022.02.123 · Cited by 66
High-entropy oxides as energy materials: from complexity to rational design
Yang, Z., Xiang, X., Yang, J. P., & Zhao, Z. (2024) · Materials Futures · doi:10.1088/2752-5724/ad8463 · Cited by 57
“For example, electrode materials used in SOFCs must endure high temperatures and mechanical stresses [127].”
Recent advances of high‐entropy electrocatalysts for water electrolysis by electrodeposition technology: a short review
Zhang, H.-M., Zhang, S., Zuo, L., Li, J., Guo, J., Wang, P., Sun, J., & Dai, L. (2024) · Rare Metals · doi:10.1007/s12598-024-02619-7 · Cited by 73
“Also, high-entropy materials have shown great promising applications in many ﬁelds, such as thermoelectric, magne-tocaloric, superconducting materials, catalysis and energy storage [39, 47–49].”
The concept of high entropy for rechargeable batteries
Li, H., Sun, X. A., & Huang, H. (2024) · Progress in Materials Science · doi:10.1016/j.pmatsci.2024.101382 · Cited by 58
Self-reconstruction of (CoNiFeCuCr)Se high-entropy selenide for efficient oxygen evolution reaction
Jiang, Z., Yuan, Y., Tan, L., Li, M., & Peng, K. C. (2023) · Applied Surface Science · doi:10.1016/j.apsusc.2023.157282 · Cited by 60
Research progresses in O3-type Ni/Fe/Mn based layered cathode materials for sodium ion batteries
Zhao, S., Shi, Q.-H., Feng, W.-L., Liu, Y., Yang, X.-X., Zou, X.-L., Lu, X.-G., & Zhao, Y. (2023) · Carbon Neutrality · doi:10.1007/s43979-023-00053-9 · Cited by 51
High-Entropy Amorphous Catalysts for Water Electrolysis: A New Frontier
Wang, G., Chen, Z., Zhu, J., Xie, J., Wei, W., Yan, Y., & Ni, B. (2025) · Nano-Micro Letters · doi:10.1007/s40820-025-01936-5 · Cited by 54
“Additionally, lattice distortion arising from atomic size mismatches induces local strain and electronic perturbations, thereby enhancing the adsorption of reaction intermediates [9, 24].”
The understanding, rational design, and application of high-entropy alloys as excellent electrocatalysts: A review
Zhou, Y., Shen, X.-W., Wang, M., Zhang, L.-F., Qian, T., Yan, C., & Lu, J. (2023) · Science China Materials · doi:10.1007/s40843-022-2436-6 · Cited by 50
High-entropy alloy catalysts: high-throughput and machine learning-driven design
Chen, L., Chen, Z., Yao, X., Su, B., Chen, W., Pang, X., Kim, K.-S., Singh, C. V., & Zou, Y. (2022) · Journal of Materials Informatics · doi:10.20517/jmi.2022.23 · Cited by 59
More Disorder is Better: Cutting-Edge Progress of High Entropy Materials in Electrochemical Energy Storage Applications
Bao, C., Chu, P., Xu, C.-X., Yuan, J., Si, L.-J., Bo, Z., Ostrikov, K., & Yang, H.-C. (2024) · Energy Storage Materials · doi:10.1016/j.ensm.2024.103408 · Cited by 49
Facile synthesis of high-entropy (Co0.2Cr0.2Fe0.2Mn0.2Ni0.2)3O4 nanopowders and their electrochemical properties as supercapacitor electrode
Li, L., Ji, P.-C., Geng, C., Li, Y., Meng, L., Zhou, B., Liang, J., Peng, J.-H., & Su, X. (2023) · Journal of Energy Storage · doi:10.1016/j.est.2023.109182 · Cited by 49
Exploring B-Site High-Entropy Configuration of Spinel Oxides for Improved Cathode Performance in Solid Oxide Fuel Cells
Lin, Z., Ma, B., Chen, Z.-H., Cheng, L., & Zhou, Y. (2023) · Journal of the European Ceramic Society · doi:10.1016/j.jeurceramsoc.2023.11.004 · Cited by 49
A perspective on high‐entropy two‐dimensional materials
Cui, Y., Zhang, Y.-Z., Cao, Z., Gu, J., Du, Z.-G., Li, B., & Yang, S.-B. (2022) · SusMat · doi:10.1002/sus2.47 · Cited by 49
High-entropy two-dimensional metal phosphorus trichalcogenides boost high-performance potassium ion storage devices via electrochemical reconstruction
Chien, P.-W., Chang, C.-B., & Tuan, H.-Y. (2023) · Energy Storage Materials · doi:10.1016/j.ensm.2023.102853 · Cited by 47
“…S ≧ 1.5 R are classified as high-entropy, while materials with 1.0 R ≦ Δ S ≦ 1.5 R and Δ S 1.0 R are classified as medium-entropy and low-entropy [24], respectively, calculated by the formula of Δ S = (cid:0) R ∑ ni = 1 x i lnx i , where R is the ideal gas constant, and x i represents the mole…”
Influential
Enhancing electrocatalytic performance in the oxygen evolution reaction of zirconium-based amorphous high-entropy oxides via controlled introduction of oxygen vacancies: experimental insights and DFT simulations.
Zhang, X., Xu, R., Wang, T., Niu, L.-Y., Gong, Y.-Y., & Li, C. (2025) · Journal of Colloid and Interface Science · doi:10.1016/j.jcis.2025.137635 · Cited by 46
High-Entropy Strategy for Electrochemical Energy Storage Materials
Ding, F.-X., Lu, Y.-X., Chen, L.-Q., & Hu, Y.-S. (2024) · Electrochemical Energy Reviews · doi:10.1007/s41918-024-00216-x · Cited by 46
“1a), while materials with S conf ⩽ 1.0 R are classified as low-entropy materials, with materials that fall between these two extremes being classified as medium-entropy materials [5, 8–10].”
Influential
Enhancement of piezo–photocatalytic activity in perovskite (Bi0·2Na0·2Ba0·2K0·2La0.2)TiO3 oxides via high entropy induced lattice distortion and energy band reconfiguration
Fu, H.-X., Li, S., Lin, Y., Wu, X., Lin, T.-F., Zhao, C.-L., Gao, M., & Lin, C. (2023) · Ceramics International · doi:10.1016/j.ceramint.2023.12.232 · Cited by 46
Enhanced energy storage properties of (Bi0.2Na0.2Ca0.2Ba0.2Sr0.2)(Ti1-Zr )O3 high entropy ceramics by Zr doping at B-site
Niu, Y., Zhang, F., Zhang, X., Zhang, Z., Bai, Y., & Wang, Z.-J. (2023) · Ceramics International · doi:10.1016/j.ceramint.2023.10.097 · Cited by 46
A medium-entropy perovskite oxide La0.7Sr0.3Co0.25Fe0.25Ni0.25Mn0.25O3-δ as intermediate temperature solid oxide fuel cells cathode material
Li, X., Shi, C., Zhang, G.-J., Zheng, G.-Z., Huang, Z.-Z., Shen, X.-S., Zhou, J., Chen, T., & Wang, S.-R. (2023) · Ceramics International · doi:10.1016/j.ceramint.2023.06.275 · Cited by 46
Activating multisite high-entropy alloy nanocrystals via enriching M–pyridinic N–C bonds for superior electrocatalytic hydrogen evolution
Wang, J., Zhang, J., Hu, Y., Jiang, H., & Li, C. (2022) · 中国科学通报：英文版 · doi:10.1016/j.scib.2022.08.022 · Cited by 60
Design of advanced electrocatalysts for the high-entropy alloys: Principle, progress, and perspective
He, B., Zu, Y., & Mei, Y. (2023) · Journal of Alloys and Compounds · doi:10.1016/j.jallcom.2023.170479 · Cited by 50
Designing strategies and enhancing mechanism for multicomponent high-entropy catalysts
Xu, H., Jin, Z., Zhang, Y., Lin, X., Xie, G., Liu, X., & Qiu, H. (2023) · Chemical Science · doi:10.1039/d2sc06403k · Cited by 86
A solution-based route to compositionally complex metal oxide structures using high-entropy layered double hydroxides
Kim, M., Oh, I., Choi, H., Jang, W.-Y., Song, J., Kim, C., Yoo, J.-W., & Cho, S. (2021) · Cell Reports Physical Science · doi:10.1016/j.xcrp.2021.100702 · Cited by 45
Innovative High‐Entropy Strategy Extending Traditional Metal Substitution for Optimizing Prussian Blue Analogues in Rechargeable Batteries
Zhou, Z., Dong, Y., Ma, Y., Zhang, H., Meng, F., Ma, Y., & Wu, Y. (2025) · SusMat · doi:10.1002/sus2.265 · Cited by 49
“In addition to the aforementioned definition based on configu-rational entropy, the second classification designates materials as “high-entropy” when they incorporate a minimum of five elements within a single lattice, with atomic concentrations ranging between 5 and 35% [48].”
Self-citation
Amorphous high-entropy IrRuCrFeCoNiOx as efficient water splitting oxygen evolution reaction electrocatalysts
Rong, W., Chen, Y., Dang, R., Huang, K., Xia, J., Zhang, B., Liu, J., Meng, H., Cao, Q., & Wu, J. (2023) · Journal of Alloys and Compounds · doi:10.1016/j.jallcom.2023.172786 · Cited by 52
High entropy materials frontier and theoretical insights for logistics CO2 reduction and hydrogenation: Electrocatalysis, photocatalysis and thermo-catalysis
Shaikh, J. S., Rittiruam, M., Saelee, T., Márquez, V., Shaikh, N. S., Khajondetchairit, P., Pathan, S. C., Jiraborvornpongsa, N., Praserthdam, S., & Praserthdam, P. (2023) · Journal of Alloys and Compounds · doi:10.1016/j.jallcom.2023.172232 · Cited by 53
Stabilization strategies for high-capacity NCM materials targeting for safety and durability improvements
Meng, J., Qu, G., & Huang, Y. (2023) · eTransportation · doi:10.1016/j.etran.2023.100233 · Cited by 51
Cluster expansions of multicomponent ionic materials: Formalism and methodology
Barroso-Luque, L., Zhong, P., Yang, J. H., Xie, F., Chen, T., Ouyang, B., & Ceder, G. (2022) · Physical review. B./Physical review. B · doi:10.1103/physrevb.106.144202 · Cited by 50
“Typical examples of such complex ionic systems include the recently discovered class of disordered rocksalts (DRX) [12,13], partially disordered spinels (PDSs) [14,15], and high-entropy perovskites [16], among many other promising multicomponent ceramic materials [17,18].”
Background
Synthetic Strategies toward High Entropy Materials: Atoms-to-Lattices for Maximum Disorder
Buckingham, M. A., Skelton, J., & Lewis, D. J. (2023) · Crystal Growth & Design · doi:10.1021/acs.cgd.3c00712 · Cited by 40
Effect of La substitution on energy storage properties of (Bi0.2Na0.2Ca0.2Ba0.2Sr0.2)TiO3 lead‐free high‐entropy ceramics
Zhang, X., Zhang, F., Niu, Y., Zhang, Z., Bai, Y., & Wang, Z.-J. (2023) · Journal of The American Ceramic Society · doi:10.1111/jace.19270 · Cited by 40
Spinel-type high-entropy (Co0.2Mn0.2Fe0.2Zn0.2Ti0.2)3O4 oxides constructed from disordered cations and oxygen vacancies
Wang, B., Yao, J.-C., Wang, J., & Chang, A.-M. (2022) · Journal of Alloys and Compounds · doi:10.1016/j.jallcom.2021.163188 · Cited by 39
A review of high-entropy alloys for next-generation solid-state advanced hydrogen storage materials
Gao, S., Qi, J., Jia, K. W., Zhang, L., Wu, F., & Xiao, X. (2025) · Composites Part B Engineering · doi:10.1016/j.compositesb.2025.113340 · Cited by 40
Research progress on P2-type layered oxide cathode materials for sodium-ion batteries
Wu, C., Xu, Y.-X., Song, J., Hou, Y., Jiang, S., He, R., Wei, A., & Tan, Q.-Q. (2024) · Chemical Engineering Journal · doi:10.1016/j.cej.2024.157264 · Cited by 38
The emerging high-entropy cathode materials for advanced Na-ion batteries: advances and perspectives
Hou, P., Gong, M.-L., Dong, M., Lin, Z.-Z., Huang, J.-Z., Zhang, H.-Z., & Li, F. (2024) · Energy Storage Materials · doi:10.1016/j.ensm.2024.103750 · Cited by 37
Photocatalytic degradation performance for high-entropy oxide (La0.2Ce0.2Gd0.2Zr0.2Fex)O2 enriched with defects
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Authors: Ma, Y., Ma, Y., Wang, Q., Schweidler, S., Botros, M., Fu, T., Hahn, H., Brezesinski, T., & Breitung, B.
Affiliations: Karlsruhe Institute of Technology (DE)
University of Waterloo (CA)
Corresponding author: Ma, Yanjiao
Brezesinski, Torsten
Breitung, Ben
ORCID: Ma, Yanjiao
Ma, Yuan
Wang, Qingsong
Schweidler, Simon
Botros, Miriam
Fu, Tongtong
Hahn, Horst
Brezesinski, Torsten
Breitung, Ben
Venue: Energy & Environmental Science
Publisher: Royal Society of Chemistry (RSC)
Published: 2021
Volume: 14
Issue: 5
Pages: 2883-2905
ISSN: 1754-5692 (ISSN-L)
1754-5706
DOI: 10.1039/d1ee00505g
OpenAlex: W3148416643
Cited by: 963
References: 186
Citations by year: 2026: 187 · 2025: 262 · 2024: 263 · 2023: 137 · 2022: 87 · 2021: 27
FWCI: 54.92
Type: journal article
Language: en
Open access: hybrid
doi.org
Licence: cc-by-nc
creativecommons.org/licenses/by-nc/3.0/ (vor, 91 d)
Locations: Energy & Environmental Science (publishedVersion, cc-by-nc)
Repository KITopen (Karlsruhe Institute of Technology) (publishedVersion, cc-by-nc-nd)
ERef Bayreuth (University of Bayreuth) (submittedVersion)
Zenodo (CERN European Organization for Nuclear Research) (submittedVersion, cc-by)
KITopen
Funders: Deutsche Forschungsgemeinschaft (BR 3499/5-1, HA 1344/43-1, SE 1407/4-2)
Carl-Zeiss-Stiftung
Helmholtz Association
Horizon 2020 (730957, 101017709)
Topics: Physical Sciences › Engineering › Mechanical Engineering › High Entropy Alloys Studies
Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Physical Sciences › Materials Science › Materials Chemistry › Machine Learning in Materials Science
Keywords: high-entropy materials, hydrogen catalysis, hydrogen storage, CO2 conversion, oxygen catalysis, electrochemical energy storage, energy materials

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High-entropy energy materials: challenges and new opportunities

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